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Incorporating Oxygen Isotopes of Oxidized Reactive Nitrogen in the Regional Atmospheric Chemistry Mechanism, version 2 (ICOIN-RACM2) 将氧化活性氮的氧同位素纳入区域大气化学机制第 2 版(ICOIN-RACM2)
IF 5.1 3区 地球科学 Q1 Mathematics Pub Date : 2024-06-13 DOI: 10.5194/gmd-17-4673-2024
W. Walters, Masayuki Takeuchi, N. L. Ng, Meredith G. Hastings
Abstract. The oxygen isotope anomaly (Δ17O = δ17O − 0.52 × δ18O > 0) has proven to be a robust tool for probing photochemical cycling and atmospheric formation pathways of oxidized reactive nitrogen (NOy). Several studies have developed modeling techniques to implicitly model Δ17O of NOy molecules based on numerous assumptions that may not always be valid. Thus, these models may be oversimplified and limit our ability to compare model Δ17O values of NOy with observations. In this work, we introduce a novel method for explicitly tracking Δ17O transfer and propagation into NOy and odd oxygen (Ox), integrated into the Regional Atmospheric Chemistry Mechanism, version 2 (RACM2). Termed ICOIN-RACM2 (InCorporating Oxygen Isotopes of NOy in RACM2), this new model includes the addition of 55 new species and 729 replicate reactions to represent the propagation of Δ17O derived from O3 into NOy and Ox. Employing this mechanism within a box model, we simulate Δ17O for various NOy and Ox molecules for chamber experiments with varying initial nitrogen oxides (NOx = NO + NO2) and α-pinene conditions, revealing response shifts in Δ17O linked to distinct oxidant conditions. Furthermore, diel cycles are simulated under two summertime scenarios, representative of an urban and rural site, revealing pronounced Δ17O diurnal patterns for several NOy components and substantial Δ17O differences associated with pollution levels (urban vs. rural). Overall, the proposed mechanism offers the potential to assess NOy oxidation chemistry in chamber studies and air quality campaigns through Δ17O model comparisons against observations. The integration of this mechanism into a 3-D atmospheric chemistry transport model is expected to notably enhance our capacity to model and anticipate Δ17O across landscapes, consequently refining model representations of atmospheric chemistry and tropospheric oxidation capacity.
摘要。氧同位素异常(Δ17O = δ17O - 0.52 × δ18O > 0)已被证明是探测氧化活性氮(NOy)的光化学循环和大气形成途径的有力工具。有几项研究开发了建模技术,根据许多假设隐含地模拟 NOy 分子的 Δ17O,但这些假设不一定总是有效的。因此,这些模型可能过于简化,限制了我们将 NOy 的模型 Δ17O 值与观测值进行比较的能力。在这项工作中,我们介绍了一种新方法,用于明确跟踪Δ17O 向 NOy 和奇数氧(Ox)的转移和传播,并将其集成到区域大气化学机制第 2 版(RACM2)中。这个新模型被称为 ICOIN-RACM2(在 RACM2 中纳入 NOy 的氧同位素),包括增加 55 个新物种和 729 个重复反应,以表示从 O3 派生的 Δ17O 向 NOy 和 Ox 的传播。利用箱式模型中的这一机制,我们在初始氮氧化物(NOx = NO + NO2)和α-蒎烯条件不同的箱式实验中模拟了各种 NOy 和 Ox 分子的 Δ17O,揭示了与不同氧化剂条件相关的 Δ17O的响应变化。此外,还模拟了城市和农村地区两种夏季情景下的昼夜循环,揭示了几种氮氧化物成分的明显Δ17O昼夜模式,以及与污染程度(城市与农村)相关的巨大Δ17O差异。总之,通过将Δ17O 模型与观测结果进行比较,所提出的机制为在室内研究和空气质量活动中评估 NOy 氧化化学性质提供了可能性。将这一机制整合到三维大气化学传输模式中,预计将显著提高我们模拟和预测跨地貌Δ17O 的能力,从而完善大气化学和对流层氧化能力的模式表征。
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引用次数: 0
Dynamic ecosystem assembly and escaping the “fire trap” in the tropics: insights from FATES_15.0.0 热带地区生态系统的动态组合与逃离 "火灾陷阱":从 FATES_15.0.0 获得的启示
IF 5.1 3区 地球科学 Q1 Mathematics Pub Date : 2024-06-13 DOI: 10.5194/gmd-17-4643-2024
J. Shuman, R. Fisher, Charles D. Koven, Ryan Knox, Lara Kueppers, Chonggang Xu
Abstract. Fire is a fundamental part of the Earth system, with impacts on vegetation structure, biomass, and community composition, the latter mediated in part via key fire-tolerance traits, such as bark thickness. Due to anthropogenic climate change and land use pressure, fire regimes are changing across the world, and fire risk has already increased across much of the tropics. Projecting the impacts of these changes at global scales requires that we capture the selective force of fire on vegetation distribution through vegetation functional traits and size structure. We have adapted the fire behavior and effects module, SPITFIRE (SPread and InTensity of FIRE), for use with the Functionally Assembled Terrestrial Ecosystem Simulator (FATES), a size-structured vegetation demographic model. We test how climate, fire regime, and fire-tolerance plant traits interact to determine the biogeography of tropical forests and grasslands. We assign different fire-tolerance strategies based on crown, leaf, and bark characteristics, which are key observed fire-tolerance traits across woody plants. For these simulations, three types of vegetation compete for resources: a fire-vulnerable tree with thin bark, a vulnerable deep crown, and fire-intolerant foliage; a fire-tolerant tree with thick bark, a thin crown, and fire-tolerant foliage; and a fire-promoting C4 grass. We explore the model sensitivity to a critical parameter governing fuel moisture and show that drier