Micro-mixing enhancement in a Taylor-Couette reactor using the inner rotors with various surface configurations

IF 3.8 3区 工程技术 Q3 ENERGY & FUELS Chemical Engineering and Processing - Process Intensification Pub Date : 2024-08-24 DOI:10.1016/j.cep.2024.109954
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Abstract

This study investigates the effects of various inner cylinder configurations on micromixing and fluid dynamics within a Taylor-Couette (TC) reactor using the inner cylinders with different surface designs, including the traditional smooth-surfaced rotor cylinder. The four innovative inner cylinders were specifically designed with axial corrugations (N40 and N80) and three-dimensional rough surfaces (NZ40 and NZ80). Micromixing efficiency was assessed experimentally using the iodide-iodate reaction as a probe. To further understand the impact of the rotors' surface structures on micromixing, computational fluid dynamics (CFD) modelling was utilized to analyse the fluid dynamics within the TC reactor. An incorporation model was employed to calculate the micromixing time. The experimental findings reveal that the segregation index decreases with increasing rotation speed for all inner cylinders. Besides, NZ80′s micro-mixing efficiency surpasses that of its counterparts, NZ40, N40, and N80. The CFD modelling results underscore the significant influence of the inner cylinder's surface configuration on the turbulence dissipation rate and volume probability distribution, which are likely to contribute positively to the micromixing efficiency within the TC reactor. Furthermore, the empirical correlations obtained have been established to understand the micro-mixing time within TC reactors using different rotating cylinders.

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利用不同表面结构的内转子增强泰勒-库瓦特反应器中的微混合效果
本研究使用不同表面设计的内筒(包括传统的光滑表面转子筒),研究了各种内筒配置对泰勒-库埃特(TC)反应器内微混合和流体动力学的影响。四种创新内筒的具体设计包括轴向波纹(N40 和 N80)和三维粗糙表面(NZ40 和 NZ80)。以碘-碘酸反应为探针,对微混合效率进行了实验评估。为了进一步了解转子表面结构对微混合的影响,利用计算流体动力学(CFD)建模来分析 TC 反应器内的流体动力学。计算微混合时间时采用了结合模型。实验结果表明,所有内筒的偏析指数都随着转速的增加而降低。此外,NZ80 的微混合效率超过了 NZ40、N40 和 N80。CFD 建模结果表明,内筒表面结构对湍流耗散率和体积概率分布有显著影响,这可能会对 TC 反应器内的微混合效率产生积极影响。此外,还建立了经验相关性,以了解使用不同旋转圆筒的 TC 反应器内的微混合时间。
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来源期刊
CiteScore
7.80
自引率
9.30%
发文量
408
审稿时长
49 days
期刊介绍: Chemical Engineering and Processing: Process Intensification is intended for practicing researchers in industry and academia, working in the field of Process Engineering and related to the subject of Process Intensification.Articles published in the Journal demonstrate how novel discoveries, developments and theories in the field of Process Engineering and in particular Process Intensification may be used for analysis and design of innovative equipment and processing methods with substantially improved sustainability, efficiency and environmental performance.
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