流体动力空化反应器的建模:现状与展望

IF 4.3 Q2 ENGINEERING, CHEMICAL ACS Engineering Au Pub Date : 2022-07-22 DOI:10.1021/acsengineeringau.2c00025
Vivek V. Ranade*, 
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引用次数: 4

摘要

流体动力空化(HC)在水、能源、化工和材料等领域的应用越来越广泛。HC产生强烈的剪切,局部热点和羟基自由基,这些被用来实现所需的物理化学转化。尽管将HC确定为最有前途的技术平台之一,但其潜力尚未在实践中得到充分转化。缺乏设计、优化和扩大HC反应器的适当模型是造成这种情况的主要原因之一。本文介绍了HC反应器的建模现状。各种流行的方法,包括经验,现象学和多尺度模型,严格审查在其应用的个人经验的光。简要讨论了这些方法在生物质预处理和废水处理等不同应用中的应用。对将这些模型扩展到乳液和结晶等其他应用的一些评论也包括在内。所提出的模型和讨论将有助于有兴趣将HC应用于各种应用的实践工程师和科学家。最后对HC反应器建模的进一步发展提出了一些看法和展望,以期对提高HC反应器计算模型保真度的进一步研究有所启发。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

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Modeling of Hydrodynamic Cavitation Reactors: Reflections on Present Status and Path Forward

Hydrodynamic cavitation (HC) is finding ever increasing applications in water, energy, chemicals, and materials sectors. HC generates intense shear, localized hot spots, and hydroxyl radicals, which are harnessed for realizing desired physicochemical transformations. Despite identification of HC as one of the most promising technology platforms, its potential is not yet adequately translated in practice. Lack of appropriate models for design, optimization, and scale-up of HC reactors is one of the primary reasons for this. In this work, the current status of modeling of HC reactors is presented. Various prevailing approaches covering empirical, phenomenological, and multiscale models are critically reviewed in light of personal experience of their application. Use of these approaches for different applications such as biomass pretreatment and wastewater treatment is briefly discussed. Some comments on extending these models for other applications like emulsions and crystallization are included. The presented models and discussion will be useful for practicing engineers and scientists interested in applying HC for a variety of applications. Some thoughts on further advances in modeling of HC reactors and outlook are shared, which may stimulate further research on improving the fidelity of computational models of HC reactors.

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ACS Engineering Au
ACS Engineering Au 化学工程技术-
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期刊介绍: )ACS Engineering Au is an open access journal that reports significant advances in chemical engineering applied chemistry and energy covering fundamentals processes and products. The journal's broad scope includes experimental theoretical mathematical computational chemical and physical research from academic and industrial settings. Short letters comprehensive articles reviews and perspectives are welcome on topics that include:Fundamental research in such areas as thermodynamics transport phenomena (flow mixing mass & heat transfer) chemical reaction kinetics and engineering catalysis separations interfacial phenomena and materialsProcess design development and intensification (e.g. process technologies for chemicals and materials synthesis and design methods process intensification multiphase reactors scale-up systems analysis process control data correlation schemes modeling machine learning Artificial Intelligence)Product research and development involving chemical and engineering aspects (e.g. catalysts plastics elastomers fibers adhesives coatings paper membranes lubricants ceramics aerosols fluidic devices intensified process equipment)Energy and fuels (e.g. pre-treatment processing and utilization of renewable energy resources; processing and utilization of fuels; properties and structure or molecular composition of both raw fuels and refined products; fuel cells hydrogen batteries; photochemical fuel and energy production; decarbonization; electrification; microwave; cavitation)Measurement techniques computational models and data on thermo-physical thermodynamic and transport properties of materials and phase equilibrium behaviorNew methods models and tools (e.g. real-time data analytics multi-scale models physics informed machine learning models machine learning enhanced physics-based models soft sensors high-performance computing)
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