Yifeng Chen, Haoran Yin, Shitao Wen, Weiyue Zhang, Shengchun Hu, Kang Sun, Jianchun Jiang, Xiaoyan Ji
{"title":"竹基活性炭在沼气处理中的应用。","authors":"Yifeng Chen, Haoran Yin, Shitao Wen, Weiyue Zhang, Shengchun Hu, Kang Sun, Jianchun Jiang, Xiaoyan Ji","doi":"10.1016/j.biortech.2025.132055","DOIUrl":null,"url":null,"abstract":"<p><p>CO<sub>2</sub>/CH<sub>4</sub> separation is crucial for biogas upgrading. In this study, the bamboo-derived activated carbons (BACs) were prepared with different ratios of potassium hydroxide (KOH)/bamboo charcoal (BC), and the hybrid sorbents of aqueous BACs were developed for CO<sub>2</sub>/CH<sub>4</sub> separation. Both the gas solubility and sorption rate were measured, and Henry's constant and liquid-side mass-transfer coefficient as well as the CO<sub>2</sub>/CH<sub>4</sub> selectivity were calculated. Meanwhile, the comprehensive performances of aqueous BACs were evaluated using a novel index, and the cost of biogas upgrading using the aqueous BACs was estimated and compared to the commercialized technology. The results proved the effectiveness of aqueous BACs, and the comprehensive performance of 7.0 wt% aqueous BAC with the KOH/BC mass ratio of 2:1 was 4.2 times than that of H<sub>2</sub>O, having the potential to decrease the average CO<sub>2</sub>/CH<sub>4</sub> separation cost by 65.0% compared to the commercialized technology.</p>","PeriodicalId":258,"journal":{"name":"Bioresource Technology","volume":" ","pages":"132055"},"PeriodicalIF":9.7000,"publicationDate":"2025-01-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Biogas upgrading using aqueous bamboo-derived activated carbons.\",\"authors\":\"Yifeng Chen, Haoran Yin, Shitao Wen, Weiyue Zhang, Shengchun Hu, Kang Sun, Jianchun Jiang, Xiaoyan Ji\",\"doi\":\"10.1016/j.biortech.2025.132055\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p><p>CO<sub>2</sub>/CH<sub>4</sub> separation is crucial for biogas upgrading. In this study, the bamboo-derived activated carbons (BACs) were prepared with different ratios of potassium hydroxide (KOH)/bamboo charcoal (BC), and the hybrid sorbents of aqueous BACs were developed for CO<sub>2</sub>/CH<sub>4</sub> separation. Both the gas solubility and sorption rate were measured, and Henry's constant and liquid-side mass-transfer coefficient as well as the CO<sub>2</sub>/CH<sub>4</sub> selectivity were calculated. Meanwhile, the comprehensive performances of aqueous BACs were evaluated using a novel index, and the cost of biogas upgrading using the aqueous BACs was estimated and compared to the commercialized technology. The results proved the effectiveness of aqueous BACs, and the comprehensive performance of 7.0 wt% aqueous BAC with the KOH/BC mass ratio of 2:1 was 4.2 times than that of H<sub>2</sub>O, having the potential to decrease the average CO<sub>2</sub>/CH<sub>4</sub> separation cost by 65.0% compared to the commercialized technology.</p>\",\"PeriodicalId\":258,\"journal\":{\"name\":\"Bioresource Technology\",\"volume\":\" \",\"pages\":\"132055\"},\"PeriodicalIF\":9.7000,\"publicationDate\":\"2025-01-10\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Bioresource Technology\",\"FirstCategoryId\":\"5\",\"ListUrlMain\":\"https://doi.org/10.1016/j.biortech.2025.132055\",\"RegionNum\":1,\"RegionCategory\":\"环境科学与生态学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"AGRICULTURAL ENGINEERING\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Bioresource Technology","FirstCategoryId":"5","ListUrlMain":"https://doi.org/10.1016/j.biortech.2025.132055","RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"AGRICULTURAL ENGINEERING","Score":null,"Total":0}
Biogas upgrading using aqueous bamboo-derived activated carbons.
CO2/CH4 separation is crucial for biogas upgrading. In this study, the bamboo-derived activated carbons (BACs) were prepared with different ratios of potassium hydroxide (KOH)/bamboo charcoal (BC), and the hybrid sorbents of aqueous BACs were developed for CO2/CH4 separation. Both the gas solubility and sorption rate were measured, and Henry's constant and liquid-side mass-transfer coefficient as well as the CO2/CH4 selectivity were calculated. Meanwhile, the comprehensive performances of aqueous BACs were evaluated using a novel index, and the cost of biogas upgrading using the aqueous BACs was estimated and compared to the commercialized technology. The results proved the effectiveness of aqueous BACs, and the comprehensive performance of 7.0 wt% aqueous BAC with the KOH/BC mass ratio of 2:1 was 4.2 times than that of H2O, having the potential to decrease the average CO2/CH4 separation cost by 65.0% compared to the commercialized technology.
期刊介绍:
Bioresource Technology publishes original articles, review articles, case studies, and short communications covering the fundamentals, applications, and management of bioresource technology. The journal seeks to advance and disseminate knowledge across various areas related to biomass, biological waste treatment, bioenergy, biotransformations, bioresource systems analysis, and associated conversion or production technologies.
Topics include:
• Biofuels: liquid and gaseous biofuels production, modeling and economics
• Bioprocesses and bioproducts: biocatalysis and fermentations
• Biomass and feedstocks utilization: bioconversion of agro-industrial residues
• Environmental protection: biological waste treatment
• Thermochemical conversion of biomass: combustion, pyrolysis, gasification, catalysis.