Synthesis strategies of metal-organic frameworks for CO2 capture

IF 3.3 3区 物理与天体物理 Q2 PHYSICS, CONDENSED MATTER Superlattices and Microstructures Pub Date : 2023-08-10 DOI:10.20517/microstructures.2023.32
Meng Sun, Xiaokang Wang, Fei Gao, Mingming Xu, Weidong Fan, Ben Xu, Daofeng Sun
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引用次数: 1

Abstract

The high consumption of fossil energy has led to increasing concentrations of carbon dioxide (CO2) in the atmosphere, making carbon capture and separation a research hotspot in this century. As novel porous materials, metal-organic frameworks (MOFs) are widely used for CO2 capture due to their unique structures and tunable properties. Currently, several relatively mature strategies have been applied to synthesize MOFs for CO2 capture. Herein, we investigate strategies for tuning the pore windows, pore sizes, open metal sites, and post-synthesis or pre-synthesis modifications of MOFs from the perspective of CO2 capture performance. Furthermore, we summarize the relevant CO2 capture technologies and research advances and describe the application of different strategies in the synthesis of CO2 capture-oriented MOFs.
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二氧化碳捕获金属-有机框架的合成策略
化石能源的大量消耗导致大气中二氧化碳浓度增加,使碳捕获与分离成为本世纪的研究热点。金属有机骨架(MOFs)作为一种新型多孔材料,因其独特的结构和可调的性能而被广泛应用于二氧化碳捕集。目前,几种相对成熟的策略已经应用于合成用于CO2捕集的mof。在此,我们从CO2捕获性能的角度研究了调整mof的孔窗、孔径、开放金属位点以及合成后或合成前修饰的策略。在此基础上,总结了CO2捕集相关技术和研究进展,并介绍了不同策略在CO2捕集型mof合成中的应用。
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来源期刊
Superlattices and Microstructures
Superlattices and Microstructures 物理-物理:凝聚态物理
CiteScore
6.10
自引率
3.20%
发文量
35
审稿时长
2.8 months
期刊介绍: Micro and Nanostructures is a journal disseminating the science and technology of micro-structures and nano-structures in materials and their devices, including individual and collective use of semiconductors, metals and insulators for the exploitation of their unique properties. The journal hosts papers dealing with fundamental and applied experimental research as well as theoretical studies. Fields of interest, including emerging ones, cover: • Novel micro and nanostructures • Nanomaterials (nanowires, nanodots, 2D materials ) and devices • Synthetic heterostructures • Plasmonics • Micro and nano-defects in materials (semiconductor, metal and insulators) • Surfaces and interfaces of thin films In addition to Research Papers, the journal aims at publishing Topical Reviews providing insights into rapidly evolving or more mature fields. Written by leading researchers in their respective fields, those articles are commissioned by the Editorial Board. Formerly known as Superlattices and Microstructures, with a 2021 IF of 3.22 and 2021 CiteScore of 5.4
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