Low-density polyamide 12 foams using Bayesian optimization and inverse design

IF 4.1 2区 化学 Q2 POLYMER SCIENCE Polymer Pub Date : 2025-02-03 DOI:10.1016/j.polymer.2025.128096
Karim Ali Shah , Rodrigo Q. Albuquerque , Christian Brütting , Marcel Dippold , Holger Ruckdäschel
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Abstract

This study introduces a novel, comprehensive approach to optimizing and designing batch foaming of low-density polyamide 12 (PA-12) using advanced machine learning (ML) techniques. Bayesian optimization was used to minimize the foam density, which decreased from approximately 900 to 150 kg/m3 in a single new experiment. A PA-12 foam density of 50 kg/m3, the lowest achieved, was recorded. In addition, an inverse design approach was used to check the robustness of the model by identifying the specific processing parameters required to achieve the desired foam density. Finally, PA-12 foams with similar densities but different processing parameters were obtained using ML. The study highlights the effectiveness of integrating these ML methodologies in the development of lightweight, high-performance polymer foams, which is much more sustainable than traditional methods for achieving low-density foams.

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来源期刊
Polymer
Polymer 化学-高分子科学
CiteScore
7.90
自引率
8.70%
发文量
959
审稿时长
32 days
期刊介绍: Polymer is an interdisciplinary journal dedicated to publishing innovative and significant advances in Polymer Physics, Chemistry and Technology. We welcome submissions on polymer hybrids, nanocomposites, characterisation and self-assembly. Polymer also publishes work on the technological application of polymers in energy and optoelectronics. The main scope is covered but not limited to the following core areas: Polymer Materials Nanocomposites and hybrid nanomaterials Polymer blends, films, fibres, networks and porous materials Physical Characterization Characterisation, modelling and simulation* of molecular and materials properties in bulk, solution, and thin films Polymer Engineering Advanced multiscale processing methods Polymer Synthesis, Modification and Self-assembly Including designer polymer architectures, mechanisms and kinetics, and supramolecular polymerization Technological Applications Polymers for energy generation and storage Polymer membranes for separation technology Polymers for opto- and microelectronics.
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