Investigation of electric field distribution on dielectric exposed to DC-pulsed He plasma jet with shielding gas

Guoqiang Liu, Yang Xia, Kefeng Shang, Dongping Liu
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Abstract

Abstract Atmospheric pressure plasma jets (APPJs) produce reactive species and electric fields for biomedical applications. Gas shields control plasma plume-surrounding gas interactions, regulating reactive species generation and electric field strength. However, the surface electric field distribution is still unclear and needs urgent attention. Here, the electric field distribution on the surface exposed to a helium APPJ with shielding gas is investigated using the Pockels technique. This study considers the influence of the type of shielding gas (ambient air, dry air, nitrogen, oxygen, nitrogen-oxygen mixture) and the flow rate (2000–6000 sccm). The results show that the surface electric field develops in three phases: establishment, maintenance, and dissipation. Both flow rate and oxygen content of the shielding gas significantly influence surface discharge behavior and the maximum electric field value. The analysis suggests that the establishment phase of the electric field results from charge transfer by ionization waves to the dielectric, while the maintenance of the electric field depends on pulse duration. During the dissipation phase, the positive surface charge attracts negatively charged species to the surface (electrons and negative ions), which causes charge neutralization at the surface. The oxygen content in the shielding gas impacts the electric field establishment phase, with a low oxygen content leading to lower photo-ionization rates and, consequently, surface discharges with branching. Shielding gas flow rates affect the amount of shielding gas mixed into the helium channel. Mixing less oxygen into the APPJ increases the electric field strength, as the ionization potential is lower than nitrogen. Excessive oxygen mixing traps more free electrons due to electronegativity, causing fewer ionized collisions and more negative ions in APPJ, ultimately lowering the electric field strength. This study shows that shielding gas type and flow rates can adjust surface charging, aiding in optimizing biomedical APPJ.
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带保护气体的直流脉冲He等离子体射流对介质电场分布的影响
大气压等离子体射流(APPJs)产生反应物质和电场,用于生物医学应用。气体屏蔽控制等离子体羽流周围的气体相互作用,调节反应物质的产生和电场强度。然而,表面电场分布尚不清楚,亟待关注。本文利用Pockels技术研究了有保护气体的氦APPJ表面的电场分布。本研究考虑了保护气体类型(环境空气、干燥空气、氮气、氧气、氮氧混合气体)和流量(2000-6000 sccm)的影响。结果表明,表面电场的发展经历了建立、维持和耗散三个阶段。保护气体的流量和含氧量对表面放电行为和最大电场值均有显著影响。分析表明,电场的建立相位是电离波向介质转移电荷的结果,而电场的维持取决于脉冲的持续时间。在耗散阶段,表面正电荷吸引带负电荷的物质(电子和负离子)到表面,这导致表面的电荷中和。保护气体中的氧含量影响电场建立阶段,低氧含量导致较低的光电离速率,从而导致具有分支的表面放电。保护气体流量影响保护气体混入氦通道的量。在APPJ中加入较少的氧会增加电场强度,因为它的电离电位比氮低。过量的氧混合由于电负性会捕获更多的自由电子,导致APPJ中的电离碰撞减少,负离子增多,最终降低电场强度。研究表明,保护气体类型和流量可以调节表面充电,有助于优化生物医学APPJ。
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