Investigating the Current-Carrying Friction Mechanism of n-Type and p-Type Two-Dimensional TMD under a Positive Electric Field

IF 8.2 2区 材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY ACS Applied Materials & Interfaces Pub Date : 2025-01-04 DOI:10.1021/acsami.4c16577
Guowei Huang, Ruichao Wang, Wenchao Wu, Wangle Xue, Peng Wang, Hongli Li, Zhenbin Gong
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Abstract

Nanofriction plays an important role in the performance and lifetime of n-type or p-type TMD-based semiconductor nanodevices. However, the mechanism of nanofriction in n-type and p-type TMD semiconductors under an electric field is still blurry. In this paper, monolayers of n-MoSe2 and p-WSe2 materials were prepared by chemical vapor deposition (CVD), and their nanofriction behavior under positive electric field was investigated. Atomic force microscopy (AFM) was used to analyze the nanofriction by the positive voltage applied through the needle tip: both the friction and the friction coefficient of MoSe2 increased with the increase of the applied voltage, while the friction and the friction coefficient of WSe2 decreased with the increase of the applied voltage. As the applied voltage increases, the friction force and energy dissipation exhibit corresponding trends in relation to the surface potential. The accumulation and dissipation of carriers represent significant factors influencing friction change. The diverse types of carriers give rise to variations in the friction laws. Our experiments have revealed the differences and mechanisms of friction in TMD materials dominated by different carrier types at positive voltages. It provides guidance for the application and modulation of n- and p-type two-dimensional semiconductor materials in the field of friction.

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正电场作用下n型和p型二维TMD载流摩擦机理研究
纳米摩擦对n型或p型tmd基半导体纳米器件的性能和寿命起着重要的作用。然而,电场作用下n型和p型TMD半导体的纳米摩擦机理尚不清楚。采用化学气相沉积(CVD)法制备了n-MoSe2和p-WSe2单层材料,研究了其在正电场作用下的纳米摩擦行为。利用原子力显微镜(AFM)分析针尖正电压作用下的纳米摩擦:MoSe2的摩擦力和摩擦系数随外加电压的增加而增加,而WSe2的摩擦力和摩擦系数随外加电压的增加而减小。随着外加电压的增加,摩擦力和能量耗散随表面电位的增加呈现相应的变化趋势。载流子的积累和耗散是影响摩擦变化的重要因素。不同类型的载流子引起摩擦规律的变化。我们的实验揭示了不同载流子类型的TMD材料在正电压下的摩擦差异及其机理。为n型和p型二维半导体材料在摩擦领域的应用和调制提供了指导。
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来源期刊
ACS Applied Materials & Interfaces
ACS Applied Materials & Interfaces 工程技术-材料科学:综合
CiteScore
16.00
自引率
6.30%
发文量
4978
审稿时长
1.8 months
期刊介绍: ACS Applied Materials & Interfaces is a leading interdisciplinary journal that brings together chemists, engineers, physicists, and biologists to explore the development and utilization of newly-discovered materials and interfacial processes for specific applications. Our journal has experienced remarkable growth since its establishment in 2009, both in terms of the number of articles published and the impact of the research showcased. We are proud to foster a truly global community, with the majority of published articles originating from outside the United States, reflecting the rapid growth of applied research worldwide.
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