设计反向传播神经网络预测TiO2-MEA/MDEA混合胺纳米流体的CO2传质增强因子

Xue Li , Jiamin Qin , Xining Wu , Chaoyang Wei , Long Xu
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摘要

本研究提出了一种新的方法,利用人工神经网络中的反向传播神经网络(BPNN)模型预测TiO2单乙醇胺/甲基二乙醇胺(MEA/MDEA)混合胺纳米流体的CO2吸收增强性能。TiO2 MEA/MDEA纳米流体的吸收增强因子是通过两步法在不同纳米颗粒固体含量(0.4–1.4​g/L)。结果表明,随着纳米粒子固体含量的增加,增强因子先增大后减小,极值出现在0.6​g/L。基于实验数据,使用相关的经验公式和反向传播神经网络(BPNN)模型来估计纳米流体的增强因子,两者都表现出良好的适用性。此外,还提出了一个结合遗传算法、粒子群算法和自适应学习率(C-BPNN)的优化模型来估计增强因子。与经验公式和BPNN相比,C-BPNN表现出更高的预测精度(所有数据R2​=​0.9966)和更快的预测速率。关键参数(纳米粒子固体含量、MEA和MDEA的浓度)的重量分析表明,在吸收增强过程中,纳米粒子固体含量的相对重要性最高(42.63%)。所有这些结果表明,神经网络可以为纳米流体转移领域的研究提供指导作用。
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Designing back propagation neural network to predict CO2 mass transfer enhancement factor of TiO2-MEA/MDEA blended amine nanofluids

This study presented a novel methodology to predict the CO2 absorption enhancement performance of TiO2-Monoethanolamine/Methyl diethanolamine (MEA/MDEA) blended amine nanofluids using back propagation neural network (BPNN) model in artificial neural networks. The absorption enhancement factor of TiO2-MEA/MDEA nanofluid were determined experimentally by a two-step method with various nanoparticle solid contents (0.4–1.4 ​g/L). The results showed that the enhancement factor was firstly increased and then decreased with the rising nanoparticle solid content, and the extreme point appeared at 0.6 ​g/L. Based on the experimental data, a relevant empirical formula and a back propagation neural network (BPNN) model were used to estimate the enhancement factor of nanofluid and both exhibited good applicability. Additionally, an optimization model incorporating genetic algorithm, particle swarm algorithm and adaptive learning rate (C-BPNN) was also proposed to estimate the enhancement factor. Compared with the empirical formula and BPNN, C-BPNN exhibited a higher prediction accuracy (all data R2 ​= ​0.9966) and a faster prediction rate. The weight analysis of key parameters (nanoparticle solid content, concentration of MEA and MDEA) showed that the relative importance of nanoparticle solid content was foremost (42.63%) in the absorption enhancement process. All these results indicate that the neural network can provide a guiding role for the research in the field of nanofluid transfer.

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