Karim Ali Shah , Rodrigo Q. Albuquerque , Christian Brütting , Marcel Dippold , Holger Ruckdäschel
{"title":"Low-density polyamide 12 foams using Bayesian optimization and inverse design","authors":"Karim Ali Shah , Rodrigo Q. Albuquerque , Christian Brütting , Marcel Dippold , Holger Ruckdäschel","doi":"10.1016/j.polymer.2025.128096","DOIUrl":null,"url":null,"abstract":"<div><div>This study introduces a novel, comprehensive approach to optimizing and designing batch foaming of low-density polyamide 12 (PA-12) using advanced machine learning (ML) techniques. Bayesian optimization was used to minimize the foam density, which decreased from approximately 900 to 150 kg/m<span><math><msup><mrow></mrow><mrow><mn>3</mn></mrow></msup></math></span> in a single new experiment. A PA-12 foam density of 50 kg/m<span><math><msup><mrow></mrow><mrow><mn>3</mn></mrow></msup></math></span>, the lowest achieved, was recorded. In addition, an inverse design approach was used to check the robustness of the model by identifying the specific processing parameters required to achieve the desired foam density. Finally, PA-12 foams with similar densities but different processing parameters were obtained using ML. The study highlights the effectiveness of integrating these ML methodologies in the development of lightweight, high-performance polymer foams, which is much more sustainable than traditional methods for achieving low-density foams.</div></div>","PeriodicalId":405,"journal":{"name":"Polymer","volume":"320 ","pages":"Article 128096"},"PeriodicalIF":4.1000,"publicationDate":"2025-02-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Polymer","FirstCategoryId":"92","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S0032386125000825","RegionNum":2,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"POLYMER SCIENCE","Score":null,"Total":0}
引用次数: 0
Abstract
This study introduces a novel, comprehensive approach to optimizing and designing batch foaming of low-density polyamide 12 (PA-12) using advanced machine learning (ML) techniques. Bayesian optimization was used to minimize the foam density, which decreased from approximately 900 to 150 kg/m in a single new experiment. A PA-12 foam density of 50 kg/m, the lowest achieved, was recorded. In addition, an inverse design approach was used to check the robustness of the model by identifying the specific processing parameters required to achieve the desired foam density. Finally, PA-12 foams with similar densities but different processing parameters were obtained using ML. The study highlights the effectiveness of integrating these ML methodologies in the development of lightweight, high-performance polymer foams, which is much more sustainable than traditional methods for achieving low-density foams.
期刊介绍:
Polymer is an interdisciplinary journal dedicated to publishing innovative and significant advances in Polymer Physics, Chemistry and Technology. We welcome submissions on polymer hybrids, nanocomposites, characterisation and self-assembly. Polymer also publishes work on the technological application of polymers in energy and optoelectronics.
The main scope is covered but not limited to the following core areas:
Polymer Materials
Nanocomposites and hybrid nanomaterials
Polymer blends, films, fibres, networks and porous materials
Physical Characterization
Characterisation, modelling and simulation* of molecular and materials properties in bulk, solution, and thin films
Polymer Engineering
Advanced multiscale processing methods
Polymer Synthesis, Modification and Self-assembly
Including designer polymer architectures, mechanisms and kinetics, and supramolecular polymerization
Technological Applications
Polymers for energy generation and storage
Polymer membranes for separation technology
Polymers for opto- and microelectronics.