Yuan Yu , Menggang Li , Miao Sun , Zhaolin Yang , Yifan Liu , Senwei Hu , Jiazuo Zhou , Yudong Li , Haiyue Yang , Chengyu Wang
{"title":"骨骼启发的 MXene 纳米气凝胶实现自发电和电容储能","authors":"Yuan Yu , Menggang Li , Miao Sun , Zhaolin Yang , Yifan Liu , Senwei Hu , Jiazuo Zhou , Yudong Li , Haiyue Yang , Chengyu Wang","doi":"10.1016/j.nantod.2024.102538","DOIUrl":null,"url":null,"abstract":"<div><div>The exceptional potential of MXene aerogels for practical applications is impeded by the energy-intensive processing and insufficient mechanical stability. Inspired by natural bones, herein, we report the MXene@regenerated nanocellulose aerogel (MRCA) with strong mechanical performance <em>via</em> dual aerogel fabrication to achieve high-performance energy generation and storage. The MRCA achieves a gravimetric capacitance of 1271.16 F g<sup>−1</sup> at 2 mA cm<sup>−2</sup>, and the energy density of the eco-friendly symmetrical MRCA-based solid-state supercapacitor reaches 0.11 mWh cm<sup>−2</sup>, positioning it as a top contender among most state-of-the-art MXene-based electrodes. Additionally, the MRCA exhibits a robust specific tensile strength of 68.35 MPa cm<sup>3</sup> g<sup>−1</sup>, resembling bone-like resilience. Therefore, MRCA can swiftly generate an open-circuit voltage of 181.24 V. The instant high voltage of MRCA transforms into diverse signals, driving MRCA-SC to release energy for electric devices in practical scenarios, paving the way for future sustainable power systems.</div></div>","PeriodicalId":395,"journal":{"name":"Nano Today","volume":"59 ","pages":"Article 102538"},"PeriodicalIF":13.2000,"publicationDate":"2024-10-28","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Bone-inspired MXene nano aerogels toward self-electricity generation and capacitive energy storage\",\"authors\":\"Yuan Yu , Menggang Li , Miao Sun , Zhaolin Yang , Yifan Liu , Senwei Hu , Jiazuo Zhou , Yudong Li , Haiyue Yang , Chengyu Wang\",\"doi\":\"10.1016/j.nantod.2024.102538\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><div>The exceptional potential of MXene aerogels for practical applications is impeded by the energy-intensive processing and insufficient mechanical stability. Inspired by natural bones, herein, we report the MXene@regenerated nanocellulose aerogel (MRCA) with strong mechanical performance <em>via</em> dual aerogel fabrication to achieve high-performance energy generation and storage. The MRCA achieves a gravimetric capacitance of 1271.16 F g<sup>−1</sup> at 2 mA cm<sup>−2</sup>, and the energy density of the eco-friendly symmetrical MRCA-based solid-state supercapacitor reaches 0.11 mWh cm<sup>−2</sup>, positioning it as a top contender among most state-of-the-art MXene-based electrodes. Additionally, the MRCA exhibits a robust specific tensile strength of 68.35 MPa cm<sup>3</sup> g<sup>−1</sup>, resembling bone-like resilience. Therefore, MRCA can swiftly generate an open-circuit voltage of 181.24 V. The instant high voltage of MRCA transforms into diverse signals, driving MRCA-SC to release energy for electric devices in practical scenarios, paving the way for future sustainable power systems.</div></div>\",\"PeriodicalId\":395,\"journal\":{\"name\":\"Nano Today\",\"volume\":\"59 \",\"pages\":\"Article 102538\"},\"PeriodicalIF\":13.2000,\"publicationDate\":\"2024-10-28\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Nano Today\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S1748013224003943\",\"RegionNum\":1,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"CHEMISTRY, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Nano Today","FirstCategoryId":"88","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S1748013224003943","RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
Bone-inspired MXene nano aerogels toward self-electricity generation and capacitive energy storage
The exceptional potential of MXene aerogels for practical applications is impeded by the energy-intensive processing and insufficient mechanical stability. Inspired by natural bones, herein, we report the MXene@regenerated nanocellulose aerogel (MRCA) with strong mechanical performance via dual aerogel fabrication to achieve high-performance energy generation and storage. The MRCA achieves a gravimetric capacitance of 1271.16 F g−1 at 2 mA cm−2, and the energy density of the eco-friendly symmetrical MRCA-based solid-state supercapacitor reaches 0.11 mWh cm−2, positioning it as a top contender among most state-of-the-art MXene-based electrodes. Additionally, the MRCA exhibits a robust specific tensile strength of 68.35 MPa cm3 g−1, resembling bone-like resilience. Therefore, MRCA can swiftly generate an open-circuit voltage of 181.24 V. The instant high voltage of MRCA transforms into diverse signals, driving MRCA-SC to release energy for electric devices in practical scenarios, paving the way for future sustainable power systems.
期刊介绍:
Nano Today is a journal dedicated to publishing influential and innovative work in the field of nanoscience and technology. It covers a wide range of subject areas including biomaterials, materials chemistry, materials science, chemistry, bioengineering, biochemistry, genetics and molecular biology, engineering, and nanotechnology. The journal considers articles that inform readers about the latest research, breakthroughs, and topical issues in these fields. It provides comprehensive coverage through a mixture of peer-reviewed articles, research news, and information on key developments. Nano Today is abstracted and indexed in Science Citation Index, Ei Compendex, Embase, Scopus, and INSPEC.