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Potential role of nuclear power in a carbon-free world 核能在无碳世界中的潜在作用
Pub Date : 2024-06-04 DOI: 10.3897/nucet.10.121449
Andrey V. Kaplienko, B. Gabaraev, Yuriy S. Cherepnin
Thermal Power Plants (ThPP), along with transport facilities, are the major sources for industrial emissions of carbon dioxide (CO2) believed to be responsible for the greenhouse effect leading to overheating of the lower atmosphere. In the opinion of many scientists, there is a threshold value of the average atmospheric temperature exceeding, which entails the potential for the development of irreversible processes threatening the existence of humankind. To avoid this danger, governments in nearly 200 countries have chosen voluntarily to reach net-zero CO2 emissions by 2050. Renewable Energy Sources (RES), including wind and solar power plants, have been selected as substitutes for ThPPs. However, energy systems based on RES only need to be multiply redundant in terms of installed capacity due to their efficiency being heavily dependent on daily, seasonal and weather factors, leave alone the scale of the required material resources (metals, polymers, concrete, glass, etc.). The major drawback of such energy systems is, however, the RES common-cause failure, e.g., in the event of a global volcanic eruption, when no energy-security requirement can be met to provide energy for satisfying the most vital needs. A need is fully evident for furnishing such energy system with another power source to be not dependent on the event that has caused the mass RES failure. With the net-zero-carbon requirement taken into account, Nuclear Power (NP) appears to be the best option in this respect. Modern NP does not however fully suits this role due to its inherent drawbacks (limited fuel resources, pending Spent Nuclear Fuel (SNF) and RadioActive Wastes (RAW) handling and nuclear-material nonproliferation issues). A potential solution to these drawbacks is a two-component NP technology in a closed nuclear-fuel cycle currently in the process of development. In Russia, where the greatest progress has been achieved in this field of development, under construction is a pilot and demonstration energy complex with the BREST-OD-300 nuclear unit expected to be started up in 2026–2027. Another promising designs to be developed are Small Modular Reactors (SMRs) / Small Nuclear Power Plants (SNPPs).
火力发电厂(ThPP)和交通设施是工业排放二氧化碳(CO2)的主要来源,据信,二氧化碳是导致大气层过热的温室效应的罪魁祸首。许多科学家认为,大气平均温度有一个临界值,如果超过这个临界值,就有可能出现不可逆转的过程,威胁到人类的生存。为了避免这一危险,近 200 个国家的政府自愿选择到 2050 年实现二氧化碳净零排放。可再生能源(RES),包括风能和太阳能发电厂,已被选为 ThPPs 的替代品。然而,基于可再生能源的能源系统在装机容量方面只需成倍冗余,因为其效率在很大程度上取决于日常、季节和天气因素,更不用说所需的材料资源(金属、聚合物、混凝土、玻璃等)的规模了。然而,这种能源系统的主要缺点是可再生能源系统的常见故障,例如,在全球火山爆发时,无法满足能源安全要求,无法提供满足最重要需求的能源。显然,有必要为这种能源系统提供另一种动力源,使其不依赖于造成可再生能源大规模故障的事件。考虑到净碳为零的要求,核能(NP)似乎是这方面的最佳选择。然而,由于其固有的缺点(燃料资源有限、乏核燃料(SNF)和放射性废物(RAW)的处理以及核材料的不扩散问题),现代核能并不能完全胜任这一角色。目前正在开发的封闭式核燃料循环中的双组分核燃料技术是解决这些缺点的潜在方案。俄罗斯在这一领域的开发取得了最大进展,目前正在建设一个试点和示范能源综合体,其中的 BREST-OD-300 核电机组预计将于 2026-2027 年启动。另一个有望开发的设计是小型模块化反应堆(SMRs)/小型核电站(SNPPs)。
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引用次数: 0
Corrosion resistance of chromium coating on the inner surface of EP823-Sh steel cladding EP823-Sh 钢包层内表面铬涂层的抗腐蚀性能
Pub Date : 2024-05-07 DOI: 10.3897/nucet.10.119642
Rafael Sh. Isayev, Pavel Dzhumaev, Irina A. Naumenko, Maria V. Leontieva-Smirnova
The processes of corrosion damage of the inner surface of the cladding are determined by corrosive reagents aggressive with respect to the cladding and the type of fuel used. Reactor irradiation of cladding made of EP823-Sh steel with mixed nitride fuel planned for use in the BREST-OD-300 reactor revealed non-uniform corrosion of the inner surface of the cladding. In this paper, the use of the chromium coating is proposed to prevent the corrosion of the inner surface of the steel fuel cladding. The results of corrosion tests of chromium coating applied to the inner surface of cladding made of EP823-Sh steel by electrolytic deposition are presented. Electron-microscopic studies of the chromium coating on EP823-Sh steel showed no significant signs of corrosion damage when tested in the environment of simulant fission products (CsI+Te) and in liquid lead at 650 °C.
