All-solid Conductive Elastomers Bridging Mechanical Performance and Sustainability for Durable and Multifunctional Electronics

IF 8.3 2区 材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY ACS Applied Materials & Interfaces Pub Date : 2025-01-25 DOI:10.1021/acsami.4c21865
Chunxiang Wei, Shaoyu Yu, Yuanyuan Wei, Wenjie Yang, SanE Zhu, Wei Yang, Junjun Huang, Hongdian Lu, Jixin Zhu
{"title":"All-solid Conductive Elastomers Bridging Mechanical Performance and Sustainability for Durable and Multifunctional Electronics","authors":"Chunxiang Wei, Shaoyu Yu, Yuanyuan Wei, Wenjie Yang, SanE Zhu, Wei Yang, Junjun Huang, Hongdian Lu, Jixin Zhu","doi":"10.1021/acsami.4c21865","DOIUrl":null,"url":null,"abstract":"The next generation of stretchable electronics seeks to integrate superior mechanical properties with sustainability and sensing stability. Ionically conductive and liquid-free elastomers have gained recognition as promising candidates, addressing the challenges of evaporation and leakage in gel-based conductors. In this study, a sustainable polymeric deep eutectic system is synergistically integrated with amino-terminated hyperbranched polyamide-modified fibers and aluminum ions, forming a conductive supramolecular network with significant improvements in mechanical performance. The elastomer exhibits remarkable tensile strength (6.69 MPa) and ultrahigh toughness (275.7 MJ/m<sup>3</sup>), capable of lifting loads 8300 times its own weight and demonstrated notch-insensitive properties. The elastomer also possessed degradable and stepwise recyclable properties, supporting its sustainability. Its excellent mechanical performance and conductivity enable stable signal output for multifunctional electronics. A wearable strain sensor is developed, demonstrating high sensitivity (gauge factor up to 4.52) and reliable repeatability under strain. Furthermore, a durable triboelectric nanogenerator is also fabricated, delivering stable signal output over one month and demonstrating strong potential for tactile sensing across various contact materials, making it highly promising for future human–machine interaction applications. This work offers feasible strategy for the design of solid elastomer-based durable electronics and highlights the potential for multifunctional applications.","PeriodicalId":5,"journal":{"name":"ACS Applied Materials & Interfaces","volume":"1 1","pages":""},"PeriodicalIF":8.3000,"publicationDate":"2025-01-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"ACS Applied Materials & Interfaces","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1021/acsami.4c21865","RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"MATERIALS SCIENCE, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0

Abstract

The next generation of stretchable electronics seeks to integrate superior mechanical properties with sustainability and sensing stability. Ionically conductive and liquid-free elastomers have gained recognition as promising candidates, addressing the challenges of evaporation and leakage in gel-based conductors. In this study, a sustainable polymeric deep eutectic system is synergistically integrated with amino-terminated hyperbranched polyamide-modified fibers and aluminum ions, forming a conductive supramolecular network with significant improvements in mechanical performance. The elastomer exhibits remarkable tensile strength (6.69 MPa) and ultrahigh toughness (275.7 MJ/m3), capable of lifting loads 8300 times its own weight and demonstrated notch-insensitive properties. The elastomer also possessed degradable and stepwise recyclable properties, supporting its sustainability. Its excellent mechanical performance and conductivity enable stable signal output for multifunctional electronics. A wearable strain sensor is developed, demonstrating high sensitivity (gauge factor up to 4.52) and reliable repeatability under strain. Furthermore, a durable triboelectric nanogenerator is also fabricated, delivering stable signal output over one month and demonstrating strong potential for tactile sensing across various contact materials, making it highly promising for future human–machine interaction applications. This work offers feasible strategy for the design of solid elastomer-based durable electronics and highlights the potential for multifunctional applications.

Abstract Image

查看原文
分享 分享
微信好友 朋友圈 QQ好友 复制链接
本刊更多论文
求助全文
约1分钟内获得全文 去求助
来源期刊
ACS Applied Materials & Interfaces
ACS Applied Materials & Interfaces 工程技术-材料科学:综合
CiteScore
16.00
自引率
6.30%
发文量
4978
审稿时长
1.8 months
期刊介绍: ACS Applied Materials & Interfaces is a leading interdisciplinary journal that brings together chemists, engineers, physicists, and biologists to explore the development and utilization of newly-discovered materials and interfacial processes for specific applications. Our journal has experienced remarkable growth since its establishment in 2009, both in terms of the number of articles published and the impact of the research showcased. We are proud to foster a truly global community, with the majority of published articles originating from outside the United States, reflecting the rapid growth of applied research worldwide.
期刊最新文献
High-Performance Mechano-Sensitive Piezoelectric Nanogenerator from Post-Treated Nylon-11,11 Textiles for Energy Harvesting and Human Motion Monitoring Frustrated Lewis Pair Meets Polyhedral Oligomeric Silsesquioxane: Water-Tolerant Hybrid Porous Networks for Robust, Efficient, and Recyclable CO2 Catalysis High-Purity Ethylene Production from Ethane/Ethylene Mixtures at Ambient Conditions by Ethane-Selective Fluorine-Doped Activated Carbon Adsorbents All-solid Conductive Elastomers Bridging Mechanical Performance and Sustainability for Durable and Multifunctional Electronics Surface Fluorination of Silicone Rubber with Enhanced Stain Resistance and Slip Properties
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
现在去查看 取消
×
提示
确定
0
微信
客服QQ
Book学术公众号 扫码关注我们
反馈
×
意见反馈
请填写您的意见或建议
请填写您的手机或邮箱
已复制链接
已复制链接
快去分享给好友吧!
我知道了
×
扫码分享
扫码分享
Book学术官方微信
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术
文献互助 智能选刊 最新文献 互助须知 联系我们:info@booksci.cn
Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。
Copyright © 2023 Book学术 All rights reserved.
ghs 京公网安备 11010802042870号 京ICP备2023020795号-1