Comparing the impacts of ozone-depleting substances and carbon dioxide on Arctic sea ice loss

The rapid decline of Arctic sea ice is widely believed to be a consequence of increasing atmospheric concentrations of greenhouse gases (GHGs). While carbon dioxide (CO2) is the dominant GHG contributor, recent work has highlighted a substantial role for ozone-depleting substances (ODS) in Arctic sea ice loss. However, a careful analysis of the mechanisms and relative impacts of CO2 versus ODS on Arctic sea ice loss has yet to be performed. This study performs this comparison over the period 1955–2005 when concentrations of ODS increased rapidly, by analyzing a suite of all-but-one-forcing ensembles of climate model integrations, designed to isolate the forced response to individual forcing agents in the context of internal climate variability. We show that ODS have played a significant role in year-round Arctic sea ice extent and volume trends over that period, accounting for 64% and 32% of extent and volume trends, respectively. These impacts represent 50% and 38% of the impact from CO2 forcing, respectively. We find that ODS act via similar physical processes to CO2, causing sea ice loss via increased summer melt, and not sea ice dynamics changes. These findings imply that the future trajectory of ODS emissions will play an important role in future Arctic sea ice evolution.