Study on the synthesis of g-C3N4/CoFe2O4/Reduced graphene oxide material and its application as photocatalyst

Tram Pham Thi Le, Ha Nguyen Thi, Hoang Do Thi Phuong, Huy Nguyen Minh, Minh Nguyen Ngoc, Phuong Diep Thi Lan, Phuong Tran Thi Thu, Nghia Nguyen Thi, Thanh Huynh Thi Minh, Linh Bui Thi Ngoc, Thien Nguyen Duc, Hoan Nguyen Thi Vuong
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Abstract

In this study, the g-C3N4/CoFe2O4/Reduced graphene oxide composites were successfully synthesized by the co-precipitation method combined with mixed phase mixture. The obtained results from characterization methods such as XRD, SEM, FT-IR, EDX,… showed that the composite has a high structure and crystallinity, and spinel ferrite particles were dispersed fairly evenly onto reduced graphene oxide sheets as well as layers of g-C3N4. The existence of Co/Fe-O and Co-O-C bonds in materials was determined. The photocatalytic activity of g-C3N4/CoFe2O4/Reduced graphene oxide (GCN/CF-rGO) was estimated through the degradation of Tetracycline (TC) in aqueous solution. TC decomposition efficiency is up to 95% after 240 minutes of reaction and is higher than that of each component material. GCN/CF-rGO is a potential catalyst for effective application in TC decomposition reaction under visible light and has the ability to implement treatment in practice.
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g-C3N4/CoFe2O4/还原性氧化石墨烯材料的合成及其光催化剂应用研究
本研究采用共沉淀法结合混合相混合物成功合成了g-C3N4/CoFe2O4/还原氧化石墨烯复合材料。XRD、SEM、FT-IR、EDX等表征方法表明,该复合材料具有较高的结构和结晶度,尖晶石铁素体颗粒均匀地分散在还原氧化石墨烯片和g-C3N4层上。测定了材料中Co/Fe-O和Co- o- c键的存在。研究了g-C3N4/CoFe2O4/还原性氧化石墨烯(GCN/CF-rGO)对四环素(TC)的光催化活性。反应240分钟后,TC分解效率可达95%以上,高于各组分物料的分解效率。GCN/CF-rGO是一种有潜力有效应用于可见光下TC分解反应的催化剂,具有在实践中实施处理的能力。
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