三组分高耐久性光催化材料的合成

Hung Hoang Van, Thoa Tran Thi
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引用次数: 0

摘要

以不同的前驱体为原料,采用共沉淀法和水热法制备了具有叔元(还原石墨烯- tio2 - fe3o4,表示为GrTiFe)组分的高耐久性、可回收性和低成本的降解有毒有机化合物的材料。通过这种方法,TiO2和Fe3O4纳米颗粒在还原的氧化石墨烯上生长。采用x射线衍射(XRD)、傅里叶变换红外光谱(FT-IR)、扫描电镜(sem)和磁滞学(magnetic hysteresis)对合成的纳米复合材料进行了表征,并对盐酸黑(MDB)的光降解反应进行了研究。结果表明,合成的复合材料的光催化活性远高于纯TiO2纳米粒子,并且复合材料可以很容易地从水中回收再利用。此外,GrTiFe还能够在模拟阳光辐射下降解有机化合物。
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Synthesis of the high durability photocatalytic materials with tertiary components
The high durability, re-collectable and low-cost materials with tertiary (reduced graphene-TiO2-Fe3O4, denoted as GrTiFe) components for degradation of toxic organic compounds have been prepared from different precursors by coprecipitation and hydrothermal methods. By this procedure, TiO2 and Fe3O4 nanoparticles have been growing on the reduced graphene oxide. The as-synthesized nanocomposites have been characterized with X-ray diffraction (XRD), Fourier transform infrared spectroscopy (FT-IR), scanning electron microscope and magnetic hysteresis, and studied on the photo-degradation reaction of Moderacid Black (MDB). The result shows that the photocatalytic activity of as-synthesized composites is much higher than that of pure TiO2 nanoparticles and the composites can be easily collected from water using a magnet for reusing. In addition, the GrTiFe is also able to degrade the organic compounds under modeling sunlight radiation.
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