日本重点污染控制城市八户的 PM2.5 特征

IF 3.9 3区 环境科学与生态学 Q2 ENVIRONMENTAL SCIENCES Atmospheric Pollution Research Pub Date : 2024-06-03 DOI:10.1016/j.apr.2024.102204
Meng Sun, Xi Zhang
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引用次数: 0

摘要

2015 年 5 月至 2021 年 2 月期间,在日本八户市城区进行了 PM2.5 采样。在整个采样期间,PM2.5 的平均浓度约为 11.7 μg m-3,其中水溶性离子浓度为 4.4 μg m-3,碳物质浓度为 3.3 μg m-3,痕量金属浓度为 0.5 μg m-3,其他物质浓度为 3.5 μg m-3。根据这些全面的成分信息,对八个来源进行了定量探索,其中船舶排放(29%)、交通排放(19%)和二次有机气溶胶(15%)对 PM2.5 浓度水平的贡献相对较高。健康风险评估结果表明,八户市的儿童面临严重的非致癌和致癌风险,HI 和 CR 的相应值分别为 8.0 和 1.2 × 10-4。船舶排放的污染物、二次硝酸盐加燃煤以及工业排放物应引起关注。高风险金属包括铅、砷、锑、钒和六价铬。具体而言,夏季船舶排放物的浓度(5.5 μg m-3)和健康风险(HI = 2.2 和 CR = 3.0 × 10-5)最高;应优先控制八户港的污染。另外两个污染源在冬季的浓度最高(2.0 和 0.5 μg m-3),主要受秋田县污染气团的影响,HI 值分别为 2.4 和 2.5,CR 值分别为 4.9 × 10-5 和 3.2 × 10-5。总之,我们的研究全面揭示了八户市 PM2.5 的特征,并对其污染原因进行了深入调查。这些信息可为制定改善空气质量的具体策略提供科学依据。
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Characteristics of PM2.5 in Hachinohe, the priority pollution control city in Japan

In the urban area of Hachinohe, Japan, PM2.5 sampling was carried out from May 2015 to February 2021. The average concentration of PM2.5 during the entire sampling period was approximately 11.7 μg m−3, with 4.4 μg m−3 for water soluble ions, 3.3 μg m−3 for carbonaceous species, 0.5 μg m−3 for trace metals, and 3.5 μg m−3 for other species. Based on this comprehensive component information, eight sources were quantitatively explored, among which ship emissions (29%), traffic emissions (19%), and secondary organic aerosols (15%) had relatively high contributions for PM2.5 concentration level. The health risk assessment indicated that the children in Hachinohe City faced serious non-carcinogenic and carcinogenic risks, with corresponding values of 8.0 for HI and 1.2 × 10−4 for CR. The pollutants from ship emissions, secondary nitrates plus coal combustion, and industrial emissions should be of concern. High risk metals included Pb, As, Sb, V, and Cr(VI). Specifically, ship emissions exhibited the highest concentration (5.5 μg m−3) and health risks (HI = 2.2 and CR = 3.0 × 10−5) in summer; priority should be given to controlling pollution in the Port of Hachinohe. The other two sources had the highest concentration in winter (2.0 and 0.5 μg m−3) and were mainly influenced by the polluted air masses from Akita Prefecture, with HI values of 2.4 and 2.5 and CR values of 4.9 × 10−5 and 3.2 × 10−5, respectively. Overall, our study comprehensively revealed the characteristics of PM2.5 in Hachinohe City and conducted an in-depth investigated into its causes of pollution. This information could serve as a scientific basis for developing specific strategies to improve air quality.

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来源期刊
Atmospheric Pollution Research
Atmospheric Pollution Research ENVIRONMENTAL SCIENCES-
CiteScore
8.30
自引率
6.70%
发文量
256
审稿时长
36 days
期刊介绍: Atmospheric Pollution Research (APR) is an international journal designed for the publication of articles on air pollution. Papers should present novel experimental results, theory and modeling of air pollution on local, regional, or global scales. Areas covered are research on inorganic, organic, and persistent organic air pollutants, air quality monitoring, air quality management, atmospheric dispersion and transport, air-surface (soil, water, and vegetation) exchange of pollutants, dry and wet deposition, indoor air quality, exposure assessment, health effects, satellite measurements, natural emissions, atmospheric chemistry, greenhouse gases, and effects on climate change.
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