{"title":"室内环境中与形状有关的气溶胶动力学:渗透、沉积和扩散","authors":"Lipeng Lv, Bin Zhao","doi":"10.1016/j.jhazmat.2024.136305","DOIUrl":null,"url":null,"abstract":"Particle shape exerts a significant influence on their dynamic behavior, and it is imperative to elucidate these effects given the potential for severe environmental toxicity associated with shaped particles. Despite extensive research on the dynamical processes of spherical particles, the behaviors of non-spherical particles have been insufficiently investigated. In this study, we have developed a suite of computation-based models that account for particle shape and have reported on the typical dynamical behaviors of non-spherical particles within indoor environments. We have explored three typical scenarios, i.e., particle penetration into indoor spaces through building cracks, indoor particle deposition, and indoor particle dispersion. The shape-induced deviations are associated with dynamical processes, showing a decrease trend among penetration, deposition, and dispersion of the non-spherical particles. The maximum discrepancy due to particle shape during the penetration process exceeds 1000%, observed with particles of approximately 0.02 <span><span style=\"\"></span><span data-mathml='<math xmlns=\"http://www.w3.org/1998/Math/MathML\"><mi is=\"true\">&#x3BC;</mi><mi is=\"true\">m</mi></math>' role=\"presentation\" style=\"font-size: 90%; display: inline-block; position: relative;\" tabindex=\"0\"><svg aria-hidden=\"true\" focusable=\"false\" height=\"1.855ex\" role=\"img\" style=\"vertical-align: -0.697ex;\" viewbox=\"0 -498.8 1482 798.9\" width=\"3.442ex\" xmlns:xlink=\"http://www.w3.org/1999/xlink\"><g fill=\"currentColor\" stroke=\"currentColor\" stroke-width=\"0\" transform=\"matrix(1 0 0 -1 0 0)\"><g is=\"true\"><use xlink:href=\"#MJMATHI-3BC\"></use></g><g is=\"true\" transform=\"translate(603,0)\"><use xlink:href=\"#MJMATHI-6D\"></use></g></g></svg><span role=\"presentation\"><math xmlns=\"http://www.w3.org/1998/Math/MathML\"><mi is=\"true\">μ</mi><mi is=\"true\">m</mi></math></span></span><script type=\"math/mml\"><math><mi is=\"true\">μ</mi><mi is=\"true\">m</mi></math></script></span> in diameter interacting with straight cracks 4.5<!-- --> <!-- -->cm in length and 0.25<!-- --> <!-- -->mm in height. Moreover, there is a discrepancy of more than 70% in the deposition of particles with a diameter of approximately 10 <span><span style=\"\"></span><span data-mathml='<math xmlns=\"http://www.w3.org/1998/Math/MathML\"><mi is=\"true\">&#x3BC;</mi><mi is=\"true\">m</mi></math>' role=\"presentation\" style=\"font-size: 90%; display: inline-block; position: relative;\" tabindex=\"0\"><svg aria-hidden=\"true\" focusable=\"false\" height=\"1.855ex\" role=\"img\" style=\"vertical-align: -0.697ex;\" viewbox=\"0 -498.8 1482 798.9\" width=\"3.442ex\" xmlns:xlink=\"http://www.w3.org/1999/xlink\"><g fill=\"currentColor\" stroke=\"currentColor\" stroke-width=\"0\" transform=\"matrix(1 0 0 -1 0 0)\"><g is=\"true\"><use xlink:href=\"#MJMATHI-3BC\"></use></g><g is=\"true\" transform=\"translate(603,0)\"><use xlink:href=\"#MJMATHI-6D\"></use></g></g></svg><span role=\"presentation\"><math xmlns=\"http://www.w3.org/1998/Math/MathML\"><mi is=\"true\">μ</mi><mi is=\"true\">m</mi></math></span></span><script type=\"math/mml\"><math><mi is=\"true\">μ</mi><mi is=\"true\">m</mi></math></script></span> on side walls when using side air supply ventilation. Similarly, a discrepancy of nearly 11% is noted for particles around 0.02 <span><span style=\"\"></span><span data-mathml='<math