研磨法制备的AgI/TiO2复合材料增强可见光催化活性

IF 2.4 4区 环境科学与生态学 Q2 WATER RESOURCES Water Quality Research Journal Pub Date : 2019-08-01 DOI:10.2166/WQRJ.2019.037
Jin Xu, Dasheng Gao, Shuang Cui, Xiaohua Wang, Ningning Liu
{"title":"研磨法制备的AgI/TiO2复合材料增强可见光催化活性","authors":"Jin Xu, Dasheng Gao, Shuang Cui, Xiaohua Wang, Ningning Liu","doi":"10.2166/WQRJ.2019.037","DOIUrl":null,"url":null,"abstract":"\n Through a simple grinding method, AgI/TiO2 composites were successfully synthesized. The as-prepared AgI/TiO2 composites were used as photocatalysts for Rhodamine B (RhB) degradation under visible light irradiation and exhibited excellent photocatalytic performance. In the presence of composites, almost 100% RhB was decomposed after 60 min. The photocatalytic activity of AgI/TiO2-0.5 composite was optimal, which was 9.5 times higher than that of pristine TiO2, and 15.6 times higher than that of AgI. Moreover, experimental results revealed that the improved photocatalytic activity was not only ascribed to the loading AgI but also resulted from the method that enabled the exposure of more active sites in the composites. In addition, the intimate interfacial contact obtained by this method could also promote the efficient separation of photogenerated electron-hole pairs. Moreover, the possible photocatalytic active species and the stability of the photocatalyst were investigated in detail.","PeriodicalId":23720,"journal":{"name":"Water Quality Research Journal","volume":null,"pages":null},"PeriodicalIF":2.4000,"publicationDate":"2019-08-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://sci-hub-pdf.com/10.2166/WQRJ.2019.037","citationCount":"1","resultStr":"{\"title\":\"Enhanced visible light photocatalytic activity of AgI/TiO2 composite fabricated by a grinding method\",\"authors\":\"Jin Xu, Dasheng Gao, Shuang Cui, Xiaohua Wang, Ningning Liu\",\"doi\":\"10.2166/WQRJ.2019.037\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"\\n Through a simple grinding method, AgI/TiO2 composites were successfully synthesized. The as-prepared AgI/TiO2 composites were used as photocatalysts for Rhodamine B (RhB) degradation under visible light irradiation and exhibited excellent photocatalytic performance. In the presence of composites, almost 100% RhB was decomposed after 60 min. The photocatalytic activity of AgI/TiO2-0.5 composite was optimal, which was 9.5 times higher than that of pristine TiO2, and 15.6 times higher than that of AgI. Moreover, experimental results revealed that the improved photocatalytic activity was not only ascribed to the loading AgI but also resulted from the method that enabled the exposure of more active sites in the composites. In addition, the intimate interfacial contact obtained by this method could also promote the efficient separation of photogenerated electron-hole pairs. Moreover, the possible photocatalytic active species and the stability of the photocatalyst were investigated in detail.\",\"PeriodicalId\":23720,\"journal\":{\"name\":\"Water Quality Research Journal\",\"volume\":null,\"pages\":null},\"PeriodicalIF\":2.4000,\"publicationDate\":\"2019-08-01\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"https://sci-hub-pdf.com/10.2166/WQRJ.2019.037\",\"citationCount\":\"1\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Water Quality Research Journal\",\"FirstCategoryId\":\"93\",\"ListUrlMain\":\"https://doi.org/10.2166/WQRJ.2019.037\",\"RegionNum\":4,\"RegionCategory\":\"环境科学与生态学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"WATER RESOURCES\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Water Quality Research Journal","FirstCategoryId":"93","ListUrlMain":"https://doi.org/10.2166/WQRJ.2019.037","RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"WATER RESOURCES","Score":null,"Total":0}
引用次数: 1

摘要

通过简单的研磨方法,成功合成了AgI/TiO2复合材料。制备的AgI/TiO2复合材料作为光催化剂,在可见光照射下降解罗丹明B (Rhodamine B, RhB),表现出优异的光催化性能。在复合材料存在的情况下,60 min后RhB几乎100%被分解。AgI/TiO2-0.5复合材料的光催化活性最佳,比原始TiO2高9.5倍,比AgI高15.6倍。此外,实验结果表明,光催化活性的提高不仅归因于负载AgI,还归因于使复合材料中暴露更多活性位点的方法。此外,该方法所获得的亲密界面接触也能促进光生电子-空穴对的有效分离。此外,还对可能的光催化活性物质和光催化剂的稳定性进行了详细的研究。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
查看原文
分享 分享
微信好友 朋友圈 QQ好友 复制链接
本刊更多论文
Enhanced visible light photocatalytic activity of AgI/TiO2 composite fabricated by a grinding method
Through a simple grinding method, AgI/TiO2 composites were successfully synthesized. The as-prepared AgI/TiO2 composites were used as photocatalysts for Rhodamine B (RhB) degradation under visible light irradiation and exhibited excellent photocatalytic performance. In the presence of composites, almost 100% RhB was decomposed after 60 min. The photocatalytic activity of AgI/TiO2-0.5 composite was optimal, which was 9.5 times higher than that of pristine TiO2, and 15.6 times higher than that of AgI. Moreover, experimental results revealed that the improved photocatalytic activity was not only ascribed to the loading AgI but also resulted from the method that enabled the exposure of more active sites in the composites. In addition, the intimate interfacial contact obtained by this method could also promote the efficient separation of photogenerated electron-hole pairs. Moreover, the possible photocatalytic active species and the stability of the photocatalyst were investigated in detail.
求助全文
通过发布文献求助,成功后即可免费获取论文全文。 去求助
来源期刊
CiteScore
4.50
自引率
8.70%
发文量
0
期刊最新文献
Facile fabricated silver Pterocarpus santilinoides biochar-based inorganic–organic hybrid nanocomposite for the photocatalytic decimation of methylene blue and micro-organisms Development of an electrocoagulation method using alternating pulse current to treat wastewater generated by tanneries Effects of different flocculants and environment on the flocculation effect of potato starch-processing wastewater Amyloid fibril–bacterial cellulose nanohybrid membrane cartridge for efficient removal of heavy metal from industrial wastewater Impacts of land use/land cover on water quality: a contemporary review for researchers and policymakers
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
现在去查看 取消
×
提示
确定
0
微信
客服QQ
Book学术公众号 扫码关注我们
反馈
×
意见反馈
请填写您的意见或建议
请填写您的手机或邮箱
已复制链接
已复制链接
快去分享给好友吧!
我知道了
×
扫码分享
扫码分享
Book学术官方微信
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术
文献互助 智能选刊 最新文献 互助须知 联系我们:info@booksci.cn
Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。
Copyright © 2023 Book学术 All rights reserved.
ghs 京公网安备 11010802042870号 京ICP备2023020795号-1