近魔角扭曲双层石墨烯的低频电阻噪声

IF 15.8 1区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY ACS Nano Pub Date : 2025-01-16 DOI:10.1021/acsnano.4c11141
Pritam Pal, Saisab Bhowmik, Aparna Parappurath, Saloni Kakkar, Kenji Watanabe, Takashi Taniguchi, Arindam Ghosh
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引用次数: 0

摘要

电阻中的低频电阻波动或噪声不仅为器件设定了性能基准,而且还形成了探测固体中重要电子相和能带结构的敏感工具。在这里,我们报告了扭曲双层石墨烯(tBLG)电阻中这种噪声的测量,其中层在接近幻角(θ ~ 1°)时取向错误。在高温下(T≥60-70 K),低能莫尔波段内波动的功率谱密度(PSD)主要为∝1/f,其中f为频率,在魔角附近通常最低,并且可以用传统的McWhorter模型很好地解释带有陷阱辅助密度迁移率波动的“1/f噪声”。在低T (> 10 K)下,测量噪声表现出强烈的两能级随机电报信号(RTS),特别是在莫尔流隙附近,其PSD值∝为1/f2,这可归因于包封氮化硼(hBN)层中特定缺陷带的费米能量共振筛选不佳。moir带内的低t噪声在积分和半积分填充处表现出一系列极小值,这与在强库仑相互作用驱动的态密度中经常观察到的van Hove奇点一致。除了提供tBLG中噪声的来源和大小的综合说明外,我们的实验还揭示了噪声对tBLG中潜在的相互作用效应比传统的时间平均输运明显更敏感。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

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Low-Frequency Resistance Noise in Near-Magic-Angle Twisted Bilayer Graphene
The low-frequency resistance fluctuations, or noise, in electrical resistance not only set a performance benchmark in devices but also form a sensitive tool to probe nontrivial electronic phases and band structures in solids. Here, we report the measurement of such noise in the electrical resistance in twisted bilayer graphene (tBLG), where the layers are misoriented close to the magic angle (θ ∼ 1°). At high temperatures (T ≳ 60–70 K), the power spectral density (PSD) of the fluctuation inside the low-energy moiré bands is predominantly ∝1/f, where f is the frequency, being generally lowest close to the magic angle, and can be well-explained within the conventional McWhorter model of the ‘1/f noise’ with trap-assisted density-mobility fluctuations. At low T (≲10 K), the measured noise exhibits a strong two-level random telegraphic signal (RTS), especially close to the moiré gap, which exhibits a ∝1/f2-like PSD that can be attributed to poorly screened resonances of the Fermi energy to specific bands of defects in the encapsulating boron nitride (hBN) layers. The low-T noise within the moiré band exhibits a series of minima at the integral as well as half-integral fillings, which align with the frequently observed van Hove singularities in the density-of-states driven by strong Coulomb interaction. Apart from providing a comprehensive account of the origin and the magnitude of noise in tBLG, our experiment also reveals noise to be significantly more sensitive to the underlying interaction effects in tBLG than the conventional time-averaged transport.
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来源期刊
ACS Nano
ACS Nano 工程技术-材料科学:综合
CiteScore
26.00
自引率
4.10%
发文量
1627
审稿时长
1.7 months
期刊介绍: ACS Nano, published monthly, serves as an international forum for comprehensive articles on nanoscience and nanotechnology research at the intersections of chemistry, biology, materials science, physics, and engineering. The journal fosters communication among scientists in these communities, facilitating collaboration, new research opportunities, and advancements through discoveries. ACS Nano covers synthesis, assembly, characterization, theory, and simulation of nanostructures, nanobiotechnology, nanofabrication, methods and tools for nanoscience and nanotechnology, and self- and directed-assembly. Alongside original research articles, it offers thorough reviews, perspectives on cutting-edge research, and discussions envisioning the future of nanoscience and nanotechnology.
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