xmlns=\"http://www.w3.org/1998/Math/MathML\"><mi is=\"true\">&#x3BC;</mi><mi is=\"true\">m</mi></math>' role=\"presentation\" style=\"font-size: 90%; display: inline-block; position: relative;\" tabindex=\"0\"><svg aria-hidden=\"true\" focusable=\"false\" height=\"1.855ex\" role=\"img\" style=\"vertical-align: -0.697ex;\" viewbox=\"0 -498.8 1482 798.9\" width=\"3.442ex\" xmlns:xlink=\"http://www.w3.org/1999/xlink\"><g fill=\"currentColor\" stroke=\"currentColor\" stroke-width=\"0\" transform=\"matrix(1 0 0 -1 0 0)\"><g is=\"true\"><use xlink:href=\"#MJMATHI-3BC\"></use></g><g is=\"true\" transform=\"translate(603,0)\"><use xlink:href=\"#MJMATHI-6D\"></use></g></g></svg><span role=\"presentation\"><math xmlns=\"http://www.w3.org/1998/Math/MathML\"><mi is=\"true\">μ</mi><mi is=\"true\">m</mi></math></span></span><script type=\"math/mml\"><math><mi is=\"true\">μ</mi><mi is=\"true\">m</mi></math></script></span> in diameter during dispersion under displacement ventilation within indoor settings. The interaction between shape-related particle dynamics, particularly their diffusion characteristics, and the properties of the flow field leads to these shape-dependent dynamical discrepancies. These findings offer a comprehensive understanding of how the shape of particles affects their indoor dynamic behavior, thereby supporting the control of hazardous particles in indoor environments.","PeriodicalId":361,"journal":{"name":"Journal of Hazardous Materials","volume":null,"pages":null},"PeriodicalIF":12.2000,"publicationDate":"2024-10-28","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Shape-Dependent Aerosol Dynamics in Indoor Environments: Penetration, Deposition, and Dispersion\",\"authors\":\"Lipeng Lv, Bin Zhao\",\"doi\":\"10.1016/j.jhazmat.2024.136305\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"Particle shape exerts a significant influence on their dynamic behavior, and it is imperative to elucidate these effects given the potential for severe environmental toxicity associated with shaped particles. Despite extensive research on the dynamical processes of spherical particles, the behaviors of non-spherical particles have been insufficiently investigated. In this study, we have developed a suite of computation-based models that account for particle shape and have reported on the typical dynamical behaviors of non-spherical particles within indoor environments. We have explored three typical scenarios, i.e., particle penetration into indoor spaces through building cracks, indoor particle deposition, and indoor particle dispersion. The shape-induced deviations are associated with dynamical processes, showing a decrease trend among penetration, deposition, and dispersion of the non-spherical particles. The maximum discrepancy due to particle shape during the penetration process exceeds 1000%, observed with particles of approximately 0.02 <span><span style=\\\"\\\"></span><span data-mathml='<math xmlns=\\\"http://www.w3.org/1998/Math/MathML\\\"><mi is=\\\"true\\\">&#x3BC;</mi><mi is=\\\"true\\\">m</mi></math>' role=\\\"presentation\\\" style=\\\"font-size: 90%; display: inline-block; position: relative;\\\" tabindex=\\\"0\\\"><svg aria-hidden=\\\"true\\\" focusable=\\\"false\\\" height=\\\"1.855ex\\\" role=\\\"img\\\" style=\\\"vertical-align: -0.697ex;\\\" viewbox=\\\"0 -498.8 1482 798.9\\\" width=\\\"3.442ex\\\" xmlns:xlink=\\\"http://www.w3.org/1999/xlink\\\"><g fill=\\\"currentColor\\\" stroke=\\\"currentColor\\\" stroke-width=\\\"0\\\" transform=\\\"matrix(1 0 0 -1 0 0)\\\"><g is=\\\"true\\\"><use xlink:href=\\\"#MJMATHI-3BC\\\"></use></g><g is=\\\"true\\\" transform=\\\"translate(603,0)\\\"><use xlink:href=\\\"#MJMATHI-6D\\\"></use></g></g></svg><span role=\\\"presentation\\\"><math xmlns=\\\"http://www.w3.org/1998/Math/MathML\\\"><mi is=\\\"true\\\">μ</mi><mi is=\\\"true\\\">m</mi></math></span></span><script type=\\\"math/mml\\\"><math><mi is=\\\"true\\\">μ</mi><mi is=\\\"true\\\">m</mi></math></script></span> in diameter interacting with straight cracks 4.5<!