fuels promote increased burning, an expansion of area for grass and fire-tolerant trees, and a reduction of area for fire-vulnerable trees. This conversion to lower biomass or grass areas with increased fuel drying results in increased fire-burned area and its effects, which could feed back to local climate variables. Simulated size-based fire mortality for trees less than 20 cm in diameter and those with fire-vulnerable traits is higher than that for larger and/or fire-tolerant trees, in agreement with observations. Fire-disturbed forests demonstrate reasonable productivity and capture observed patterns of aboveground biomass in areas dominated by natural vegetation for the recent historical period but have a large bias in less disturbed areas. Though the model predicts a greater extent of burned fraction than observed in areas with grass dominance, the resulting biogeography of fire-tolerant, thick-bark trees and fire-vulnerable, thin-bark trees corresponds to observations across the tropics. In areas with more than 2500 mm of precipitation, simulated fire frequency and burned area are low, with fire intensities below 150 kW m−1, consistent with observed understory fire behavior across the Amazon. Areas drier than this demonstrate fire intensities consistent with those measured in savannas and grasslands, with high values up to 4000 kW m−1. The results support a positive grass–fire feedback across the region and suggest that forests which have existed without frequent burning may be vulnerable at
摘要火灾是地球系统的一个基本组成部分,对植被结构、生物量和群落组成都有影响,后者部分是通过树皮厚度等关键耐火特征来实现的。由于人为气候变化和土地使用压力,世界各地的火灾机制正在发生变化,热带大部分地区的火灾风险已经增加。要预测这些变化在全球范围内的影响,我们就必须通过植被功能特征和大小结构来捕捉火灾对植被分布的选择性影响。我们对火灾行为和影响模块 SPITFIRE(火灾蔓延和强度)进行了调整,以便与植被大小结构模型功能组装陆地生态系统模拟器(FATES)一起使用。我们测试了气候、火灾机制和耐火植物特性如何相互作用,以决定热带森林和草原的生物地理学。我们根据树冠、树叶和树皮的特征来确定不同的耐火策略,这些特征是在木本植物中观察到的主要耐火特征。在这些模拟中,有三种植被在争夺资源:树皮薄、树冠深、叶片不耐火的易燃树;树皮厚、树冠薄、叶片耐火的耐火树;以及促进火灾的 C4 草。我们探讨了模型对控制燃料湿度的关键参数的敏感性,结果表明,更干燥的燃料会增加燃烧,扩大草和耐火树木的面积,减少易燃树木的面积。随着燃料更加干燥,生物量或草地面积减少,导致火灾燃烧面积及其影响增加,这可能会反馈到当地的气候变量。直径小于 20 厘米的树木和具有易燃特性的树木的模拟火灾死亡率高于较大和/或耐火的树木,这与观测结果一致。受火灾干扰的森林显示出合理的生产力,并捕捉到了近代历史时期以天然植被为主的地区地面生物量的观测模式,但在干扰较少的地区存在较大偏差。虽然模型预测的烧毁部分范围大于草地为主地区的观测结果,但由此产生的耐火厚皮树和易燃薄皮树的生物地理分布与整个热带地区的观测结果一致。在降水量超过 2500 毫米的地区,模拟火灾频率和燃烧面积较低,火灾强度低于 150 kW m-1,与亚马逊地区观测到的林下火灾行为一致。比这更干燥的地区的火灾强度与热带稀树草原和草原的测量值一致,最高可达 4000 kW m-1。这些结果支持了整个地区的草-火正反馈,并表明在没有频繁燃烧的情况下,森林可能会在较高的火灾强度下变得脆弱,这在气候和土地使用压力加剧的情况下更值得关注。FATES 能够捕捉火灾干扰与植物耐火策略之间的联系,从而确定生物地理学,这为评估这些关键碳储存区在整个热带地区不断变化的条件下的脆弱性和恢复力提供了有用的工具。
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引用次数: 0
Multivariate adjustment of drizzle bias using machine learning in European climate projections 在欧洲气候预测中利用机器学习对细雨偏差进行多变量调整
IF 5.1 3区 地球科学 Q1 Mathematics Pub Date : 2024-06-13 DOI: 10.5194/gmd-17-4689-2024
G. Lazoglou, Theo Economou, Christina Anagnostopoulou, G. Zittis, Anna Tzyrkalli, Pantelis Georgiades, J. Lelieveld
Abstract. Precipitation holds significant importance as a climate parameter in various applications, including studies on the impacts of climate change. However, its simulation or projection accuracy is low, primarily due to its high stochasticity. Specifically, climate models often overestimate the frequency of light rainy days while simultaneously underestimating the total amounts of extreme observed precipitation. This phenomenon, known as “drizzle bias”, specifically refers to the model's tendency to overestimate the occurrence of light precipitation events. Consequently, even though the overall precipitation totals are generally well represented, there is often a significant bias in the number of rainy days. The present study aims to minimize the drizzle bias in model output by developing and applying two statistical approaches. In the first approach, the number of rainy days is adjusted based on the assumption that the relationship between observed and simulated rainy days remains the same in time (thresholding). In the second, a machine learning method (random forest or RF) is used for the development of a statistical model that describes the relationship between several climate (modelled) variables and the observed number of wet days. The results demonstrate that employing a multivariate approach yields results that are comparable to the conventional thresholding approach when correcting sub-periods with similar climate characteristics. However, the importance of utilizing RF becomes evident when addressing periods exhibiting extreme events, marked by a significantly distinct frequency of rainy days. These disparities are particularly pronounced when considering higher temporal resolutions. Both methods are illustrated on data from three EURO-CORDEX climate models. The two approaches are trained during a calibration period, and they are applied for the selected evaluation period.
