N. V. Kuzmenkova, V. G. Petrov, A. K. Rozhkova, E. A. Tokar, K. Shi, S. N. Kalmykov, X. Hou
{"title":"彼得大帝湾水、悬浮物和底层沉积物中镎、钚和镅的分布情况","authors":"N. V. Kuzmenkova, V. G. Petrov, A. K. Rozhkova, E. A. Tokar, K. Shi, S. N. Kalmykov, X. Hou","doi":"10.1134/S1066362224010156","DOIUrl":null,"url":null,"abstract":"<p>The content of <sup>237</sup>Np, <sup>239,240</sup>Pu, and <sup>241</sup>Am in seawater, suspended matter, and bottom sediment cores of the Ussuri and Amur Bays, sampled in July 2021 and August 2022, was analyzed. The activity concentrations of <sup>237</sup>Np, <sup>239,240</sup>Pu, and <sup>241</sup>Am in the water of Peter the Great Bay were determined for the first time and were found to be equal to (19–105) × 10<sup>–3</sup>, 2.0–5.3, and 24.1–33.5 mBq/m<sup>3</sup>, respectively. The activity concentrations as well as the <sup>239</sup>Pu/<sup>240</sup>Pu isotope ratio (⁓0.18) in the bottom sediments definitely indicate that global fallout is the main source of plutonium in the investigated territory. The sedimentation rates were determined for the Amur Bay (in the Razdolnaya River estuary), 0.9 mm/year, and for the Ussuri Bay, 4.1 mm/year. Actinide transfer coefficients were determined for Peter the Great Bay in the system dissolved forms (including colloids)–suspended matter–bottom sediment.</p>","PeriodicalId":747,"journal":{"name":"Radiochemistry","volume":"66 1","pages":"115 - 123"},"PeriodicalIF":0.9000,"publicationDate":"2024-04-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Distribution of Np, Pu, and Am in Water, Suspended Matter, and Bottom Sediments of Peter the Great Bay\",\"authors\":\"N. V. Kuzmenkova, V. G. Petrov, A. K. Rozhkova, E. A. Tokar, K. Shi, S. N. Kalmykov, X. Hou\",\"doi\":\"10.1134/S1066362224010156\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p>The content of <sup>237</sup>Np, <sup>239,240</sup>Pu, and <sup>241</sup>Am in seawater, suspended matter, and bottom sediment cores of the Ussuri and Amur Bays, sampled in July 2021 and August 2022, was analyzed. The activity concentrations of <sup>237</sup>Np, <sup>239,240</sup>Pu, and <sup>241</sup>Am in the water of Peter the Great Bay were determined for the first time and were found to be equal to (19–105) × 10<sup>–3</sup>, 2.0–5.3, and 24.1–33.5 mBq/m<sup>3</sup>, respectively. The activity concentrations as well as the <sup>239</sup>Pu/<sup>240</sup>Pu isotope ratio (⁓0.18) in the bottom sediments definitely indicate that global fallout is the main source of plutonium in the investigated territory. The sedimentation rates were determined for the Amur Bay (in the Razdolnaya River estuary), 0.9 mm/year, and for the Ussuri Bay, 4.1 mm/year. Actinide transfer coefficients were determined for Peter the Great Bay in the system dissolved forms (including colloids)–suspended matter–bottom sediment.</p>\",\"PeriodicalId\":747,\"journal\":{\"name\":\"Radiochemistry\",\"volume\":\"66 1\",\"pages\":\"115 - 123\"},\"PeriodicalIF\":0.9000,\"publicationDate\":\"2024-04-23\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Radiochemistry\",\"FirstCategoryId\":\"1085\",\"ListUrlMain\":\"https://link.springer.com/article/10.1134/S1066362224010156\",\"RegionNum\":0,\"RegionCategory\":null,\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q4\",\"JCRName\":\"CHEMISTRY, INORGANIC & NUCLEAR\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Radiochemistry","FirstCategoryId":"1085","ListUrlMain":"https://link.springer.com/article/10.1134/S1066362224010156","RegionNum":0,"RegionCategory":null,"ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q4","JCRName":"CHEMISTRY, INORGANIC & NUCLEAR","Score":null,"Total":0}
Distribution of Np, Pu, and Am in Water, Suspended Matter, and Bottom Sediments of Peter the Great Bay
The content of 237Np, 239,240Pu, and 241Am in seawater, suspended matter, and bottom sediment cores of the Ussuri and Amur Bays, sampled in July 2021 and August 2022, was analyzed. The activity concentrations of 237Np, 239,240Pu, and 241Am in the water of Peter the Great Bay were determined for the first time and were found to be equal to (19–105) × 10–3, 2.0–5.3, and 24.1–33.5 mBq/m3, respectively. The activity concentrations as well as the 239Pu/240Pu isotope ratio (⁓0.18) in the bottom sediments definitely indicate that global fallout is the main source of plutonium in the investigated territory. The sedimentation rates were determined for the Amur Bay (in the Razdolnaya River estuary), 0.9 mm/year, and for the Ussuri Bay, 4.1 mm/year. Actinide transfer coefficients were determined for Peter the Great Bay in the system dissolved forms (including colloids)–suspended matter–bottom sediment.
期刊介绍:
Radiochemistry is a journal that covers the theoretical and applied aspects of radiochemistry, including basic nuclear physical properties of radionuclides; chemistry of radioactive elements and their compounds; the occurrence and behavior of natural and artificial radionuclides in the environment; nuclear fuel cycle; radiochemical analysis methods and devices; production and isolation of radionuclides, synthesis of labeled compounds, new applications of radioactive tracers; radiochemical aspects of nuclear medicine; radiation chemistry and after-effects of nuclear transformations.