包层内表面的腐蚀破坏过程是由对包层和所用燃料类型具有侵蚀性的腐蚀试剂决定的。对计划用于 BREST-OD-300 反应堆的 EP823-Sh 钢包层和混合氮化物燃料进行反应堆辐照后发现,包层内表面的腐蚀并不均匀。本文建议使用铬涂层来防止钢制燃料包壳内表面的腐蚀。本文介绍了通过电解沉积法对 EP823-Sh 钢制覆层内表面进行铬涂层腐蚀试验的结果。对 EP823-Sh 钢铬涂层进行的电子显微镜研究表明,在模拟裂变产物(CsI+Te)环境和 650 °C 下的液态铅环境中进行测试时,没有发现明显的腐蚀破坏迹象。
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引用次数: 0
A brief investigation of the dose field virtual simulation tools for reactor decommissioning and preliminary design for the HWRR reactor in China 反应堆退役剂量场虚拟仿真工具的简要调查和中国水力发电反应堆的初步设计
Pub Date : 2024-01-22 DOI: 10.3897/nucet.10.114088
Yaping Guo, Peng Nie, Ruizhi Li, Lijun Zhang, Xingwang Zhang, Ren Ren, Zelong Zhao
The calculation and visualization of the dose field in the decommissioning of nuclear facilities is one of the important functions of the decommissioning virtual simulation system. The dose field simulation tools can provide radiation field distribution and play an important role in determining the decommissioning plan and protecting personnel during the engineering implementation process. This article investigates the development of dose field calculation and visualization in the reactor decommissioning virtual simulation systems. A preliminary technology plan suitable for the development of the decommissioning dose field calculation and visualization display programs of the first Heavy Water Research Reactor (HWRR) in China is proposed. The applicability of the selected scheme is analyzed. The functional requirement and development direction of the HWRR reactor decommissioning dose field tool are preliminarily determined. Furthermore, the reactor vessel of HWRR reactor is modeled, the dose field distribution is calculated and visualized based on the preliminary decommissioning code. This research can provide technical support for the development of the decommissioning simulation system for the first HWRR reactor in China.
