Design and experimental study of solar-driven biomass gasification based on direct irradiation solar thermochemical reactor

IF 12.5 1区 工程技术 Q1 ENGINEERING, CHEMICAL Chemical Engineering Journal Pub Date : 2024-10-24 DOI:10.1016/j.cej.2024.157062
Shuoshuo Wang, Xiaoli Zhu, Yun Liu, Zhang Bai, Qibin Liu, Xiankun Huang, Hongzhi Wang, Fan Jiao
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Abstract

Solar-driven biomass steam gasification is a promising technology to produce H2-rich syngas, meanwhile achieve flexible storage of renewable energy. However, the solar gasification application also faces numerous challenges, due to its involved complex chemical reaction characteristics and the inherent the multi-physics energy conversion processes. This work designs a novel direct irradiation solar gasification reactor, with the improved optical acceptance structure and reasonable test module, and the wheat straw particle is selected as experimental sample. Employing a 9 kWe high flux solar simulator, the maximum temperature of reaction bed in this prototype reactor reaches to 1260 °C, with the average solar flux of 1171.3 kW/m2. With adjustable radiation flux as experiment factor, under the highest total radiation of 3.35 kW, the molar fraction of H2 in the produced syngas is 47.1 % with the energy upgrade factor of 1.15, and the cellulose component completes decomposition. Increasing the mass flow rate of steam reduces the syngas output while raising the H2/CO ratio of the syngas. In addition, smaller biomass particle size facilitates the reaction, thereby improving the conversion efficiency of direct irradiation gasification. The investigation results provide a meaningful reference for the efficient utilization of abundant solar and biomass energy.
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基于直接辐照太阳能热化学反应器的太阳能驱动生物质气化设计与实验研究
太阳能驱动的生物质蒸汽气化技术在生产富含 H2- 的合成气的同时,还能实现可再生能源的灵活储存,是一项前景广阔的技术。然而,由于涉及复杂的化学反应特性和固有的多物理场能量转换过程,太阳能气化应用也面临着诸多挑战。本研究设计了一种新型的直接辐照太阳能气化反应器,改进了光接收结构和合理的测试模块,并选择小麦秸秆颗粒作为实验样品。采用 9 kWe 高通量太阳能模拟器,在平均太阳通量为 1171.3 kW/m2 的条件下,该反应器原型反应床的最高温度达到 1260 ℃。以可调节的辐射通量作为实验系数,在最高总辐射量为 3.35 kW 的情况下,产生的合成气中 H2 的摩尔分数为 47.1%,能量提升系数为 1.15,纤维素成分完成分解。提高蒸汽的质量流量可减少合成气的输出,同时提高合成气中的 H2/CO 比率。此外,较小的生物质颗粒尺寸有利于反应的进行,从而提高了直接辐照气化的转化效率。研究结果为高效利用丰富的太阳能和生物质能提供了有意义的参考。
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来源期刊
Chemical Engineering Journal
Chemical Engineering Journal 工程技术-工程:化工
CiteScore
21.70
自引率
9.30%
发文量
6781
审稿时长
2.4 months
期刊介绍: The Chemical Engineering Journal is an international research journal that invites contributions of original and novel fundamental research. It aims to provide an international platform for presenting original fundamental research, interpretative reviews, and discussions on new developments in chemical engineering. The journal welcomes papers that describe novel theory and its practical application, as well as those that demonstrate the transfer of techniques from other disciplines. It also welcomes reports on carefully conducted experimental work that is soundly interpreted. The main focus of the journal is on original and rigorous research results that have broad significance. The Catalysis section within the Chemical Engineering Journal focuses specifically on Experimental and Theoretical studies in the fields of heterogeneous catalysis, molecular catalysis, and biocatalysis. These studies have industrial impact on various sectors such as chemicals, energy, materials, foods, healthcare, and environmental protection.
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