摘要降水量作为一个气候参数,在各种应用中具有重要意义,包括对气候变化影响的研究。然而,降水的模拟或预测精度较低,这主要是由于其高度随机性。具体来说,气候模型经常会高估小雨日的频率,同时低估观测到的极端降水总量。这种现象被称为 "小雨偏差",特指模式倾向于高估小雨降水事件的发生率。因此,尽管总体降水总量一般都得到了很好的体现,但雨天的数量往往存在明显偏差。本研究旨在通过开发和应用两种统计方法,尽量减少模式输出中的小雨偏差。在第一种方法中,根据观测到的降雨日数与模拟的降雨日数之间的关系在时间上保持不变的假设(阈值)来调整降雨日数。第二种方法是使用机器学习方法(随机森林或 RF)建立统计模型,描述多个气候(模拟)变量与观测到的降雨日数之间的关系。结果表明,在校正具有相似气候特征的子时段时,采用多元方法得出的结果与传统的阈值法相当。然而,在处理以明显不同的降雨日频率为标志的极端事件时期时,利用 RF 的重要性就显而易见了。这些差异在考虑更高的时间分辨率时尤为明显。这两种方法都在三个 EURO-CORDEX 气候模型的数据中进行了说明。这两种方法在校准期间进行了训练,并应用于选定的评估期。
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引用次数: 0
Development and evaluation of the interactive Model for Air Pollution and Land Ecosystems (iMAPLE) version 1.0 开发和评估空气污染与土地生态系统互动模型(iMAPLE)1.0 版
IF 5.1 3区 地球科学 Q1 Mathematics Pub Date : 2024-06-12 DOI: 10.5194/gmd-17-4621-2024
Xu Yue, Hao Zhou, Chenguang Tian, Yimian Ma, Yihan Hu, C. Gong, Hui Zheng, Hong Liao
Abstract. Land ecosystems are important sources and sinks of atmospheric components. In turn, air pollutants affect the exchange rates of carbon and water fluxes between ecosystems and the atmosphere. However, these biogeochemical processes are usually not well presented in Earth system models, limiting the explorations of interactions between land ecosystems and air pollutants from regional to global scales. Here, we develop and validate the interactive Model for Air Pollution and Land Ecosystems (iMAPLE) by upgrading the Yale Interactive Terrestrial Biosphere Model with process-based water cycles, fire emissions, wetland methane (CH4) emissions, and trait-based ozone (O3) damage. Within iMAPLE, soil moisture and temperature are dynamically calculated based on the water and energy balance in soil layers. Fire emissions are dependent on dryness, lightning, population, and fuel load. Wetland CH4 is produced but consumed through oxidation, ebullition, diffusion, and plant-mediated transport. The trait-based scheme unifies O3 sensitivity of different plant functional types (PFTs) with the leaf mass per area. Validations show correlation coefficients (R) of 0.59–0.86 for gross primary productivity (GPP) and 0.57–0.84 for evapotranspiration (ET) across the six PFTs at 201 flux tower sites and yield an average R of 0.68 for CH4 emissions at 44 sites. Simulated soil moisture and temperature match reanalysis data with high R above 0.86 and low normalized mean biases (NMBs) within 7 %, leading to reasonable simulations of global GPP (R=0.92, NMB=1.3 %) and ET (R=0.93, NMB=-10.4 %) against satellite-based observations for 2001–2013. The model predicts an annual global area burned of 507.1 Mha, close to the observations of 475.4 Mha with a spatial R of 0.66 for 1997–2016. The wetland CH4 emissions are estimated to be 153.45 Tg [CH4] yr−1 during 2000–2014, close to the multi-model mean of 148 Tg [CH4] yr−1. The model also shows reasonable responses of GPP and ET to the changes in diffuse radiation and yields mean O3 damage of 2.9 % to global GPP. iMAPLE provides an advanced tool for studying the interactions between land ecosystems and air pollutants.