核设施退役过程中剂量场的计算和可视化是退役虚拟仿真系统的重要功能之一。剂量场仿真工具可以提供辐射场分布,在工程实施过程中对退役方案的确定和人员保护起到重要作用。本文研究了反应堆退役虚拟仿真系统中剂量场计算和可视化的开发。提出了适合中国第一座重水研究堆退役剂量场计算和可视化显示程序开发的初步技术方案。分析了所选方案的适用性。初步确定了重水堆退役剂量场工具的功能要求和开发方向。此外,还对华龙一号反应堆容器进行了建模,并基于初步的退役代码对剂量场分布进行了计算和可视化。该研究可为我国首座华龙一号反应堆退役模拟系统的开发提供技术支持。
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引用次数: 0
Assessment of the possibility for large-scale 238Pu production in a VVER-1000 power reactor 评估在 VVER-1000 型动力反应堆中大规模生产 238Pu 的可能性
Pub Date : 2023-12-21 DOI: 10.3897/nucet.9.117199
A. Shmelev, N. Geraskin, V. Apse, G. G. Kulikov, E. G. Kulikov, Vasily B. Glebov
The paper presents the estimates for the possibility for large-scale production of 238Pu in the core of a VVER-1000 power reactor. The Np-fraction of minor actinides extracted from transuranic radioactive waste is proposed to be used as the starting material. The irradiation device with NpO2 fuel elements is installed at the reactor core center. The NpO2 fuel lattice pitch is varied and the irradiation device is surrounded by a heavy moderator layer to create the best possible spectral conditions for large-scale production (~ 3 kg/year) of conditioned plutonium with the required isotopic composition (not less than 85% of 238Pu and not more than 2 ppm of 236Pu). Plutonium with such isotopic composition can be used as the thermal source in thermoelectric radioisotope generators and in cardiac pacemakers. It has been demonstrated that the estimated scale of the 238Pu production in a VVER-type power reactor exceeds considerably the existing scale of its production in research reactors.
本文对在 VVER-1000 型动力反应堆堆芯中大规模生产 238Pu 的可能性进行了估算。建议使用从超铀放射性废物中提取的小锕系元素的镎馏分作为起始材料。带有二氧化铌燃料元件的辐照装置安装在反应堆堆芯中心。二氧化铌燃料的晶格间距是变化的,辐照装置周围有重载慢化剂层,以便为大规模生产(约 3 千克/年)具有所需同位素组成(238Pu 不低于 85%,236Pu 不超过 2 ppm)的有条件钚创造最佳光谱条件。具有这种同位素组成的钚可用作热电放射性同位素发生器和心脏起搏器的热源。事实证明,在 VVER 型动力反应堆中生产 238Pu 的估计规模大大超过了在研究反应堆中生产 238Pu 的现有规模。
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引用次数: 0
Some economic aspects of reducing americium production in a two-component system of thermal and fast reactors 减少热堆和快堆两部分系统镅生产的一些经济问题
Pub Date : 2023-12-19 DOI: 10.3897/nucet.9.116655
A. Gulevich, V. Usanov, V. Dekusar, V. A. Eliseev, A. Moseev, E. S. Khnykina
The article analyzes the economic aspects of reducing the production of americium during the transition from a single-component nuclear energy system (NES) based on thermal reactors in an open fuel cycle to a two-component system with thermal and fast reactors in a closed nuclear fuel cycle. Scenarios for the development of these systems in Russia up to the end of the century are modeled. Two methods are considered for reducing the production of americium in a two-component NES with fast sodium reactors. The first method, closing the fuel cycle for plutonium in BN reactors of SFR type, is based on the use of plutonium separated from spent nuclear fuel of thermal reactors with the shortest possible (according to technical specifications) time for MOX fuel preparation and use thus preventing the main part of plutonium-241 from decay into americium. The second way is transmutation of americium. The study was carried out by using the mathematical code CYCLE designed for modeling of the NES with closed nuclear fuel cycle (NFC). The technical and economic data used in the paper was taken from published studies of Russian specialists and materials of European Union specialists presented in the IAEA/INPRO SYNERGIES project. The results of the research show that the efficiency of closing the NFC by using plutonium from thermal reactors in MOX fuel of fast sodium reactors is comparable to the efficiency of the homogeneous transmutation considered in the paper. The combination of the americium accumulation prevention method and transmutation method might significantly reduce the rate of the americium accumulation in a nuclear energy system, but the estimated costs of the considered homogeneous transmutation can significantly worsen the economic performance of sodium fast reactors.
