Xu Yue, Hao Zhou, Chenguang Tian, Yimian Ma, Yihan Hu, C. Gong, Hui Zheng, Hong Liao
{"title":"开发和评估空气污染与土地生态系统互动模型(iMAPLE)1.0 版","authors":"Xu Yue, Hao Zhou, Chenguang Tian, Yimian Ma, Yihan Hu, C. Gong, Hui Zheng, Hong Liao","doi":"10.5194/gmd-17-4621-2024","DOIUrl":null,"url":null,"abstract":"Abstract. Land ecosystems are important sources and sinks of atmospheric components. In turn, air pollutants affect the exchange rates of carbon and water fluxes between ecosystems and the atmosphere. However, these biogeochemical processes are usually not well presented in Earth system models, limiting the explorations of interactions between land ecosystems and air pollutants from regional to global scales. Here, we develop and validate the interactive Model for Air Pollution and Land Ecosystems (iMAPLE) by upgrading the Yale Interactive Terrestrial Biosphere Model with process-based water cycles, fire emissions, wetland methane (CH4) emissions, and trait-based ozone (O3) damage. Within iMAPLE, soil moisture and temperature are dynamically calculated based on the water and energy balance in soil layers. Fire emissions are dependent on dryness, lightning, population, and fuel load. Wetland CH4 is produced but consumed through oxidation, ebullition, diffusion, and plant-mediated transport. The trait-based scheme unifies O3 sensitivity of different plant functional types (PFTs) with the leaf mass per area. Validations show correlation coefficients (R) of 0.59–0.86 for gross primary productivity (GPP) and 0.57–0.84 for evapotranspiration (ET) across the six PFTs at 201 flux tower sites and yield an average R of 0.68 for CH4 emissions at 44 sites. Simulated soil moisture and temperature match reanalysis data with high R above 0.86 and low normalized mean biases (NMBs) within 7 %, leading to reasonable simulations of global GPP (R=0.92, NMB=1.3 %) and ET (R=0.93, NMB=-10.4 %) against satellite-based observations for 2001–2013. The model predicts an annual global area burned of 507.1 Mha, close to the observations of 475.4 Mha with a spatial R of 0.66 for 1997–2016. The wetland CH4 emissions are estimated to be 153.45 Tg [CH4] yr−1 during 2000–2014, close to the multi-model mean of 148 Tg [CH4] yr−1. The model also shows reasonable responses of GPP and ET to the changes in diffuse radiation and yields mean O3 damage of 2.9 % to global GPP. iMAPLE provides an advanced tool for studying the interactions between land ecosystems and air pollutants.\n","PeriodicalId":4,"journal":{"name":"ACS Applied Energy Materials","volume":"11 1","pages":""},"PeriodicalIF":5.5000,"publicationDate":"2024-06-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Development and evaluation of the interactive Model for Air Pollution and Land Ecosystems (iMAPLE) version 1.0\",\"authors\":\"Xu Yue, Hao Zhou, Chenguang Tian, Yimian Ma, Yihan Hu, C. Gong, Hui Zheng, Hong Liao\",\"doi\":\"10.5194/gmd-17-4621-2024\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"Abstract. Land ecosystems are important sources and sinks of atmospheric components. In turn, air pollutants affect the exchange rates of carbon and water fluxes between ecosystems and the atmosphere. However, these biogeochemical processes are usually not well presented in Earth system models, limiting the explorations of interactions between land ecosystems and air pollutants from regional to global scales. Here, we develop and validate the interactive Model for Air Pollution and Land Ecosystems (iMAPLE) by upgrading the Yale Interactive Terrestrial Biosphere Model with process-based water cycles, fire emissions, wetland methane (CH4) emissions, and trait-based ozone (O3) damage. Within iMAPLE, soil moisture and temperature are dynamically calculated based on the water and energy balance in soil layers. Fire emissions are dependent on dryness, lightning, population, and fuel load. Wetland CH4 is produced but consumed through oxidation, ebullition, diffusion, and plant-mediated transport. The trait-based scheme unifies O3 sensitivity of different plant functional types (PFTs) with the leaf mass per area. Validations show correlation coefficients (R) of 0.59–0.86 for gross primary productivity (GPP) and 0.57–0.84 for evapotranspiration (ET) across the six PFTs at 201 flux tower sites