摘要陆地生态系统是大气成分的重要来源和吸收汇。反过来,空气污染物也会影响生态系统与大气之间碳和水通量的交换率。然而,这些生物地球化学过程通常没有在地球系统模型中得到很好的呈现,从而限制了从区域到全球尺度的陆地生态系统与空气污染物之间相互作用的探索。在此,我们开发并验证了空气污染与陆地生态系统互动模型(iMAPLE),将耶鲁互动陆地生物圈模型升级为基于过程的水循环、火灾排放、湿地甲烷(CH4)排放和基于性状的臭氧(O3)破坏。在 iMAPLE 中,土壤水分和温度是根据土壤层中的水分和能量平衡动态计算的。火灾排放取决于干燥度、闪电、人口和燃料负荷。湿地 CH4 通过氧化、沸腾、扩散和植物介导的迁移产生并消耗。基于性状的方案将不同植物功能类型(PFTs)对 O3 的敏感性与单位面积的叶片质量统一起来。验证结果表明,在 201 个通量塔站点的六个植物功能类型中,总初级生产力(GPP)的相关系数(R)为 0.59-0.86,蒸散量(ET)的相关系数(R)为 0.57-0.84,44 个站点的甲烷排放量的平均相关系数(R)为 0.68。模拟的土壤水分和温度与再分析数据相匹配,R 值高达 0.86 以上,归一化平均偏差(NMBs)低至 7%以内,从而根据卫星观测数据对 2001-2013 年全球 GPP(R 值=0.92,NMB=1.3%)和蒸散发(R 值=0.93,NMB=-10.4%)进行了合理模拟。该模型预测全球每年的焚烧面积为 5.071 亿公顷,接近 1997-2016 年的观测值 4.754 亿公顷,空间 R 值为 0.66。据估计,2000-2014 年期间湿地的 CH4 排放量为 153.45 Tg [CH4]/yr-1,接近多模型平均值 148 Tg [CH4]/yr-1。该模型还显示了 GPP 和蒸散发对漫射辐射变化的合理响应,并得出 O3 对全球 GPP 的平均损害为 2.9%。iMAPLE 为研究陆地生态系统与空气污染物之间的相互作用提供了先进的工具。
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引用次数: 0
StraitFlux – precise computations of water strait fluxes on various modeling grids StraitFlux - 在各种建模网格上精确计算海峡通量
IF 5.1 3区 地球科学 Q1 Mathematics Pub Date : 2024-06-12 DOI: 10.5194/gmd-17-4603-2024
S. Winkelbauer, Michael Mayer, L. Haimberger
Abstract. Oceanic transports shape the global climate, but the evaluation and validation of this key quantity based on reanalysis and model data are complicated by the distortion of the used curvilinear ocean model grids towards their displaced north poles. Combined with the large number of different grid types, this has made the exact calculation of oceanic transports a challenging and time-consuming task. Use of data interpolated to standard latitude/longitude grids is not an option, since transports computed from interpolated velocity fields are not mass-consistent. We present two methods for transport calculations on grids with variously shifted north poles, different orientations, and different Arakawa partitions. The first method calculates net transports through arbitrary sections using line integrals, while the second method generates cross sections of the vertical–horizontal planes of these sections using vector projection algorithms. Apart from the input data on the original model grids, the user only needs to specify the start and endpoints of the required section to get the net transports (for the first method) and their cross sections (for the second method). Integration of the cross sections along their depth and horizontal extent yields net transports in very good quantitative agreement with the line integration method. This allows us to calculate oceanic fluxes through almost arbitrary sections to compare them with observed oceanic volume and energy transports at available sections, such as the RAPID array or at Fram Strait and other Arctic gateways, or to compare them amongst reanalyses and to model integrations from the Coupled Model Intercomparison Projects (CMIPs). We implemented our methods in a Python package called StraitFlux. This paper represents its scientific documentation and demonstrates its application on outputs of multiple CMIP6 models and several ocean reanalyses. We also analyze the robustness and computational performance of the tools, as well as the uncertainties in the results. The package is available on GitHub and Zenodo and can be installed using pypi.
