分裂和延迟完全相干的自由电子激光器脉冲推进超快x射线科学:费米自由电子激光器的交流/直流光学装置

A. Simoncig, M. Manfredda, G. Gaio, N. Mahne, L. Raimondi, C. Fava, S. Gerusina, R. Gobessi, A. Abrami, F. Capotondi, D. De Angelis, R. Menk, M. Pancaldi, E. Pedersoli, M. Zangrando
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摘要

自由电子激光器(FELs)是目前世界上最先进的光源,由于它们具有激光相干超短脉冲的能力,其标志是光子能量弥合了极紫外(EUV)和软(SXR)和硬(HXR) x射线之间的差距,同时具有独特的高亮度和飞秒(fs)时间尺度的持续时间。FELs可以利用时间分辨的方法,利用同步加速器光源中日常使用的光谱,主要是将EUV、SXR和HXR脉冲与光学脉冲结合起来。尽管如此,超快x射线科学的下一个进展与这些时间分辨方案的扩展密切相关,以执行专门从事EUV, SXR和HXR脉冲的实验,从而触发(和探测)其(或附近)电子共振的物质,揭示隐藏在宽带应用主要感兴趣的物质相背后的微观机制。事实上,设计下一代量子器件,以及为药理学应用定制新型生物分子,只是两个例子,可以通过这种光学方法得到强有力的推动。要做到这一点,必须在不影响辐射相干性和光子传输的情况下,对FELs脉冲进行分裂和延迟(及时)。在种子FERMI FEL(意大利的里雅斯特),这个目标是由被称为AC/DC的光学设备实现的,AC/DC代表自动相关器/延迟创造者,设计用于分割传入的EUV和/或SXR脉冲,在这两个脉冲之间引入可调延迟,以子fs的固有分辨率为标志,并由光学数字指向反馈系统辅助。
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Splitting and delaying fully coherent FELs pulses for advancing ultrafast x-ray science: the AC/DC optical device at the FERMI FEL
Free-electron lasers (FELs) are currently the most advanced light sources operating worldwide, thanks to their capability to lase coherent ultrashort pulses, marked by photon energies bridging the gap between the Extreme-Ultraviolet (EUV) and the Soft (SXR) and Hard (HXR) X-Rays, alongside with unique high-brightness and temporal duration lying in the femtosecond (fs) timescale. FELs can exploit, in a time-resolved approach, spectroscopies daily employed at synchrotron light sources, mostly combining EUV, SXR and HXR pulses with optical ones. Nonetheless, the next advances in ultrafast x-Ray science are strongly linked to the extension of these time-resolved schemes to perform experiments engaging exclusively EUV, SXR and HXR pulses, so triggering (and probing) matter at its (or nearby) electronic resonance(s), to reveal the microscopic mechanisms hiding behind matter phases of primary interest for broadband applications. Indeed, designing the next generation of quantum devices, as well as tailoring a new classes of biomolecules for pharmacological applications, are just two examples that can be strongly boosted by means of this optical approach. To do this, is mandatory to split and delay (in time) FELs pulses, without impacting on both the radiation coherence properties and on the photon transport. At the seeded FERMI FEL (Trieste, Italy) this goal is committed by the optical device known as AC/DC, which stands for the Auto Correlator/Delay Creator, designed to split the incoming EUV and/or SXR pulse, introducing a tunable delay between these two pulses, marked by an intrinsic resolution in the sub-fs, and aided by an opto-numerical pointing feedback system.
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