文章分析了在从基于开放燃料循环中热反应堆的单组分核能系统(NES)向包含封闭核燃料循环中热反应堆和快堆的双组分系统过渡期间减少镅生产的经济方面。模拟了到本世纪末俄罗斯发展这些系统的情景。考虑了两种方法,以减少带有快钠反应堆的双组份核燃料循环系统中的镅产量。第一种方法是关闭 SFR 型 BN 反应堆中的钚燃料循环,其基础是使用从热反应堆乏核燃料中分离出来的钚,以尽可能短的时间(根据技术规范)制备和使用 MOX 燃料,从而防止钚-241 的主要部分衰变为镅。第二种方法是镅的嬗变。这项研究使用了为封闭式核燃料循环(NFC)核能源系统建模而设计的数学代码 CYCLE。论文中使用的技术和经济数据来自俄罗斯专家发表的研究报告和国际原子能机构/INPRO SYNERGIES 项目中欧盟专家提供的材料。研究结果表明,在快钠堆的混合氧化物燃料中使用来自热反应堆的钚来关闭核燃料循环的效率与本文所考虑的均相嬗变的效率相当。镅积累预防方法和嬗变方法的结合可能会显著降低核能系统中的镅积累率,但所考虑的均相嬗变的估计成本会显著恶化钠快堆的经济性能。
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引用次数: 0
Study into the dependence of the Co-60 and Lu-177g production efficiency on the energy structure of neutron flux density 研究 Co-60 和 Lu-177g 的生产效率与中子通量密度能量结构的关系
Pub Date : 2023-12-19 DOI: 10.3897/nucet.9.116662
Ruben A. Shaginyan, Valery V. Korobeinikov, Viktor Yu. Stogov
At present, the existing approaches to production of artificial isotopes are mostly based on the development experience from previous years. This work aims to develop an algorithm for selecting the most effective irradiation modes for target materials. The study is based on sequential modeling of irradiation of target isotopes by neutrons of different ‘single-group’ fluxes at the same neutron flux density within each energy group (BNAB-93). In this study, a flux density equal to 2×1015 n/(cm2×s) was used for each energy group. This approach will help ‘designing’ and selecting the actual neutron spectrum that has the highest efficiency compared to alternatives. The study modelled Co-60 and Lu-177g production for each energy group. The kinetics was analyzed in the most efficient groups in terms of specific activity. The maximum specific activity for Co-60 is reached in group 17 and is equal to 1 kCi/g. For the scheme of Lu-177g production through Lu-176 the maximum specific activity is reached in group 26 and is equal to 58.5 kCi/g. For the scheme of Lu-177g production through Yb-176, the maximum specific activity is reached in group 17 and is equal to 260 Ci/g, advantageous for production are groups 15–17 and 26.
目前,生产人造同位素的现有方法大多基于前几年的开发经验。这项工作旨在开发一种算法,用于选择对目标材料最有效的辐照模式。研究基于在每个能量组(BNAB-93)内以相同的中子通量密度用不同 "单组 "通量的中子辐照目标同位素的顺序建模。在这项研究中,每个能量组使用的通量密度等于 2×1015 n/(cm2×s)。这种方法有助于 "设计 "和选择与其他方法相比效率最高的实际中子能谱。研究模拟了每个能量组的 Co-60 和 Lu-177g 产生情况。从比活度的角度对效率最高的组别进行了动力学分析。第 17 组达到了 Co-60 的最大比活度,等于 1 kCi/g。通过 Lu-176 生产 Lu-177g 的方案在第 26 组达到最大比活度,相当于 58.5 kCi/g。在通过 Yb-176 生产 Lu-177g 的方案中,第 17 组达到最大比活度,等于 260 Ci/g。
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引用次数: 0
A computer code for optimizing the neutronics model parameters based on results of reactor physics experiments 根据反应堆物理实验结果优化中子模型参数的计算机代码
Pub Date : 2023-12-19 DOI: 10.3897/nucet.9.117198
A. Andrianov, O. Andrianova, Yury A. Korovin, Iliya S. Kuptsov, Anastasiya A. Spiridonova
The paper describes in brief the functional capabilities of a computer code for optimizing the neutronics model parameters (neutron data, technological parameters, and their covariance matrices) based on results of reactor physics experiments using conditional nonlinear multi-parameter optimization algorithms. The code’s application scope includes adjustment of neutron constants, technological parameters and their covariance matrices based on integral measurement results, formulation of requiremen117198ts with respect to the neutron data uncertainties for achieving the target accuracies in calculation of the reactor functionals, and estimation of the reactor performance prediction accuracy, as well as the informativity and similarity metrics of reactor physics experiments with respect to each other and in relation to the target reactor system. The paper also considers some examples of using the code to refine the neutronics models of nuclear reactor and fuel cycle systems based on results of reactor physics experiments.
