利用受控自氧化技术从低价值石油馏分中生产高价值产品的前景

IF 7 2区 化学 Q1 CHEMISTRY, MULTIDISCIPLINARY Chemical record Pub Date : 2024-04-17 DOI:10.1002/tcr.202400015
Muhammad N. Siddiquee
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引用次数: 0

摘要

在常规和非常规石油资源的升级和提炼过程中,会产生大量低价值的轻质石油馏分和低价值的重质石油馏分,如轻质石脑油、高纯度煤层气和真空残渣。石油工业强调经济多样化,旨在通过具有成本效益和可持续的方法从这些低石油馏分中生产出高价值产品。受控自氧化(空气氧化)有可能从低价值轻质石油馏分中生产出具有重要工业价值的含氧化合物,包括醇和酮。生成的醇还可以通过催化脱水转化为烯烃。在受控自氧化之后,低价值重质石油馏分可用于生产增值产品,包括碳纤维前体。这将降低高需求产品碳纤维的生产成本。本综述强调了开发一种替代性、可持续和经济的方法,通过受控自氧化方法从低价值石油馏分中生产增值产品的前景。
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Prospect of Controlled Autoxidation to Produce High-Value Products from the Low-Value Petroleum Fractions

Substantial amounts of low-value light petroleum fractions and low-value heavy petroleum fractions, such as light naphtha, HVGO, and vacuum residue, are generated during the upgrading and refining of conventional and unconventional petroleum resources. The oil industry emphasizes economic diversification, aiming to produce high-value products from these low petroleum fractions through cost-effective and sustainable methods. Controlled autoxidation (oxidation with air) has the potential to produce industrially important oxygenates, including alcohols, and ketones, from the low-value light petroleum fractions. The produced alcohols can also be converted to olefin through catalytic dehydration. Following controlled autoxidation, the low-value heavy petroleum fractions can be utilized to produce value-added products, including carbon fiber precursors. It would reduce the production cost of a highly demandable product, carbon fiber. This review highlights the prospect of developing an alternative, sustainable, and economic method to produce value-added products from the low-value petroleum fractions following a controlled autoxidation approach.

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来源期刊
Chemical record
Chemical record 化学-化学综合
CiteScore
11.00
自引率
3.00%
发文量
188
审稿时长
>12 weeks
期刊介绍: The Chemical Record (TCR) is a "highlights" journal publishing timely and critical overviews of new developments at the cutting edge of chemistry of interest to a wide audience of chemists (2013 journal impact factor: 5.577). The scope of published reviews includes all areas related to physical chemistry, analytical chemistry, inorganic chemistry, organic chemistry, polymer chemistry, materials chemistry, bioorganic chemistry, biochemistry, biotechnology and medicinal chemistry as well as interdisciplinary fields. TCR provides carefully selected highlight papers by leading researchers that introduce the author''s own experimental and theoretical results in a framework designed to establish perspectives with earlier and contemporary work and provide a critical review of the present state of the subject. The articles are intended to present concise evaluations of current trends in chemistry research to help chemists gain useful insights into fields outside their specialization and provide experts with summaries of recent key developments.
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