Solid electrolyte membranes for all-solid-state rechargeable batteries

IF 15 1区 工程技术 Q1 ENERGY & FUELS Etransportation Pub Date : 2024-02-19 DOI:10.1016/j.etran.2024.100319
Nini Zhang , Xiaolei Zhao , Gaozhan Liu , Zhe Peng , Jinghua Wu , Mingyang Men , Xiayin Yao
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Abstract

All-solid-state lithium batteries employing solid electrolyte instead of organic liquid electrolyte and separator have been regarded as one of the most favorable candidates for next generation energy storage devices due to their unparalleled safety and energy density. Recently, significant progresses have been made on developing suitable solid electrolytes for all-solid-state lithium batteries with high ionic conductivity, wide electrochemical window and favorable electrode compatibility. Nevertheless, owing to the brittle nature of inorganic solid electrolytes and limited mechanic property of solid polymer electrolytes, the typical thickness of solid electrolyte layers is excessively thick, which prevents further enhancing the energy density of all-solid-state rechargeable batteries. In this short review, we summary recent research progresses on solid electrolyte membranes based on wet coating, frame support and dry film methods. In particular, the critical parameters such as thickness, conductivity and mechanical property are discussed in detail. Finally, the future development directions of the solid electrolyte membranes are proposed.

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用于全固态充电电池的固体电解质膜
采用固态电解质代替有机液态电解质和隔膜的全固态锂电池因其无与伦比的安全性和能量密度,已被视为下一代储能设备最有利的候选材料之一。最近,在为全固态锂电池开发具有高离子电导率、宽电化学窗口和良好电极兼容性的合适固体电解质方面取得了重大进展。然而,由于无机固态电解质的脆性和固态聚合物电解质的有限力学性能,固态电解质层的厚度通常过厚,这阻碍了全固态充电电池能量密度的进一步提高。在这篇简短的综述中,我们总结了基于湿涂层、框架支撑和干膜方法的固体电解质膜的最新研究进展。特别是详细讨论了厚度、电导率和机械性能等关键参数。最后,提出了固体电解质膜的未来发展方向。
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来源期刊
Etransportation
Etransportation Engineering-Automotive Engineering
CiteScore
19.80
自引率
12.60%
发文量
57
审稿时长
39 days
期刊介绍: eTransportation is a scholarly journal that aims to advance knowledge in the field of electric transportation. It focuses on all modes of transportation that utilize electricity as their primary source of energy, including electric vehicles, trains, ships, and aircraft. The journal covers all stages of research, development, and testing of new technologies, systems, and devices related to electrical transportation. The journal welcomes the use of simulation and analysis tools at the system, transport, or device level. Its primary emphasis is on the study of the electrical and electronic aspects of transportation systems. However, it also considers research on mechanical parts or subsystems of vehicles if there is a clear interaction with electrical or electronic equipment. Please note that this journal excludes other aspects such as sociological, political, regulatory, or environmental factors from its scope.
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