{"title":"改性微石墨催化的高氯酸盐生物降解及群落变化分析","authors":"","doi":"10.1016/j.jece.2024.114189","DOIUrl":null,"url":null,"abstract":"<div><p>This study investigates the effectiveness of modified micrometer graphite (MMG) in enhancing the biodegradation of perchlorate in sludge. Different MMG types, specifically GO205, GO003, ATGO205, and ATGO003, were evaluated for their impact on perchlorate degradation rates. The results showed a significant acceleration in perchlorate reduction, particularly with the MMG variant GO205, which achieved complete degradation within 48 hours, marking a six-fold increase compared to controls. This rapid degradation also correlated with enhanced microbial activity, as indicated by increased cytochrome C concentrations and electron transport system activity, suggesting a boost in overall microbial metabolic functions. Additionally, shifts in the microbial community composition were observed, with a notable increase in perchlorate-reducing bacteria populations. The study highlights MMG's potential to improve perchlorate remediation processes efficiently and offers promising insights into its application in treating perchlorate-contaminated environments.</p></div>","PeriodicalId":15759,"journal":{"name":"Journal of Environmental Chemical Engineering","volume":null,"pages":null},"PeriodicalIF":7.4000,"publicationDate":"2024-09-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Modified micro-graphite catalysed biodegradation of perchlorate and the analysis of community changes\",\"authors\":\"\",\"doi\":\"10.1016/j.jece.2024.114189\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><p>This study investigates the effectiveness of modified micrometer graphite (MMG) in enhancing the biodegradation of perchlorate in sludge. Different MMG types, specifically GO205, GO003, ATGO205, and ATGO003, were evaluated for their impact on perchlorate degradation rates. The results showed a significant acceleration in perchlorate reduction, particularly with the MMG variant GO205, which achieved complete degradation within 48 hours, marking a six-fold increase compared to controls. This rapid degradation also correlated with enhanced microbial activity, as indicated by increased cytochrome C concentrations and electron transport system activity, suggesting a boost in overall microbial metabolic functions. Additionally, shifts in the microbial community composition were observed, with a notable increase in perchlorate-reducing bacteria populations. The study highlights MMG's potential to improve perchlorate remediation processes efficiently and offers promising insights into its application in treating perchlorate-contaminated environments.</p></div>\",\"PeriodicalId\":15759,\"journal\":{\"name\":\"Journal of Environmental Chemical Engineering\",\"volume\":null,\"pages\":null},\"PeriodicalIF\":7.4000,\"publicationDate\":\"2024-09-18\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Journal of Environmental Chemical Engineering\",\"FirstCategoryId\":\"5\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S2213343724023200\",\"RegionNum\":2,\"RegionCategory\":\"工程技术\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"ENGINEERING, CHEMICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Journal of Environmental Chemical Engineering","FirstCategoryId":"5","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S2213343724023200","RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"ENGINEERING, CHEMICAL","Score":null,"Total":0}
Modified micro-graphite catalysed biodegradation of perchlorate and the analysis of community changes
This study investigates the effectiveness of modified micrometer graphite (MMG) in enhancing the biodegradation of perchlorate in sludge. Different MMG types, specifically GO205, GO003, ATGO205, and ATGO003, were evaluated for their impact on perchlorate degradation rates. The results showed a significant acceleration in perchlorate reduction, particularly with the MMG variant GO205, which achieved complete degradation within 48 hours, marking a six-fold increase compared to controls. This rapid degradation also correlated with enhanced microbial activity, as indicated by increased cytochrome C concentrations and electron transport system activity, suggesting a boost in overall microbial metabolic functions. Additionally, shifts in the microbial community composition were observed, with a notable increase in perchlorate-reducing bacteria populations. The study highlights MMG's potential to improve perchlorate remediation processes efficiently and offers promising insights into its application in treating perchlorate-contaminated environments.
期刊介绍:
The Journal of Environmental Chemical Engineering (JECE) serves as a platform for the dissemination of original and innovative research focusing on the advancement of environmentally-friendly, sustainable technologies. JECE emphasizes the transition towards a carbon-neutral circular economy and a self-sufficient bio-based economy. Topics covered include soil, water, wastewater, and air decontamination; pollution monitoring, prevention, and control; advanced analytics, sensors, impact and risk assessment methodologies in environmental chemical engineering; resource recovery (water, nutrients, materials, energy); industrial ecology; valorization of waste streams; waste management (including e-waste); climate-water-energy-food nexus; novel materials for environmental, chemical, and energy applications; sustainability and environmental safety; water digitalization, water data science, and machine learning; process integration and intensification; recent developments in green chemistry for synthesis, catalysis, and energy; and original research on contaminants of emerging concern, persistent chemicals, and priority substances, including microplastics, nanoplastics, nanomaterials, micropollutants, antimicrobial resistance genes, and emerging pathogens (viruses, bacteria, parasites) of environmental significance.