Tunable Topological Transitions Probed by the Quantum Hall Effect in Twisted Double Bilayer Graphene

IF 9.1 1区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY Nano Letters Pub Date : 2024-12-20 DOI:10.1021/acs.nanolett.4c04242
Zehao Jia, Xiangyu Cao, Shihao Zhang, Jinshan Yang, Jingyi Yan, Yuda Zhang, Xin Lu, Pengliang Leng, Enze Zhang, Linfeng Ai, Xiaoyi Xie, Minsheng Li, Li Qian, Jianpeng Liu, Shaoming Dong, Faxian Xiu
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Abstract

The moiré system provides a tunable platform for investigating exotic quantum phases. Particularly, the displacement field D is crucial for tuning the electronic structures and topological properties of twisted double bilayer graphene (TDBG). Here, we present a series of D-tunable topological transitions by the evolution of quantum Hall phases (QHPs) in the valence bands of TDBG. As D increases, we observe the alternating emergence of two distinct quantum Hall regions originating from full-filling and half-filling, which we attribute to the D-induced Lifshitz transition. Moreover, we delve into the remote valence bands of TDBG and observe a transition in the sequence of Landau levels upon the application of D, shifting from 8N + 4 to 8N. This observation, combined with theoretical calculations, unveils an alteration in the Berry phase. Our findings highlight the TDBG as an exemplary platform for understanding the origin of the topological transitions in the graphene-based moiré systems.

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扭曲双双层石墨烯中量子霍尔效应探测的可调谐拓扑跃迁
该系统为研究奇异量子相提供了一个可调的平台。特别是,位移场D对于调整扭曲双双层石墨烯(TDBG)的电子结构和拓扑性质至关重要。在这里,我们通过TDBG价带中量子霍尔相(QHPs)的演化提出了一系列d可调谐的拓扑跃迁。随着D的增加,我们观察到两个不同的量子霍尔区域交替出现,它们起源于全填充和半填充,我们将其归因于D诱导的Lifshitz跃迁。此外,我们深入研究了TDBG的远价带,观察到D在朗道能级序列上发生了从8N + 4到8N的转变。这一观察与理论计算相结合,揭示了贝里相的变化。我们的发现强调了TDBG作为理解石墨烯基moirosystems中拓扑转变起源的范例平台。
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来源期刊
Nano Letters
Nano Letters 工程技术-材料科学:综合
CiteScore
16.80
自引率
2.80%
发文量
1182
审稿时长
1.4 months
期刊介绍: Nano Letters serves as a dynamic platform for promptly disseminating original results in fundamental, applied, and emerging research across all facets of nanoscience and nanotechnology. A pivotal criterion for inclusion within Nano Letters is the convergence of at least two different areas or disciplines, ensuring a rich interdisciplinary scope. The journal is dedicated to fostering exploration in diverse areas, including: - Experimental and theoretical findings on physical, chemical, and biological phenomena at the nanoscale - Synthesis, characterization, and processing of organic, inorganic, polymer, and hybrid nanomaterials through physical, chemical, and biological methodologies - Modeling and simulation of synthetic, assembly, and interaction processes - Realization of integrated nanostructures and nano-engineered devices exhibiting advanced performance - Applications of nanoscale materials in living and environmental systems Nano Letters is committed to advancing and showcasing groundbreaking research that intersects various domains, fostering innovation and collaboration in the ever-evolving field of nanoscience and nanotechnology.
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