-- --> <!-- -->cm in length and 0.25<!-- --> <!-- -->mm in height. Moreover, there is a discrepancy of more than 70% in the deposition of particles with a diameter of approximately 10 <span><span style=\\\"\\\"></span><span data-mathml='<math xmlns=\\\"http://www.w3.org/1998/Math/MathML\\\"><mi is=\\\"true\\\">&#x3BC;</mi><mi is=\\\"true\\\">m</mi></math>' role=\\\"presentation\\\" style=\\\"font-size: 90%; display: inline-block; position: relative;\\\" tabindex=\\\"0\\\"><svg aria-hidden=\\\"true\\\" focusable=\\\"false\\\" height=\\\"1.855ex\\\" role=\\\"img\\\" style=\\\"vertical-align: -0.697ex;\\\" viewbox=\\\"0 -498.8 1482 798.9\\\" width=\\\"3.442ex\\\" xmlns:xlink=\\\"http://www.w3.org/1999/xlink\\\"><g fill=\\\"currentColor\\\" stroke=\\\"currentColor\\\" stroke-width=\\\"0\\\" transform=\\\"matrix(1 0 0 -1 0 0)\\\"><g is=\\\"true\\\"><use xlink:href=\\\"#MJMATHI-3BC\\\"></use></g><g is=\\\"true\\\" transform=\\\"translate(603,0)\\\"><use xlink:href=\\\"#MJMATHI-6D\\\"></use></g></g></svg><span role=\\\"presentation\\\"><math xmlns=\\\"http://www.w3.org/1998/Math/MathML\\\"><mi is=\\\"true\\\">μ</mi><mi is=\\\"true\\\">m</mi></math></span></span><script type=\\\"math/mml\\\"><math><mi is=\\\"true\\\">μ</mi><mi is=\\\"true\\\">m</mi></math></script></span> on side walls when using side air supply ventilation. Similarly, a discrepancy of nearly 11% is noted for particles around 0.02 <span><span style=\\\"\\\"></span><span data-mathml='<math xmlns=\\\"http://www.w3.org/1998/Math/MathML\\\"><mi is=\\\"true\\\">&#x3BC;</mi><mi is=\\\"true\\\">m</mi></math>' role=\\\"presentation\\\" style=\\\"font-size: 90%; display: inline-block; position: relative;\\\" tabindex=\\\"0\\\"><svg aria-hidden=\\\"true\\\" focusable=\\\"false\\\" height=\\\"1.855ex\\\" role=\\\"img\\\" style=\\\"vertical-align: -0.697ex;\\\" viewbox=\\\"0 -498.8 1482 798.9\\\" width=\\\"3.442ex\\\" xmlns:xlink=\\\"http://www.w3.org/1999/xlink\\\"><g fill=\\\"currentColor\\\" stroke=\\\"currentColor\\\" stroke-width=\\\"0\\\" transform=\\\"matrix(1 0 0 -1 0 0)\\\"><g is=\\\"true\\\"><use xlink:href=\\\"#MJMATHI-3BC\\\"></use></g><g is=\\\"true\\\" transform=\\\"translate(603,0)\\\"><use xlink:href=\\\"#MJMATHI-6D\\\"></use></g></g></svg><span role=\\\"presentation\\\"><math xmlns=\\\"http://www.w3.org/1998/Math/MathML\\\"><mi is=\\\"true\\\">μ</mi><mi is=\\\"true\\\">m</mi></math></span></span><script type=\\\"math/mml\\\"><math><mi is=\\\"true\\\">μ</mi><mi is=\\\"true\\\">m</mi></math></script></span> in diameter during dispersion under displacement ventilation within indoor settings. The interaction between shape-related particle dynamics, particularly their diffusion characteristics, and the properties of the flow field leads to these shape-dependent dynamical discrepancies. These findings offer a comprehensive understanding of how the shape of particles affects their indoor dynamic behavior, thereby supporting the control of hazardous particles in indoor environments.