摘要。海洋传输量影响着全球气候,但由于使用的曲线海洋模式网格向其偏移的北极变形,基于再分析和模式数据对这一关键量的评估和验证变得复杂。再加上大量不同类型的网格,这使得精确计算海洋传输量成为一项具有挑战性且耗时的任务。使用插值到标准纬度/经度网格的数据是不可行的,因为根据插值速度场计算出的传输量与质量不一致。我们提出了两种在具有不同偏移北极、不同方向和不同荒川分区的网格上进行传输计算的方法。第一种方法使用线积分计算通过任意截面的净传输量,第二种方法使用矢量投影算法生成这些截面的垂直-水平面横截面。除了原始模型网格上的输入数据外,用户只需指定所需断面的起点和终点,即可获得净传输量(第一种方法)及其横截面(第二种方法)。将横截面沿其深度和水平范围进行积分,得到的净输送量与线积分法在数量上非常一致。这样,我们就可以计算几乎任意断面的海洋通量,将其与 RAPID 阵列或弗拉姆海峡和其他北极门户等现有断面观测到的海洋体积和能量传输进行比较,或与再分析和耦合模式相互比较项目(CMIPs)的模式积分进行比较。我们在一个名为 StraitFlux 的 Python 软件包中实现了我们的方法。本文介绍了它的科学文献,并演示了它在多个 CMIP6 模式和多个海洋再分析输出中的应用。我们还分析了工具的鲁棒性和计算性能,以及结果的不确定性。该软件包可在 GitHub 和 Zenodo 上下载,并可使用 pypi 安装。
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引用次数: 0
A general comprehensive evaluation method for cross-scale precipitation forecasts 跨尺度降水预报的一般综合评估方法
IF 5.1 3区 地球科学 Q1 Mathematics Pub Date : 2024-06-10 DOI: 10.5194/gmd-17-4579-2024
Bing Zhang, Mingjian Zeng, Anning Huang, Zhengkun Qin, Couhua Liu, Wenru Shi, Xin Li, Kefeng Zhu, Chun-Lai Gu, Jialing Zhou
Abstract. With the development of refined numerical forecasts, problems such as score distortion due to the division of precipitation thresholds in both traditional and improved scoring methods for precipitation forecasts and the increasing subjective risk arising from the scale setting of the neighborhood spatial verification method have become increasingly prominent. To address these issues, a general comprehensive evaluation method (GCEM) is developed for cross-scale precipitation forecasts by directly analyzing the proximity of precipitation forecasts and observations in this study. In addition to the core indicator of the precipitation accuracy score (PAS), the GCEM system also includes score indices for insufficient precipitation forecasts, excessive precipitation forecasts, precipitation forecast biases, and clear/rainy forecasts. The PAS does not distinguish the magnitude of precipitation and does not delimit the area of influence; it constitutes a fair scoring formula with objective performance and can be suitable for evaluating rainfall events such as general and extreme precipitation. The PAS can be used to calculate the accuracy of numerical models or quantitative precipitation forecasts, enabling the quantitative evaluation of the comprehensive capability of various refined precipitation forecasting products. Based on the GCEM, comparative experiments between the PAS and threat score (TS) are conducted for two typical precipitation weather processes. The results show that relative to the TS, the PAS better aligns with subjective expectations, indicating that the PAS is more reasonable than the TS. In the case of an extreme-precipitation event in Henan, China, two high-resolution models were evaluated using the PAS, TS, and fraction skill score (FSS), verifying the evaluation ability of PAS scoring for predicting extreme-precipitation events. In addition, other indices of the GCEM are utilized to analyze the range and extent of both insufficient and excessive forecasts of precipitation, as well as the precipitation forecasting ability for different weather processes. These indices not only provide overall scores similar to those of the TS for individual cases but also support two-dimensional score distribution plots which can comprehensively reflect the performance and characteristics of precipitation forecasts. Both theoretical and practical applications demonstrate that the GCEM exhibits distinct advantages and potential promotion and application value compared to the various mainstream precipitation forecast verification methods.
摘要随着精细化数值预报的发展,传统的降水预报评分方法和改进的降水预报评分方法中由于降水阈值划分导致的评分失真、邻域空间验证方法的尺度设置导致的主观风险增大等问题日益突出。针对这些问题,本研究通过直接分析降水预报与观测资料的接近程度,建立了跨尺度降水预报的一般综合评价方法(GCEM)。除了降水准确性评分(PAS)这一核心指标外,GCEM 系统还包括降水预报不足、降水预报过多、降水预报偏差和晴雨预报等评分指标。PAS 不区分降水量的大小,也不划定影响范围;它是一个具有客观性能的公平评分公式,适用于评估一般降水和极端降水等降水事件。PAS 可用于计算数值模式或定量降水预报的准确性,从而对各种精细化降水预报产品的综合能力进行定量评估。在 GCEM 的基础上,针对两种典型的降水天气过程进行了 PAS 和威胁评分(TS)的对比实验。结果表明,相对于 TS,PAS 更符合主观预期,表明 PAS 比 TS 更合理。以中国河南的一次极端降水事件为例,利用 PAS、TS 和分数技能得分(FSS)对两个高分辨率模型进行了评估,验证了 PAS 评分对预测极端降水事件的评估能力。此外,还利用 GCEM 的其他指数分析了降水预报不足和过度的范围和程度,以及不同天气过程的降水预报能力。这些指数不仅提供了与 TS 指数类似的单个案例的总体评分,而且支持二维评分分布图,能够全面反映降水预报的性能和特点。理论和实际应用均表明,与各种主流降水预报验证方法相比,GCEM具有明显的优势和潜在的推广应用价值。
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引用次数: 0
EvalHyd v0.1.2: a polyglot tool for the evaluation of deterministic and probabilistic streamflow predictions EvalHyd v0.1.2:用于评估确定性和概率性流量预测的多语言工具
IF 5.1 3区 地球科学 Q1 Mathematics Pub Date : 2024-06-10 DOI: 10.5194/gmd-17-4561-2024
T. Hallouin, F. Bourgin, C. Perrin, Maria-Helena Ramos, V. Andréassian
Abstract. The evaluation of streamflow predictions forms an essential part of most hydrological modelling studies published in the literature. The evaluation process typically involves the computation of some evaluation metrics, but it can also involve the preliminary processing of the predictions as well as the subsequent processing of the computed metrics. In order for published hydrological studies to be reproducible, these steps need to be carefully documented by the authors. The availability of a single tool performing all of these tasks would simplify not only the documentation by the authors but also the reproducibility by the readers. However, this requires such a tool to be polyglot (i.e. usable in a variety of programming languages) and openly accessible so that it can be used by everyone in the hydrological community. To this end, we developed a new tool named evalhyd that offers metrics and functionalities for the evaluation of deterministic and probabilistic streamflow predictions. It is open source, and it can be used in Python, in R, in C++, or as a command line tool. This article describes the tool and illustrates its functionalities using Global Flood Awareness System (GloFAS) reforecasts over France as an example data set.