and yield an average R of 0.68 for CH4 emissions at 44 sites. Simulated soil moisture and temperature match reanalysis data with high R above 0.86 and low normalized mean biases (NMBs) within 7 %, leading to reasonable simulations of global GPP (R=0.92, NMB=1.3 %) and ET (R=0.93, NMB=-10.4 %) against satellite-based observations for 2001–2013. The model predicts an annual global area burned of 507.1 Mha, close to the observations of 475.4 Mha with a spatial R of 0.66 for 1997–2016. The wetland CH4 emissions are estimated to be 153.45 Tg [CH4] yr−1 during 2000–2014, close to the multi-model mean of 148 Tg [CH4] yr−1. The model also shows reasonable responses of GPP and ET to the changes in diffuse radiation and yields mean O3 damage of 2.9 % to global GPP. iMAPLE provides an advanced tool for studying the interactions between land ecosystems and air pollutants.\\n\",\"PeriodicalId\":4,\"journal\":{\"name\":\"ACS Applied Energy Materials\",\"volume\":\"11 1\",\"pages\":\"\"},\"PeriodicalIF\":5.5000,\"publicationDate\":\"2024-06-12\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"ACS Applied Energy Materials\",\"FirstCategoryId\":\"89\",\"ListUrlMain\":\"https://doi.org/10.5194/gmd-17-4621-2024\",\"RegionNum\":3,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"CHEMISTRY, PHYSICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"ACS Applied Energy Materials","FirstCategoryId":"89","ListUrlMain":"https://doi.org/10.5194/gmd-17-4621-2024","RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
Development and evaluation of the interactive Model for Air Pollution and Land Ecosystems (iMAPLE) version 1.0
Abstract. Land ecosystems are important sources and sinks of atmospheric components. In turn, air pollutants affect the exchange rates of carbon and water fluxes between ecosystems and the atmosphere. However, these biogeochemical processes are usually not well presented in Earth system models, limiting the explorations of interactions between land ecosystems and air pollutants from regional to global scales. Here, we develop and validate the interactive Model for Air Pollution and Land Ecosystems (iMAPLE) by upgrading the Yale Interactive Terrestrial Biosphere Model with process-based water cycles, fire emissions, wetland methane (CH4) emissions, and trait-based ozone (O3) damage. Within iMAPLE, soil moisture and temperature are dynamically calculated based on the water and energy balance in soil layers. Fire emissions are dependent on dryness, lightning, population, and fuel load. Wetland CH4 is produced but consumed through oxidation, ebullition, diffusion, and plant-mediated transport. The trait-based scheme unifies O3 sensitivity of different plant functional types (PFTs) with the leaf mass per area. Validations show correlation coefficients (R) of 0.59–0.86 for gross primary productivity (GPP) and 0.57–0.84 for evapotranspiration (ET) across the six PFTs at 201 flux tower sites and yield an average R of 0.68 for CH4 emissions at 44 sites. Simulated soil moisture and temperature match reanalysis data with high R above 0.86 and low normalized mean biases (NMBs) within 7 %, leading to reasonable simulations of global GPP (R=0.92, NMB=1.3 %) and ET (R=0.93, NMB=-10.4 %) against satellite-based observations for 2001–2013. The model predicts an annual global area burned of 507.1 Mha, close to the observations of 475.4 Mha with a spatial R of 0.66 for 1997–2016. The wetland CH4 emissions are estimated to be 153.45 Tg [CH4] yr−1 during 2000–2014, close to the multi-model mean of 148 Tg [CH4] yr−1. The model also shows reasonable responses of GPP and ET to the changes in diffuse radiation and yields mean O3 damage of 2.9 % to global GPP. iMAPLE provides an advanced tool for studying the interactions between land ecosystems and air pollutants.
期刊介绍:
ACS Applied Energy Materials is an interdisciplinary journal publishing original research covering all aspects of materials, engineering, chemistry, physics and biology relevant to energy conversion and storage. The journal is devoted to reports of new and original experimental and theoretical research of an applied nature that integrate knowledge in the areas of materials, engineering, physics, bioscience, and chemistry into important energy applications.