Examination of fuel elements irradiated in the reactor of the World’s First NPP after long-term storage

Sergey N. Ivanov, Sergey I. Porollo, Sergey V. Shulepin, Yury D. Baranaev, Vladimir F. Timofeev, Yury V. Kharizomenov
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Abstract

Examinations of fuel elements with two different fuel compositions, U-Mo+Mg and UO 2 +Mg, irradiated in the AM reactor after their long-term storage do not reveal any visible defects on the surface of their outer claddings. However, in the fuel elements with U-Mo fuel, an increase in the diameter of the outer cladding is observed. This is most noticeable in the upper part of the fuel element. Storage of the fuel elements with UO 2 fuel for 15–22 years does not lead to a change in their diameter within the measurement accuracy. At the same time, metallographic studies have shown that on the external surface of the outer cladding and the internal surface of the inner cladding of the fuel elements with U-Mo+Mg and UO 2 +Mg fuel compositions, after long-term storage, defects are observed in the form of intergranular and irregular frontal corrosion, pits and pittings up to 20 µm deep. No interaction is found at the points of contact between the fuel claddings and the fuel composition of the layers. There is no noticeable decrease in the thickness of the outer and inner claddings of the fuel elements after long-term storage, nor does the thickness of the claddings at the locations of defects go beyond its minimum initial value, taking into account the technological tolerance for variations in thickness. It is noteworthy, however, that cracks are found in both types of fuel elements both in the fuel grains and in the magnesium matrix. As a result of long-term storage of the fuel elements with U-Mo fuel for 45–55 years, the mechanical properties of their outer claddings gradually degrade, due to which the plasticity of the cladding is significantly reduced.
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Examination的燃料元件辐照后的反应堆,在世界上第一个核电站的长期储存
对两种不同燃料成分的燃料元件(U-Mo+Mg和UO 2 +Mg)在长期储存后在AM反应堆中辐照的检查未发现其外包层表面有任何可见的缺陷。然而,在使用铀钼燃料的燃料元件中,可以观察到外包层直径的增加。这在燃料元件的上部最为明显。使用UO 2燃料的燃料元件储存15-22年不会导致其直径在测量精度范围内发生变化。同时,金相研究表明,在U-Mo+Mg和UO 2 +Mg燃料成分的燃料元件的外包层外表面和内包层内表面,经过长期存放后,出现了晶间和不规则的正面腐蚀,凹坑和点蚀深度可达20µm。在燃料包壳和各层燃料组成之间的接触点没有发现相互作用。考虑到厚度变化的技术公差,长期储存后燃料元件的内外包层厚度没有明显下降,缺陷位置的包层厚度也没有超过其最小初始值。然而,值得注意的是,在两种类型的燃料元件中,在燃料颗粒和镁基体中都发现了裂纹。铀钼燃料元件长期存放45 ~ 55年,其外包层的力学性能逐渐退化,包层的塑性明显降低。
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