\",\"PeriodicalId\":361,\"journal\":{\"name\":\"Journal of Hazardous Materials\",\"volume\":null,\"pages\":null},\"PeriodicalIF\":12.2000,\"publicationDate\":\"2024-10-28\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Journal of Hazardous Materials\",\"FirstCategoryId\":\"93\",\"ListUrlMain\":\"https://doi.org/10.1016/j.jhazmat.2024.136305\",\"RegionNum\":1,\"RegionCategory\":\"环境科学与生态学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"ENGINEERING, ENVIRONMENTAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Journal of Hazardous Materials","FirstCategoryId":"93","ListUrlMain":"https://doi.org/10.1016/j.jhazmat.2024.136305","RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"ENGINEERING, ENVIRONMENTAL","Score":null,"Total":0}
Shape-Dependent Aerosol Dynamics in Indoor Environments: Penetration, Deposition, and Dispersion
Particle shape exerts a significant influence on their dynamic behavior, and it is imperative to elucidate these effects given the potential for severe environmental toxicity associated with shaped particles. Despite extensive research on the dynamical processes of spherical particles, the behaviors of non-spherical particles have been insufficiently investigated. In this study, we have developed a suite of computation-based models that account for particle shape and have reported on the typical dynamical behaviors of non-spherical particles within indoor environments. We have explored three typical scenarios, i.e., particle penetration into indoor spaces through building cracks, indoor particle deposition, and indoor particle dispersion. The shape-induced deviations are associated with dynamical processes, showing a decrease trend among penetration, deposition, and dispersion of the non-spherical particles. The maximum discrepancy due to particle shape during the penetration process exceeds 1000%, observed with particles of approximately 0.02 in diameter interacting with straight cracks 4.5 cm in length and 0.25 mm in height. Moreover, there is a discrepancy of more than 70% in the deposition of particles with a diameter of approximately 10 on side walls when using side air supply ventilation. Similarly, a discrepancy of nearly 11% is noted for particles around 0.02 in diameter during dispersion under displacement ventilation within indoor settings. The interaction between shape-related particle dynamics, particularly their diffusion characteristics, and the properties of the flow field leads to these shape-dependent dynamical discrepancies. These findings offer a comprehensive understanding of how the shape of particles affects their indoor dynamic behavior, thereby supporting the control of hazardous particles in indoor environments.
期刊介绍:
The Journal of Hazardous Materials serves as a global platform for promoting cutting-edge research in the field of Environmental Science and Engineering. Our publication features a wide range of articles, including full-length research papers, review articles, and perspectives, with the aim of enhancing our understanding of the dangers and risks associated with various materials concerning public health and the environment. It is important to note that the term "environmental contaminants" refers specifically to substances that pose hazardous effects through contamination, while excluding those that do not have such impacts on the environment or human health. Moreover, we emphasize the distinction between wastes and hazardous materials in order to provide further clarity on the scope of the journal. We have a keen interest in exploring specific compounds and microbial agents that have adverse effects on the environment.