Analyzing Homogeneity of Highly Viscous Polymer Suspensions in Change Can Mixers.

IF 4.7 3区 工程技术 Q1 POLYMER SCIENCE Polymers Pub Date : 2024-09-23 DOI:10.3390/polym16182675
Michael Roland Larsen, Erik Tomas Holmen Olofsson, Jon Spangenberg
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Abstract

The mixing of highly viscous non-Newtonian suspensions is a critical process in various industrial applications. This computational fluid dynamics (CFD) study presents an in-depth analysis of non-isothermal mixing performance in change can mixers. The aim of the study was to identify parameters that significantly influence both distributive and dispersive mixing in these mixers, which are essential for optimizing industrial mixing processes. The study employed a numerical design of experiments (DOE) approach to identify the parameters that most significantly influence both distributive and dispersive mixing, as measured by the Kramer mixing index (MKramer) and the Ica Manas-Zloczower mixing index λMZ¯. The investigated parameters included mixing time, number of arms, arm size ratio, revolutions per minute (RPM), z-axis rotation, z-axis movement, and initial and mixing temperatures. The methodology involved employing the bootstrap forest algorithm for predicting the mixing indices, achieving an R2 of 0.949 for MKramer and an R2 of 0.836 for λMZ¯. The results indicate that the z-axis rotation has the greatest impact on both distributive and dispersive mixing. An increased number of arms negatively impacted λMZ, but had a small positive effect on MKramer. Surprisingly, in this study, neither the initial temperature of the material nor the mixing temperature significantly impacted the mixing performance. These findings highlight the relative importance of operational parameters over traditional temperature factors and provide a new perspective on mixing science.

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分析变罐混合器中高粘性聚合物悬浮液的均匀性。
高粘度非牛顿悬浮液的混合是各种工业应用中的一个关键过程。这项计算流体动力学(CFD)研究深入分析了变罐混合器中的非等温混合性能。研究的目的是确定对这些混合器中的分布式混合和分散式混合有重大影响的参数,这些参数对优化工业混合过程至关重要。研究采用了数值实验设计(DOE)方法,以确定对分布式和分散式混合影响最大的参数,这些参数由克拉默混合指数(MKramer)和伊卡马纳斯-兹洛佐尔混合指数 λMZ¯ 度量。研究参数包括混合时间、臂数、臂尺寸比、每分钟转数(RPM)、Z 轴旋转、Z 轴移动以及初始温度和混合温度。该方法采用自举森林算法预测混合指数,MKramer 的 R2 为 0.949,λMZ¯ 的 R2 为 0.836。结果表明,z 轴旋转对分布式和分散式混合的影响最大。臂的增加对 λMZ 有负面影响,但对 MKramer 有微小的正面影响。令人惊讶的是,在本研究中,材料的初始温度和混合温度都不会对混合性能产生显著影响。这些发现突出了操作参数相对于传统温度因素的重要性,为混合科学提供了一个新的视角。
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来源期刊
Polymers
Polymers POLYMER SCIENCE-
CiteScore
8.00
自引率
16.00%
发文量
4697
审稿时长
1.3 months
期刊介绍: Polymers (ISSN 2073-4360) is an international, open access journal of polymer science. It publishes research papers, short communications and review papers. Our aim is to encourage scientists to publish their experimental and theoretical results in as much detail as possible. Therefore, there is no restriction on the length of the papers. The full experimental details must be provided so that the results can be reproduced. Polymers provides an interdisciplinary forum for publishing papers which advance the fields of (i) polymerization methods, (ii) theory, simulation, and modeling, (iii) understanding of new physical phenomena, (iv) advances in characterization techniques, and (v) harnessing of self-assembly and biological strategies for producing complex multifunctional structures.
期刊最新文献
Correction: Rehman et al. Nanocomposite Membranes for PEM-FCs: Effect of LDH Introduction on the Physic-Chemical Performance of Various Polymer Matrices. Polymers 2023, 15, 502. Analysis and Evaluation of Load-Carrying Capacity of CFRP-Reinforced Steel Structures. Analyzing Homogeneity of Highly Viscous Polymer Suspensions in Change Can Mixers. Cross-Linking Agents in Three-Component Materials Dedicated to Biomedical Applications: A Review. High-Quality Foaming and Weight Reduction in Microcellular-Injection-Molded Polycarbonate Using Supercritical Fluid Carbon Dioxide under Gas Counter Pressure.
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