中国中部区域气溶胶迁移过程中气溶胶的垂直分布及其与大气边界层结构的关系

IF 7.6 2区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES Environmental Pollution Pub Date : 2024-09-14 DOI:10.1016/j.envpol.2024.124967
Xiaoyun Sun, Yue Zhou, Tianliang Zhao, Weikang Fu, Zhuang Wang, Chune Shi, Hao Zhang, Yuqing Zhang, Qingjian Yang, Zhuozhi Shu
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引用次数: 0

摘要

大气边界层(ABL)结构是改变气溶胶垂直分布和调节区域气溶胶传输对受体区域大气环境影响的关键因素。受体区域很少研究不同垂直气溶胶分布的大气边界层结构的长期特征,以及白天和夜间气溶胶传输与昼夜大气边界层转换相互作用的不同影响机制。基于9年(2013-2021年)卫星获取的气溶胶消光系数剖面和气象探测数据,我们以华中地区输送贡献显著的城市武汉为研究对象,揭示了区域输送过程中一般的冬季输送高度∼500 m和相应的不稳定ABL结构。通过将典型的昼夜气溶胶输送与高分辨率激光雷达观测结果进行对比,发现ABL顶部附近的气溶胶输送与强烈的机械混合为受体区域重气溶胶污染的形成提供了充分的气象条件,而这种气象条件在夜间输送时更为有利,日出后ABL得到充分发展。这些发现加深了我们对 ABL 对受体区域空气污染影响的理解,对区域大气环境的精确防控具有重要意义。
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Vertical distribution of aerosols and association with atmospheric boundary layer structures during regional aerosol transport over central China
Atmospheric boundary layer (ABL) structure was a crucial factor in altering the vertical aerosol distribution and modulating the impact of regional aerosol transport on the atmospheric environment in the receptor region. The long-term characteristics of ABL structures for different vertical aerosol distributions and the distinct influencing mechanisms between daytime and nighttime aerosol transport interacting with the diurnal ABL transition have rarely been studied in the receptor regions. Based on 9-year (2013–2021) satellite-retrieved profiles of aerosol extinction coefficients and meteorological sounding data, we targeted Wuhan, an urban city with noteworthy transport contribution in central China, to reveal the general wintertime transport height of ∼500 m and the corresponding unstable ABL structure during regional transport. By comparing typical daytime and nighttime aerosol transport with high-resolution Lidar observations, the aerosol transport near the ABL top coupled with intense mechanical mixing provided sufficient meteorological conditions for heavy aerosol pollution formation in the receptor regions, which was more favorable during nighttime transport followed by the adequate ABL development after sunrise. These findings enhance our comprehension of the ABL impact on air pollution in the receptor regions, which have implications for the precise prevention and control of the regional atmospheric environment.
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来源期刊
Environmental Pollution
Environmental Pollution 环境科学-环境科学
CiteScore
16.00
自引率
6.70%
发文量
2082
审稿时长
2.9 months
期刊介绍: Environmental Pollution is an international peer-reviewed journal that publishes high-quality research papers and review articles covering all aspects of environmental pollution and its impacts on ecosystems and human health. Subject areas include, but are not limited to: • Sources and occurrences of pollutants that are clearly defined and measured in environmental compartments, food and food-related items, and human bodies; • Interlinks between contaminant exposure and biological, ecological, and human health effects, including those of climate change; • Contaminants of emerging concerns (including but not limited to antibiotic resistant microorganisms or genes, microplastics/nanoplastics, electronic wastes, light, and noise) and/or their biological, ecological, or human health effects; • Laboratory and field studies on the remediation/mitigation of environmental pollution via new techniques and with clear links to biological, ecological, or human health effects; • Modeling of pollution processes, patterns, or trends that is of clear environmental and/or human health interest; • New techniques that measure and examine environmental occurrences, transport, behavior, and effects of pollutants within the environment or the laboratory, provided that they can be clearly used to address problems within regional or global environmental compartments.
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