等离子体纳米锥点接触-绝缘体-金属结构的光整流

R. Mupparapu, J. Cunha, F. Tantussi, A. Jacassi, L. Summerer, M. Patrini, A. Giugni, A. Alabastri, R. Proietti Zaccaria
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摘要

最近已经进行了许多努力,以发展在高频率下工作的整流装置,特别是专门用于光收集和光探测应用。为此,已经实施了各种整流策略,例如激光诱导的STM隧道,金属-绝缘体-金属(MIM)行波二极管,等离子体纳米隙光学天线,天线二极管耦合平面MIM,以及MIM点接触尖端或晶须二极管。然而,开发高频整流天线(整流天线)仍然是一个主要的技术挑战,因为只有最近的进展才能制造出近红外和可见光频率的高效可调谐纳米天线。本文报道了一种基于等离子体载流子产生的新型整流天线。所提出的整流结构由宽谐振金锥形纳米尖端天线与金属氧化物/金属样品表面接触组成,形成点接触隧道二极管。纳米尺寸的天线顶端,旨在最大化表面等离子激元(SPPs)阻尼,允许从光场到费米能级以上的激发电荷的有效能量转换,后者可以通过电子隧道过程从点接触位置收集。我们演示了在280太赫兹下的整流操作,其功率转换效率比最先进的功率转换效率高一个数量级,我们将其归因于高效的等离子体载流子生成和收集。
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Light rectification with plasmonic nano-cone point contact-insulator-metal architecture
Numerous efforts have been recently undertaken towards the development of rectifying devices operating at high frequencies especially dedicated to light harvesting and photo detection applications. To this end various rectification strategies have been implemented, such as laser-induced STM tunneling, metal-insulator-metal (MIM) travelling wave diodes, plasmonic nanogap optical antennas, antenna-diode coupled planar MIM, and MIM point-contact sharp-tip or whisker diodes. However, developing high frequency rectifying antennas (rectennas) remains a major technological challenge, as only recent progresses enabled the fabrication of efficient tunable nano-antennas at near infrared and visible frequencies. Here we report on a new type of rectenna based on plasmonic carrier generation. The proposed rectifying structure consists of a broadly resonant gold conical nano-tip antenna in contact with a metal-oxide/metal sample surface, forming a point-contact tunneling diode. The nano-sized antenna apex, designed to maximize the Surface Plasmon Polaritons (SPPs) damping, allows for an efficient power conversion from the light field into excited charges above the Fermi level, the latter ones collectable from the point-contact location through an electronic tunneling process. We demonstrated rectification operation at 280 THz with a power conversion efficiency one order of magnitude higher than the state-of-the-art which we attribute to efficient plasmonic carrier generation and collection.
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