本文简要介绍了基于反应堆物理实验结果,利用条件非线性多参数优化算法对中子模型参数(中子数据、技术参数及其协方差矩阵)进行优化的计算机代码的功能。该代码的应用范围包括:根据积分测量结果调整中子常数、技术参数及其协方差矩阵;制定与中子数据不确定性相关的要求 117198t,以实现反应堆功能计算的目标精度;估算反应堆性能预测精度;以及反应堆物理实验相互之间以及与目标反应堆系统相关的信息性和相似性指标。论文还考虑了根据反应堆物理实验结果使用该代码完善核反应堆和燃料循环系统中子模型的一些实例。
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引用次数: 0
Principles of construction and development of an automatic protection system for steam generators of fast reactors 建造和开发快堆蒸汽发生器自动保护系统的原则
Pub Date : 2023-12-19 DOI: 10.3897/nucet.9.116657
Vyacheslav V. Borisov, Aleksey A. Kamaev, Olga I. Myazdrikova, Stepan A. Mikhin, Ilia А. Pakhomov, Sergey V. Perevoznikov
On the example of domestic fast reactors BN-350, BN-600, BN-800, the evolution of technical solutions for the automatic protection system of sodium-water steam generators (SG APS) is analyzed. The structural diagrams and main characteristics of the SG APS equipment of listed reactors are presented. The effectiveness of the SG APS in conditions of real leaks in steam generators of BN reactors is analyzed. The issues of development and creation of the SG APS of designed BN-1200 and INU MBIR are considered.
以国产快堆 BN-350、BN-600、BN-800 为例,分析了钠水蒸汽发生器自动保护系统(SG APS)技术方案的演变。介绍了所列反应堆钠水蒸汽发生器自动保护系统设备的结构图和主要特点。分析了 SG APS 在 BN 反应堆蒸汽发生器实际泄漏条件下的有效性。考虑了为 BN-1200 和 INU MBIR 设计的 SG APS 的开发和创建问题。
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引用次数: 0
Analytical dependence of burnup on enrichment of prospective fuel and parameters of reactors fuel campaign 燃耗与预期燃料浓缩度和反应堆燃料运行参数的分析关系
Pub Date : 2023-12-12 DOI: 10.3897/nucet.9.116653
Evgeny V. Semenov, V. V. Kharitonov
The paper is devoted to the definition of an analytical expression for estimating the burnup depth of nuclear fuel depending on its enrichment level, the periodicity of refueling, thermal stressthermal stress and the duration of the time period between refueling (reactor campaign) in a wide range of changes in key parameters for different types of thermal neutron reactors. The analytical expressions obtained in the work for the burnup depth are compared with numerous neutron physics calculations and experimental data from different authors for uranium fuel enrichment up to 9%. Calculations of the fuel share of the cost of electricity of nuclear power plants with PWR type reactors were performed and its sensitivity to changes in burnup depth and enrichment of fuel, the refueling periodicity, as well as to market prices for natural uranium, conversion, enrichment, fabrication of fuel assemblies and SNF handling were determined.
