Theoretical Study on Near-Resonant Third-Order Nonlinear Optical Properties (γ) of Dendritic Molecular Aggregates: Intermolecular-Interaction and Relaxation Effects on γ
H. Fujita, M. Nakano, M. Takahata, S. Kiribayashi, K. Yamaguchi
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Abstract
Abstract Second hyperplarizability (γ) of dendritic molecular aggregate (D25) is calculated using a coupled-dipole model in the Markoff approximation. At the near resonant region, intermolecular-interaction and relaxation effects on γ are found to remarkably change the γ value.
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