道路微环境中湍流和弥散变化的综合实地研究

IF 10.8 1区 环境科学与生态学 Q1 ENGINEERING, ENVIRONMENTAL 环境科学与技术 Pub Date : 2024-10-05 DOI:10.1021/acs.est.4c04217
Sheng Xiang, Shaojun Zhang, Peter Brimblecombe, Yu Ting Yu, Kenneth E. Noll, Haobing Liu, Ye Wu, Ke Hao
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引用次数: 0

摘要

汽车尾气排放的与交通有关的空气污染物(TRAPs)会扩散到附近的微环境中,造成潜在的暴露风险。因此,准确识别 TRAPs 的排放热点对于评估潜在的暴露风险至关重要。我们通过综合实地测量研究了湍流动能(TKE)与污染物扩散(D)之间的关系。我们在一条限制轻型车辆通行的道路附近进行了为期五年的近路采样活动(以 5 分钟为基础),并在孤立的试验场进行了路面采样活动(以 5 秒为基础)。首先根据车辆排放和污染物浓度计算 D 值,然后与 TKE 测量值配对。在这里,共收集了 198 对近道路测量数据和 377 对道路测量数据。在近道路测量中,TKE 和 D 与车辆流速呈正相关(R2 ≥ 0.69),而在道路测量中,它们显示出相似的衰减模式和对车辆类型的敏感性。通过这些测量,在 TKE 和 D 之间建立了关系(TKE-D),显示出稳健的相关性(R2 ≥ 0.61)和一致的斜率值(1.1-1.3)。这些发现为 TKE 和 D 之间的正相关关系提供了实地证据,而与测量技术或地点无关。TKE-D 关系使得以 TKE 为唯一输入的车辆排放估算成为可能,有助于识别高时空分辨率的排放热点。
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An Integrated Field Study of Turbulence and Dispersion Variations in Road Microenvironments
Traffic-related air pollutants (TRAPs) emitted from vehicle tailpipes disperse into nearby microenvironments, posing potential exposure risks. Thus, accurately identifying the emission hotspots of TRAPs is essential for assessing potential exposure risks. We investigated the relationship between turbulent kinetic energy (TKE) and pollutant dispersion (D) through an integrated field measurement. A five-year near-road sampling campaign (5 min based) near a light-duty vehicle-restricted roadway and an on-road sampling campaign (5 s based) on isolated proving grounds were conducted. The D was first calculated based on vehicle emission and pollutant concentrations and then paired with TKE measurements. Here, 198 near-road and 377 on-road measurement pairs were collected. In the near-road measurements, TKE and D showed a positive relationship (R2 ≥ 0.69) with the vehicle flow rate, while they showed similar decay patterns and sensitivity to vehicle types in the on-road measurements. A relationship between TKE and D (TKE-D) was developed through these measurements, demonstrating a robust correlation (R2 ≥ 0.61) and consistent slope values (1.1–1.3). These findings provide field evidence for the positive association between TKE and D, irrespective of the measurement techniques or locations. The TKE-D relationship enables vehicle emission estimation with TKE as the sole input, facilitating the identification of emission hotspots with high spatiotemporal resolution.
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来源期刊
环境科学与技术
环境科学与技术 环境科学-工程:环境
CiteScore
17.50
自引率
9.60%
发文量
12359
审稿时长
2.8 months
期刊介绍: Environmental Science & Technology (ES&T) is a co-sponsored academic and technical magazine by the Hubei Provincial Environmental Protection Bureau and the Hubei Provincial Academy of Environmental Sciences. Environmental Science & Technology (ES&T) holds the status of Chinese core journals, scientific papers source journals of China, Chinese Science Citation Database source journals, and Chinese Academic Journal Comprehensive Evaluation Database source journals. This publication focuses on the academic field of environmental protection, featuring articles related to environmental protection and technical advancements.
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