Efficient, Polarization-Diverse State Generation with Tunable Black Phosphorus Cavity Heterostructures and Active Metasurfaces

IF 6.5 1区 物理与天体物理 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY ACS Photonics Pub Date : 2025-02-13 DOI:10.1021/acsphotonics.4c01933
Samuel K. W. Seah, Souvik Biswas, Claudio U. Hail, Min Seok Jang, Harry A. Atwater
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Abstract

The dynamic, on-demand generation of different polarization states of light has diverse applications in optical communications, imaging, sensing, and quantum information processing. Such active polarization control is typically achieved using active metasurfaces or spatial light modulators based on liquid crystal media that have limited switching speeds and conversion efficiency. Layered van der Waals low-dimensional materials provide new avenues for more versatile polarization control with an operating frequency several orders of magnitude higher than that for liquid crystal devices. Here, we report the design of a heterostructure for efficient, polarization-selective free-space phase modulation or amplitude modulation by integrating electrically tunable, optically anisotropic black phosphorus (BP) into high quality factor (Q ∼ 7500 to 11000) distributed Bragg reflector-based Fabry–Perot cavities. These devices achieve a respective phase tuning range of 210° and an amplitude tuning range of 99%. We also introduce designs for BP heterostructures that employ two twisted cross-aligned BP layers that are able to access polarization states covering 75% of the Poincaré sphere from voltage tuning alone. Finally, we introduce a design for an active metasurface polarization beam splitter based on our cavity heterostructures with an electrically tunable angle of diffraction that leverages spatially engineered polarization gradients. These structures open a pathway for further structuring of light by controlling the phase and amplitude along independent orthogonal directions.

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按需动态生成不同偏振态的光在光通信、成像、传感和量子信息处理方面有着多种应用。这种主动偏振控制通常使用基于液晶介质的有源元表面或空间光调制器来实现,但其开关速度和转换效率有限。层状范德华低维材料为实现更多功能的偏振控制提供了新途径,其工作频率比液晶器件高出几个数量级。在此,我们报告了一种异质结构的设计,通过将电可调、光学各向异性的黑磷(BP)集成到基于高品质因数(Q ∼ 7500 至 11000)分布式布拉格反射器的法布里-珀罗腔中,实现高效的偏振选择性自由空间相位调制或振幅调制。这些器件的相位调谐范围分别达到 210°,振幅调谐范围达到 99%。我们还介绍了采用两个扭曲交叉排列的 BP 层的 BP 异质结构设计,仅通过电压调谐就能获得覆盖 75% 波恩卡莱球面的偏振态。最后,我们在空腔异质结构的基础上介绍了一种有源元表面偏振分束器的设计,这种分束器具有电可调衍射角,可利用空间工程设计的偏振梯度。这些结构为沿着独立的正交方向控制相位和振幅,进一步构造光的结构开辟了道路。
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来源期刊
ACS Photonics
ACS Photonics NANOSCIENCE & NANOTECHNOLOGY-MATERIALS SCIENCE, MULTIDISCIPLINARY
CiteScore
11.90
自引率
5.70%
发文量
438
审稿时长
2.3 months
期刊介绍: Published as soon as accepted and summarized in monthly issues, ACS Photonics will publish Research Articles, Letters, Perspectives, and Reviews, to encompass the full scope of published research in this field.
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