Mountaintop Removal Coal Mining Contaminates Snowpack across a Broad Region

IF 10.8 1区 环境科学与生态学 Q1 ENGINEERING, ENVIRONMENTAL 环境科学与技术 Pub Date : 2024-06-18 DOI:10.1021/acs.est.4c02596
Colin A. Cooke*, Kira M. Holland, Craig A. Emmerton, Paul E. Drevnick, Alison S. Criscitiello and Brandi Newton, 
{"title":"Mountaintop Removal Coal Mining Contaminates Snowpack across a Broad Region","authors":"Colin A. Cooke*,&nbsp;Kira M. Holland,&nbsp;Craig A. Emmerton,&nbsp;Paul E. Drevnick,&nbsp;Alison S. Criscitiello and Brandi Newton,&nbsp;","doi":"10.1021/acs.est.4c02596","DOIUrl":null,"url":null,"abstract":"<p >Mountaintop removal coal mining is a source of downstream pollution. Here, we show that mountaintop removal coal mining also pollutes ecosystems downwind. We sampled regional snowpack near the end of winter along a transect of sites located 3–60 km downwind of coal mining in the Elk River valley of British Columbia, Canada. Vast quantities of polycyclic aromatic compounds (PACs), a toxic class of organic contaminants, are emitted and transported atmospherically far from emission sources. Summed PAC (ΣPAC) snowpack concentrations ranged from 29–94,866 ng/L. Snowpack ΣPAC loads, which account for variable snowpack depth, ranged from &lt;10 μg/m<sup>2</sup> at sites &gt;50 km southeast of the mines to &gt;1000 μg/m<sup>2</sup> at sites in the Elk River valley near mining operations, with one site &gt;15,000 μg/m<sup>2</sup>. Outside of the Elk River valley, snowpack ΣPAC loads exhibited a clear spatial pattern decreasing away from the mines. The compositional fingerprint of this PAC pollution matches closely with Elk River valley coal. Beyond our study region, modeling results suggest a depositional footprint extending across western Canada and the northwestern United States. These findings carry important implications for receiving ecosystems and for communities located close to mountaintop removal coal mines exposed to air pollution elevated in PACs.</p><p >Snowpack samples from across the southern Canadian Rockies reveal widespread polycyclic aromatic compound pollution sourced from mountaintop removal coal mining.</p>","PeriodicalId":36,"journal":{"name":"环境科学与技术","volume":null,"pages":null},"PeriodicalIF":10.8000,"publicationDate":"2024-06-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/epdf/10.1021/acs.est.4c02596","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"环境科学与技术","FirstCategoryId":"1","ListUrlMain":"https://pubs.acs.org/doi/10.1021/acs.est.4c02596","RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"ENGINEERING, ENVIRONMENTAL","Score":null,"Total":0}
引用次数: 0

Abstract

Mountaintop removal coal mining is a source of downstream pollution. Here, we show that mountaintop removal coal mining also pollutes ecosystems downwind. We sampled regional snowpack near the end of winter along a transect of sites located 3–60 km downwind of coal mining in the Elk River valley of British Columbia, Canada. Vast quantities of polycyclic aromatic compounds (PACs), a toxic class of organic contaminants, are emitted and transported atmospherically far from emission sources. Summed PAC (ΣPAC) snowpack concentrations ranged from 29–94,866 ng/L. Snowpack ΣPAC loads, which account for variable snowpack depth, ranged from <10 μg/m2 at sites >50 km southeast of the mines to >1000 μg/m2 at sites in the Elk River valley near mining operations, with one site >15,000 μg/m2. Outside of the Elk River valley, snowpack ΣPAC loads exhibited a clear spatial pattern decreasing away from the mines. The compositional fingerprint of this PAC pollution matches closely with Elk River valley coal. Beyond our study region, modeling results suggest a depositional footprint extending across western Canada and the northwestern United States. These findings carry important implications for receiving ecosystems and for communities located close to mountaintop removal coal mines exposed to air pollution elevated in PACs.

Snowpack samples from across the southern Canadian Rockies reveal widespread polycyclic aromatic compound pollution sourced from mountaintop removal coal mining.

Abstract Image

Abstract Image

查看原文
分享 分享
微信好友 朋友圈 QQ好友 复制链接
本刊更多论文
开山采煤污染了整个地区的积雪。
开山采煤是下游污染的一个来源。在这里,我们证明了开山采煤也会污染下风向的生态系统。我们在加拿大不列颠哥伦比亚省埃尔克河流域煤矿开采的下风向 3-60 公里处的一个横断面上对临近冬末的区域积雪进行了采样。多环芳香族化合物(PAC)是一类有毒的有机污染物,其排放和大气传输距离排放源很远。雪层中 PAC(ΣPAC)的总浓度介于 29-94866 纳克/升之间。雪堆 ΣPAC 负荷(考虑到不同的雪堆深度)从矿区东南方向大于 50 公里处的 2 到埃尔克河流域采矿作业附近地点的大于 1000 μg/m2 不等,其中一个地点大于 15,000 μg/m2。在埃尔克河河谷以外的地区,雪堆 ΣPAC 负荷呈现出明显的空间模式,即在远离矿区的地方逐渐降低。这种 PAC 污染的成分特征与埃尔克河流域的煤炭非常吻合。在我们的研究区域之外,建模结果表明沉积足迹遍及加拿大西部和美国西北部。这些研究结果对受体生态系统和位于暴露于高浓度 PAC 空气污染的移山煤矿附近的社区具有重要意义。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
求助全文
约1分钟内获得全文 去求助
来源期刊
环境科学与技术
环境科学与技术 环境科学-工程:环境
CiteScore
17.50
自引率
9.60%
发文量
12359
审稿时长
2.8 months
期刊介绍: Environmental Science & Technology (ES&T) is a co-sponsored academic and technical magazine by the Hubei Provincial Environmental Protection Bureau and the Hubei Provincial Academy of Environmental Sciences. Environmental Science & Technology (ES&T) holds the status of Chinese core journals, scientific papers source journals of China, Chinese Science Citation Database source journals, and Chinese Academic Journal Comprehensive Evaluation Database source journals. This publication focuses on the academic field of environmental protection, featuring articles related to environmental protection and technical advancements.
期刊最新文献
Crystalline Phase Regulates Microbial Methylation Potential of Mercury Bound to MoS2 Nanosheets: Implications for Safe Design of Mercury Removal Materials. New Perspective to Evaluate the Carbon Offsetting by Urban Blue-Green Infrastructure: Direct Carbon Sequestration and Indirect Carbon Reduction. Occurrence, Sources and Virulence Potential of Arcobacter butzleri in Urban Municipal Stormwater Systems. Viral and Bacterial Community Dynamics in Food Waste and Digestate from Full-Scale Biogas Plants. High-Resolution Mass Spectrometry for Human Exposomics: Expanding Chemical Space Coverage.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
现在去查看 取消
0
微信
客服QQ
Book学术公众号 扫码关注我们
反馈
×
意见反馈
请填写您的意见或建议
请填写您的手机或邮箱
已复制链接
已复制链接
快去分享给好友吧!
我知道了
×
扫码分享
扫码分享
Book学术官方微信
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术
文献互助 智能选刊 最新文献 互助须知 联系我们:info@booksci.cn
Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。
Copyright © 2023 Book学术 All rights reserved.
ghs 京公网安备 11010802042870号 京ICP备2023020795号-1