摘要在文献发表的大多数水文建模研究中,水流预测评估都是必不可少的一部分。评估过程通常包括计算一些评估指标,但也可能涉及预测的初步处理以及计算指标的后续处理。为了使已发表的水文研究报告具有可重复性,作者需要仔细记录这些步骤。如果有一个能完成所有这些任务的工具,不仅能简化作者的记录工作,还能简化读者的重现工作。然而,这就要求这种工具必须是多语言的(即可以使用多种编程语言),并且可以公开访问,以便水文界的每个人都能使用。为此,我们开发了一款名为 evalhyd 的新工具,它提供了用于评估确定性和概率性流量预测的指标和功能。该工具开源,可在 Python、R、C++ 中使用,也可作为命令行工具使用。本文将以全球洪水预警系统(GloFAS)对法国的再预测数据集为例,介绍该工具并说明其功能。
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引用次数: 0
A perspective on the next generation of Earth system model scenarios: towards representative emission pathways (REPs) 透视下一代地球系统模式假设:走向代表性排放路径 (REP)
IF 5.1 3区 地球科学 Q1 Mathematics Pub Date : 2024-06-05 DOI: 10.5194/gmd-17-4533-2024
M. Meinshausen, C. Schleussner, Kathleen Beyer, Greg Bodeker, Olivier Boucher, J. Canadell, John S. Daniel, Aïda Diongue-Niang, Fatima Driouech, Erich Fischer, P. Forster, Michael Grose, Gerrit Hansen, Z. Hausfather, T. Ilyina, J. Kikstra, Joyce Kimutai, A. King, June-Yi Lee, Chris Lennard, T. Lissner, A. Nauels, Glen P. Peters, Anna Pirani, G. Plattner, Hans-Ove Pörtner, J. Rogelj, Maisa Rojas, Joyashree Roy, B. Samset, Benjamin M. Sanderson, R. Séférian, S. Seneviratne, Christopher J. Smith, S. Szopa, Adelle Thomas, D. Urge-Vorsatz, G. Velders, T. Yokohata, T. Ziehn, Zebedee R. J. Nicholls
Abstract. In every Intergovernmental Panel on Climate Change (IPCC) Assessment cycle, a multitude of scenarios are assessed, with different scope and emphasis throughout the various Working Group reports and special reports, as well as their respective chapters. Within the reports, the ambition is to integrate knowledge on possible climate futures across the Working Groups and scientific research domains based on a small set of “framing pathways” such as the so-called representative concentration pathways (RCPs) in the Fifth IPCC Assessment Report (AR5) and the shared socioeconomic pathway (SSP) scenarios in the Sixth Assessment Report (AR6). This perspective, initiated by discussions at the IPCC Bangkok workshop in April 2023 on the “Use of Scenarios in AR6 and Subsequent Assessments”, is intended to serve as one of the community contributions to highlight the needs for the next generation of framing pathways that is being advanced under the Coupled Model Intercomparison Project (CMIP) umbrella, which will influence or even predicate the IPCC AR7 consideration of framing pathways. Here we suggest several policy research objectives that such a set of framing pathways should ideally fulfil, including mitigation needs for meeting the Paris Agreement objectives, the risks associated with carbon removal strategies, the consequences of delay in enacting that mitigation, guidance for adaptation needs, loss and damage, and for achieving mitigation in the wider context of societal development goals. Based on this context, we suggest that the next generation of climate scenarios for Earth system models should evolve towards representative emission pathways (REPs) and suggest key categories for such pathways. These framing pathways should address the most critical mitigation policy and adaptation plans that need to be implemented over the next 10 years. In our view, the most important categories are those relevant in the context of the Paris Agreement long-term goal, specifically an immediate action (low overshoot) 1.5 °C pathway and a delayed action (high overshoot) 1.5 °C pathway. Two other key categories are a pathway category approximately in line with current (as expressed by 2023) near- and long-term policy objectives, as well as a higher-emission category that is approximately in line with “current policies” (as expressed by 2023). We also argue for the scientific and policy relevance in exploring two “worlds that could have been”. One of these categories has high-emission trajectories well above what is implied by current policies and the other has very-low-emission trajectories which assume that global mitigation action in line with limiting warming to 1.5 °C without overshoot had begun in 2015. Finally, we note that the timely provision of new scientific information on pathways is critical to inform the development and implementation of climate policy. Under the Paris Agreement, for the second global stocktake, which will occur in 2028, and to in
