{"title":"利用石墨烯与核/壳量子点混合异质结构的空气稳定型和紫外-近红外宽带光电探测器","authors":"","doi":"10.1016/j.optlastec.2024.111768","DOIUrl":null,"url":null,"abstract":"<div><p>Photodetectors based on PbSe quantum dots (QDs) are commonly used for light detection in the near-infrared (NIR) region. Nevertheless, the performance of photodetectors based on PbSe QDs is constrained by ineffective carrier transfer and poor photo and thermal stabilities. Herein, a promising strategy that harnesses PbSe/PbS core/shell QDs structures is developed and demonstrated to enhance the long-term stability of photodetectors, further combining with graphene to form hybrid heterojunctions that effectively promote carrier transfer. As a result, the devices exhibit a broad photoresponse to the incident light at range of 365–1250 nm, and also possess a high photosensitivity of 1.5 × 10<sup>4</sup> A/W and a high detectivity of 4.0 × 10<sup>13</sup> Jones. Moreover, the lifetime of graphene-PbSe/PbS core/shell QDs hybrid photodetector was 9 times greater than that of uncoated QDs devices. The enormous boost might be attributed to the passivation and protection provided by the core–shell structure, and graphene’s efficient extraction of charge carriers.</p></div>","PeriodicalId":19511,"journal":{"name":"Optics and Laser Technology","volume":null,"pages":null},"PeriodicalIF":4.6000,"publicationDate":"2024-09-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Air-stable and UV-NIR broadband photodetectors utilizing graphene and core/shell quantum dots hybrid heterostructure\",\"authors\":\"\",\"doi\":\"10.1016/j.optlastec.2024.111768\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><p>Photodetectors based on PbSe quantum dots (QDs) are commonly used for light detection in the near-infrared (NIR) region. Nevertheless, the performance of photodetectors based on PbSe QDs is constrained by ineffective carrier transfer and poor photo and thermal stabilities. Herein, a promising strategy that harnesses PbSe/PbS core/shell QDs structures is developed and demonstrated to enhance the long-term stability of photodetectors, further combining with graphene to form hybrid heterojunctions that effectively promote carrier transfer. As a result, the devices exhibit a broad photoresponse to the incident light at range of 365–1250 nm, and also possess a high photosensitivity of 1.5 × 10<sup>4</sup> A/W and a high detectivity of 4.0 × 10<sup>13</sup> Jones. Moreover, the lifetime of graphene-PbSe/PbS core/shell QDs hybrid photodetector was 9 times greater than that of uncoated QDs devices. The enormous boost might be attributed to the passivation and protection provided by the core–shell structure, and graphene’s efficient extraction of charge carriers.</p></div>\",\"PeriodicalId\":19511,\"journal\":{\"name\":\"Optics and Laser Technology\",\"volume\":null,\"pages\":null},\"PeriodicalIF\":4.6000,\"publicationDate\":\"2024-09-12\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Optics and Laser Technology\",\"FirstCategoryId\":\"101\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S003039922401226X\",\"RegionNum\":2,\"RegionCategory\":\"物理与天体物理\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"OPTICS\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Optics and Laser Technology","FirstCategoryId":"101","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S003039922401226X","RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"OPTICS","Score":null,"Total":0}
Air-stable and UV-NIR broadband photodetectors utilizing graphene and core/shell quantum dots hybrid heterostructure
Photodetectors based on PbSe quantum dots (QDs) are commonly used for light detection in the near-infrared (NIR) region. Nevertheless, the performance of photodetectors based on PbSe QDs is constrained by ineffective carrier transfer and poor photo and thermal stabilities. Herein, a promising strategy that harnesses PbSe/PbS core/shell QDs structures is developed and demonstrated to enhance the long-term stability of photodetectors, further combining with graphene to form hybrid heterojunctions that effectively promote carrier transfer. As a result, the devices exhibit a broad photoresponse to the incident light at range of 365–1250 nm, and also possess a high photosensitivity of 1.5 × 104 A/W and a high detectivity of 4.0 × 1013 Jones. Moreover, the lifetime of graphene-PbSe/PbS core/shell QDs hybrid photodetector was 9 times greater than that of uncoated QDs devices. The enormous boost might be attributed to the passivation and protection provided by the core–shell structure, and graphene’s efficient extraction of charge carriers.
期刊介绍:
Optics & Laser Technology aims to provide a vehicle for the publication of a broad range of high quality research and review papers in those fields of scientific and engineering research appertaining to the development and application of the technology of optics and lasers. Papers describing original work in these areas are submitted to rigorous refereeing prior to acceptance for publication.
The scope of Optics & Laser Technology encompasses, but is not restricted to, the following areas:
•development in all types of lasers
•developments in optoelectronic devices and photonics
•developments in new photonics and optical concepts
•developments in conventional optics, optical instruments and components
•techniques of optical metrology, including interferometry and optical fibre sensors
•LIDAR and other non-contact optical measurement techniques, including optical methods in heat and fluid flow
•applications of lasers to materials processing, optical NDT display (including holography) and optical communication
•research and development in the field of laser safety including studies of hazards resulting from the applications of lasers (laser safety, hazards of laser fume)
•developments in optical computing and optical information processing
•developments in new optical materials
•developments in new optical characterization methods and techniques
•developments in quantum optics
•developments in light assisted micro and nanofabrication methods and techniques
•developments in nanophotonics and biophotonics
•developments in imaging processing and systems