{"title":"研究无直流偏压电介质的镓铌共掺杂钛酸锶钡陶瓷","authors":"Piyush Sapkota, Keito Yagasaki, Ichiro Fujii, Shintaro Ueno, Satoshi Wada","doi":"10.35848/1347-4065/ad690c","DOIUrl":null,"url":null,"abstract":"The Ba<sub>0.8</sub>Sr<sub>0.2</sub>Ti<sub>1−2<italic toggle=\"yes\">x</italic>\n</sub>Ga<sub>\n<italic toggle=\"yes\">x</italic>\n</sub>Nb<sub>\n<italic toggle=\"yes\">x</italic>\n</sub>O<sub>3</sub> (0 ≤ <italic toggle=\"yes\">x</italic> ≤ 0.10) ceramics were fabricated and the electrical properties were evaluated regarding DC-bias and temperature characteristics of the dielectric properties. The ceramics with <italic toggle=\"yes\">x</italic> = 0.10 exhibited a stable dielectric constant with a change of–40% within 25 °C–150 °C. The dielectric loss of all the co-doped ceramics was below 2% within 25 °C–200 °C. The Ba<sub>0.8</sub>Sr<sub>0.2</sub>Ti<sub>1−2<italic toggle=\"yes\">x</italic>\n</sub>Ga<sub>\n<italic toggle=\"yes\">x</italic>\n</sub>Nb<sub>\n<italic toggle=\"yes\">x</italic>\n</sub>O<sub>3</sub> ceramics showed a higher dielectric constant with a lower DC-bias dependence as compared to previous study on co-doped BaTiO<sub>3</sub> ceramics. The Ba<sub>0.8</sub>Sr<sub>0.2</sub>Ti<sub>0.20</sub>Ga<sub>0.10</sub>Nb<sub>0.10</sub>O<sub>3</sub> ceramics exhibited the best results of DC-bias dependence ≈−24%, dielectric constant at 100 kV cm<sup>−1</sup> ≈ 560, and the dielectric constant at 0 kV cm<sup>−1</sup> ≈ 735. The better results for the Ga–Nb co-doped BST ceramics might be due to the higher contribution of the ionic polarization in the BST base matrix resulting in a shallower potential energy curve.","PeriodicalId":14741,"journal":{"name":"Japanese Journal of Applied Physics","volume":"37 1","pages":""},"PeriodicalIF":1.5000,"publicationDate":"2024-08-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Investigation of Ga–Nb co-doped barium strontium titanate ceramics for DC-bias free dielectrics\",\"authors\":\"Piyush Sapkota, Keito Yagasaki, Ichiro Fujii, Shintaro Ueno, Satoshi Wada\",\"doi\":\"10.35848/1347-4065/ad690c\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"The Ba<sub>0.8</sub>Sr<sub>0.2</sub>Ti<sub>1−2<italic toggle=\\\"yes\\\">x</italic>\\n</sub>Ga<sub>\\n<italic toggle=\\\"yes\\\">x</italic>\\n</sub>Nb<sub>\\n<italic toggle=\\\"yes\\\">x</italic>\\n</sub>O<sub>3</sub> (0 ≤ <italic toggle=\\\"yes\\\">x</italic> ≤ 0.10) ceramics were fabricated and the electrical properties were evaluated regarding DC-bias and temperature characteristics of the dielectric properties. The ceramics with <italic toggle=\\\"yes\\\">x</italic> = 0.10 exhibited a stable dielectric constant with a change of–40% within 25 °C–150 °C. The dielectric loss of all the co-doped ceramics was below 2% within 25 °C–200 °C. The Ba<sub>0.8</sub>Sr<sub>0.2</sub>Ti<sub>1−2<italic toggle=\\\"yes\\\">x</italic>\\n</sub>Ga<sub>\\n<italic toggle=\\\"yes\\\">x</italic>\\n</sub>Nb<sub>\\n<italic toggle=\\\"yes\\\">x</italic>\\n</sub>O<sub>3</sub> ceramics showed a higher dielectric constant with a lower DC-bias dependence as compared to previous study on co-doped BaTiO<sub>3</sub> ceramics. The Ba<sub>0.8</sub>Sr<sub>0.2</sub>Ti<sub>0.20</sub>Ga<sub>0.10</sub>Nb<sub>0.10</sub>O<sub>3</sub> ceramics exhibited the best results of DC-bias dependence ≈−24%, dielectric constant at 100 kV cm<sup>−1</sup> ≈ 560, and the dielectric constant at 0 kV cm<sup>−1</sup> ≈ 735. The better results for the Ga–Nb co-doped BST ceramics might be due to the higher contribution of the ionic polarization in the BST base matrix resulting in a shallower potential energy curve.