摘要。在政府间气候变化专门委员会(IPCC)的每个评估周期中,都会对多种情景进行评估,各工作组报告和特别报告及其各自章节的范围和重点各不相同。在这些报告中,我们的目标是在一小套 "框架路径 "的基础上,整合各工作组和科研领域对可能的气候未来的认识,如第五次政府间气候变化专门委员会评估报告(AR5)中的所谓代表性浓度路径(RCPs)和第六次评估报告(AR6)中的共享社会经济路径(SSP)情景。本视角由 2023 年 4 月 IPCC 曼谷研讨会上关于 "在 AR6 及后续评估中使用情景 "的讨论发起,旨在作为社区贡献之一,强调在耦合模式相互比较项目(CMIP)框架下正在推进的下一代框架路径的需求,这将影响甚至预示 IPCC AR7 对框架路径的考虑。在此,我们提出了一系列政策研究目标,理想情况下,这套框架路径应满足这些目标,包括实现《巴黎协定》目标的减排需求、与碳清除战略相关的风险、延迟实施减排的后果、对适应需求、损失和损害的指导,以及在更广泛的社会发展目标背景下实现减排。基于这一背景,我们建议地球系统模式的下一代气候情景应朝着代表性排放路径(REP)方向发展,并提出了此类路径的关键类别。这些路径框架应涉及未来 10 年需要实施的最关键的减缓政策和适应计划。我们认为,最重要的类别是与《巴黎协定》长期目标相关的类别,特别是立即行动(低过冲)1.5 °C路径和延迟行动(高过冲)1.5 °C路径。另外两个关键类别是大致符合当前(截至 2023 年)近期和长期政策目标的路径类别,以及大致符合 "当前政策"(截至 2023 年)的高排放类别。我们还论证了探索两个 "可能的世界 "的科学和政策相关性。其中一个类别的高排放轨迹远高于当前政策所暗示的水平,而另一个类别的极低排放轨迹则假定全球减缓行动从 2015 年开始,将升温控制在 1.5 °C,且不出现超调。最后,我们注意到,及时提供有关路径的新科学信息对于制定和实施气候政策至关重要。根据《巴黎协定》,为了在 2028 年进行第二次全球评估,并为随后制定直至 2040 年的国家确定的贡献(NDCs)提供信息,需要在 2027 年之前提供科学投入。在制定社区建模活动(包括 CMIP7 下的建模活动)的时间表时,应认真考虑这些需求。
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引用次数: 3
Development of a multiphase chemical mechanism to improve secondary organic aerosol formation in CAABA/MECCA (version 4.7.0) 开发多相化学机制,改善 CAABA/MECCA 中二次有机气溶胶的形成(4.7.0 版)
IF 5.1 3区 地球科学 Q1 Mathematics Pub Date : 2024-05-24 DOI: 10.5194/gmd-17-4311-2024
Felix Wieser, Rolf Sander, C. Cho, H. Fuchs, Torsten Hohaus, A. Novelli, R. Tillmann, D. Taraborrelli
Abstract. During the last few decades, the impact of multiphase chemistry on secondary organic aerosols (SOAs) has been demonstrated to be the key to explaining laboratory experiments and field measurements. However, global atmospheric models still show large biases when simulating atmospheric observations of organic aerosols (OAs). Major reasons for the model errors are the use of simplified chemistry schemes of the gas-phase oxidation of vapours and the parameterization of heterogeneous surface reactions. The photochemical oxidation of anthropogenic and biogenic volatile organic compounds (VOCs) leads to products that either produce new SOA or are taken up by existing aqueous media like cloud droplets and deliquescent aerosols. After partitioning, aqueous-phase processing results in polyols, organosulfates, and other products with a high molar mass and oxygen content. In this work, we introduce the formation of new low-volatility organic compounds (LVOCs) to the multiphase chemistry box model CAABA/MECCA. Most notable are the additions of the SOA precursors, limonene and n-alkanes (5 to 8 C atoms), and a semi-explicit chemical mechanism for the formation of LVOCs from isoprene oxidation in the gas and aqueous phases. Moreover, Henry's law solubility constants and their temperature dependences are estimated for the partitioning of organic molecules to the aqueous phase. Box model simulations indicate that the new chemical scheme predicts the enhanced formation of LVOCs, which are known for being precursor species to SOAs. As expected, the model predicts that LVOCs are positively correlated to temperature but negatively correlated to NOx levels. However, the aqueous-phase processing of isoprene epoxydiols (IEPOX) displays a more complex dependence on these two key variables. Semi-quantitative comparison with observations from the SOAS campaign suggests that the model may overestimate methylbutane-1,2,3,4-tetrol (MeBuTETROL) from IEPOX. Further application of the mechanism in the modelling of two chamber experiments, one in which limonene is consumed by ozone and one in which isoprene is consumed by NO3 shows a sufficient agreement with experimental results within model limitations. The extensions in CAABA/MECCA are transferred to the 3D atmospheric model MESSy for a comprehensive evaluation of the impact of aqueous- and/or aerosol-phase chemistry on SOA at a global scale in a follow-up study.