本文致力于定义一个分析表达式,用于估算核燃料的燃耗深度,该表达式取决于不同类型热中子反应堆在关键参数变化范围较大的情况下的浓缩水平、换料周期、热应力和换料间隔时间(反应堆运行)。工作中获得的关于燃耗深度的分析表达式与不同作者针对铀燃料浓缩度高达 9% 的情况所做的大量中子物理计算和实验数据进行了比较。对压水堆型反应堆核电厂电力成本中的燃料份额进行了计算,并确定了其对燃耗深度和燃料浓缩度变化、换料周期以及天然铀市场价格、转换、浓缩、燃料组件制造和 SNF 处理的敏感性。
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引用次数: 0
Radioecological modeling of the 131I activity dynamics in the pasture vegetation of Mazovia in the year of the Chernobyl accident: Reconstruction, verification, reliability assessments 切尔诺贝利事故发生当年马佐维亚牧场植被中 131I 活性动态的放射生态学模型:重建、验证、可靠性评估
Pub Date : 2023-12-12 DOI: 10.3897/nucet.9.116654
Oleg K. Vlasov, I. Zvonova, N. V. Shchukina, S. Chekin
A radioecological model, which is a system of linear differential equations describing the dynamics of the transport of 137Cs and 131I radionuclides along the food chain after their release into the atmosphere after the Chernobyl accident, was used to reconstruct “instrumental” data of the 131I activities in the grass pastures in the central part of Mazovia. Four atmospheric models were used for the reconstruction: direct calculation, homogeneous cloud – inhomogeneous rainfall, inhomogeneous cloud – homogeneous rainfall, and a model with recalculation of the 137Cs and 131I activities in the atmosphere. The “instrumental” data were reconstructed based on data from direct measurements of the 131I activity in lawn grass. It has been shown that the direct calculation and homogeneous cloud models lead to a better agreement of the calculated and reconstructed “instrumental” data than the inhomogeneous cloud model. The arithmetic mean ratio of the calculated and reconstructed “instrumental” data lie in a range of 0.84 to 0.95 for the direct calculation and homogeneous cloud models, and in a range of 1.7 to 3.0 for the inhomogeneous cloud model. The mean geometric deviation for all models is constant and equal to 1.7. Instrumental and reconstructed “instrumental” data show a significant decrease in the specific activity of 131I in grass due to its wash-off by continuous rainfall, both during rainfall and after most of the deposition takes place. Due to this effect, the coefficient of the 131I retention on grass in the form of the maximum activity ratio to the 137Cs deposition density decreases from 34 to 1.4 m2/kg while it increases from 1 to 29 kBq/m2 as the result of the rainfall growth from 0 to 40 mm.
切尔诺贝利事故发生后,137Cs 和 131I 放射性核素释放到大气中,放射性生态学模型是描述这两种放射性核素沿食物链迁移动态的线性微分方程系统,该模型用于重建马佐维亚中部草场 131I 放射性活度的 "仪器 "数据。重建中使用了四种大气模型:直接计算、均质云-非均质降雨、非均质云-均质降雨以及重新计算大气中 137Cs 和 131I 活性的模型。仪器 "数据是根据对草坪草中 131I 活性的直接测量数据重建的。结果表明,直接计算和均质云模型与非均质云模型相比,计算和重建的 "仪器 "数据的一致性更好。直接计算和均质云模型的计算和重建 "仪器 "数据的算术平均比率在 0.84 至 0.95 之间,非均质云模型在 1.7 至 3.0 之间。所有模型的平均几何偏差都是恒定的,等于 1.7。仪器数据和重建的 "仪器 "数据显示,在降雨过程中和大部分沉积发生后,由于连续降雨对 131I 的冲刷,草地中 131I 的比活度显著下降。由于这种影响,131I 在草地上的保留系数(最大活性与 137Cs 沉积密度之比)从 34 m2/kg 降至 1.4 m2/kg,而随着降雨量从 0 毫米增至 40 毫米,则从 1 kBq/m2 增至 29 kBq/m2。
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引用次数: 0
期刊
Nuclear Energy and Technology
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