\",\"PeriodicalId\":14741,\"journal\":{\"name\":\"Japanese Journal of Applied Physics\",\"volume\":\"37 1\",\"pages\":\"\"},\"PeriodicalIF\":1.5000,\"publicationDate\":\"2024-08-21\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Japanese Journal of Applied Physics\",\"FirstCategoryId\":\"101\",\"ListUrlMain\":\"https://doi.org/10.35848/1347-4065/ad690c\",\"RegionNum\":4,\"RegionCategory\":\"物理与天体物理\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q3\",\"JCRName\":\"PHYSICS, APPLIED\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Japanese Journal of Applied Physics","FirstCategoryId":"101","ListUrlMain":"https://doi.org/10.35848/1347-4065/ad690c","RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"PHYSICS, APPLIED","Score":null,"Total":0}
Investigation of Ga–Nb co-doped barium strontium titanate ceramics for DC-bias free dielectrics
The Ba0.8Sr0.2Ti1−2xGaxNbxO3 (0 ≤ x ≤ 0.10) ceramics were fabricated and the electrical properties were evaluated regarding DC-bias and temperature characteristics of the dielectric properties. The ceramics with x = 0.10 exhibited a stable dielectric constant with a change of–40% within 25 °C–150 °C. The dielectric loss of all the co-doped ceramics was below 2% within 25 °C–200 °C. The Ba0.8Sr0.2Ti1−2xGaxNbxO3 ceramics showed a higher dielectric constant with a lower DC-bias dependence as compared to previous study on co-doped BaTiO3 ceramics. The Ba0.8Sr0.2Ti0.20Ga0.10Nb0.10O3 ceramics exhibited the best results of DC-bias dependence ≈−24%, dielectric constant at 100 kV cm−1 ≈ 560, and the dielectric constant at 0 kV cm−1 ≈ 735. The better results for the Ga–Nb co-doped BST ceramics might be due to the higher contribution of the ionic polarization in the BST base matrix resulting in a shallower potential energy curve.
期刊介绍:
The Japanese Journal of Applied Physics (JJAP) is an international journal for the advancement and dissemination of knowledge in all fields of applied physics. JJAP is a sister journal of the Applied Physics Express (APEX) and is published by IOP Publishing Ltd on behalf of the Japan Society of Applied Physics (JSAP).
JJAP publishes articles that significantly contribute to the advancements in the applications of physical principles as well as in the understanding of physics in view of particular applications in mind. Subjects covered by JJAP include the following fields:
• Semiconductors, dielectrics, and organic materials
• Photonics, quantum electronics, optics, and spectroscopy
• Spintronics, superconductivity, and strongly correlated materials
• Device physics including quantum information processing
• Physics-based circuits and systems
• Nanoscale science and technology
• Crystal growth, surfaces, interfaces, thin films, and bulk materials
• Plasmas, applied atomic and molecular physics, and applied nuclear physics
• Device processing, fabrication and measurement technologies, and instrumentation
• Cross-disciplinary areas such as bioelectronics/photonics, biosensing, environmental/energy technologies, and MEMS