摘要在过去几十年中,多相化学对二次有机气溶胶(SOAs)的影响已被证明是解释实验室实验和实地测量的关键。然而,全球大气模型在模拟大气中的有机气溶胶(OAs)观测结果时仍存在较大偏差。造成模型误差的主要原因是使用了简化的气相蒸汽氧化化学方案和异质表面反应参数化。人为和生物挥发性有机化合物(VOC)的光化学氧化作用会产生新的 SOA,或被现有的水介质(如云滴和潮解气溶胶)吸收。经过分区后,水相处理会产生多元醇、有机硫酸盐和其他具有高摩尔质量和氧含量的产物。在这项工作中,我们在多相化学盒模型 CAABA/MECCA 中引入了新的低挥发性有机化合物 (LVOC) 的形成。最值得注意的是加入了 SOA 前体--柠檬烯和正构烷烃(5 至 8 个 C 原子),以及异戊二烯在气相和水相氧化形成低挥发性有机化合物的半明了化学机制。此外,还估算了有机分子在水相中的亨利定律溶解常数及其温度相关性。方框模型模拟表明,新的化学方案预测 LVOCs 的形成会增强,众所周知,LVOCs 是 SOAs 的前体物种。正如预期的那样,模型预测 LVOC 与温度呈正相关,但与氮氧化物水平呈负相关。不过,异戊二烯环氧二醇(IEPOX)的水相处理与这两个关键变量的关系更为复杂。与 SOAS 活动的观测结果进行半定量比较后发现,该模型可能会高估 IEPOX 产生的甲基丁烷-1,2,3,4-四醇(MeBuTETROL)。将该机制进一步应用于两个室实验的建模中,一个是臭氧消耗柠檬烯的实验,另一个是 NO3 消耗异戊二烯的实验,结果表明在模型限制范围内与实验结果充分吻合。CAABA/MECCA 中的扩展功能被转移到三维大气模型 MESSy 中,以便在后续研究中全面评估全球范围内水相和/或气溶胶相化学对 SOA 的影响。
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引用次数: 0
Simple process-led algorithms for simulating habitats (SPLASH v.2.0): robust calculations of water and energy fluxes 模拟生境的简单过程主导算法(SPLASH v.2.0):水和能量通量的稳健计算
IF 5.1 3区 地球科学 Q1 Mathematics Pub Date : 2024-05-24 DOI: 10.5194/gmd-17-4229-2024
David Sandoval, I. Prentice, Rodolfo L. B. Nóbrega
Abstract. The current representation of key processes in land surface models (LSMs) for estimating water and energy balances still relies heavily on empirical equations that require calibration oriented to site-specific characteristics. When multiple parameters are used, different combinations of parameter values can produce equally acceptable results, leading to a risk of obtaining “the right answers for the wrong reasons”, compromising the reproducibility of the simulations and limiting the ecological interpretability of the results. To address this problem and reduce the need for free parameters, here we present novel formulations based on first principles to calculate key components of water and energy balances, extending the already parsimonious SPLASH model v.1.0 (Davis et al., 2017, GMD). We found analytical solutions for many processes, enabling us to increase spatial resolution and include the terrain effects directly in the calculations without unreasonably inflating computational demands. This calibration-free model estimates quantities such as net radiation, evapotranspiration, condensation, soil water content, surface runoff, subsurface lateral flow, and snow-water equivalent. These quantities are derived from readily available meteorological data such as near-surface air temperature, precipitation, and solar radiation, as well as soil physical properties. Whenever empirical formulations were required, e.g., pedotransfer functions and albedo–snow cover relationships, we selected and optimized the best-performing equations through a combination of remote sensing and globally distributed terrestrial observational datasets. Simulations at global scales at different resolutions were run to evaluate spatial patterns, while simulations with point-based observations were run to evaluate seasonal patterns using data from hundreds of stations and comparisons with the VIC-3L model, demonstrating improved performance based on statistical tests and observational comparisons. In summary, our model offers a more robust, reproducible, and ecologically interpretable solution compared to more complex LSMs.
摘要。目前,用于估算水量和能量平衡的地表模型(LSMs)对关键过程的表述仍主要依赖于经验方程,这些方程需要根据具体地点的特征进行校准。当使用多个参数时,不同的参数值组合可产生同样可接受的结果,从而导致 "因错误原因而获得正确答案 "的风险,影响模拟的可重复性,并限制了结果的生态可解释性。为了解决这个问题并减少对自由参数的需求,我们在此提出了基于第一性原理的新公式,以计算水和能量平衡的关键组成部分,并扩展了已经很简洁的 SPLASH 模型 v.1.0(Davis 等人,2017 年,GMD)。我们找到了许多过程的解析解,使我们能够提高空间分辨率,并将地形效应直接纳入计算,而不会不合理地增加计算需求。该免校准模型可估算净辐射、蒸散、凝结、土壤含水量、地表径流、地下侧向流和雪水当量等量。这些数据都是通过近地面气温、降水和太阳辐射等现成的气象数据以及土壤物理特性得出的。每当需要使用经验公式时,例如,在计算雪泥转移函数和反照率-雪盖关系时,我们都会结合遥感和全球分布的陆地观测数据集,选择并优化性能最佳的方程。我们运行了不同分辨率的全球尺度模拟,以评估空间模式;同时利用数百个站点的数据和 VIC-3L 模型的比较结果,运行了基于点观测的模拟,以评估季节模式。总之,与更复杂的 LSM 相比,我们的模型提供了一个更稳健、可重现和可从生态学角度解释的解决方案。
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引用次数: 0
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