Enhancing selectivity and sensitivity in gas sensors through noble metal-decorated ZnO and machine learning

IF 6.9 2区 材料科学 Q2 CHEMISTRY, PHYSICAL Applied Surface Science Pub Date : 2025-06-01 Epub Date: 2025-02-21 DOI:10.1016/j.apsusc.2025.162750
Yeong Min Kwon , Yeseul Son , Do Hyung Lee , Min Hyeok Lim , Jin Kyu Han , Moonjeong Jang , Seoungwoong Park , Saewon Kang , Soonmin Yim , Sung Myung , Jongsun Lim , Sun Sook Lee , Garam Bae , Soo-Hyun Kim , Wooseok Song
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Abstract

The growing need for highly sensitive and selective gas sensors has spurred extensive research on enhancing metal–oxide–semiconductor-based sensors. In this study, we explored the gas-sensing performance of ZnO thin films functionalized with noble metals (Ir, Ru, and IrRu alloys) via atomic layer deposition for the detection of hazardous gases. The incorporation of noble metals led to significant improvements in the gas-sensing behavior driven by both electronic and chemical sensitization mechanisms. To further enhance gas selectivity, machine learning-based data analysis was employed, enabling precise classification of various gases with 100 % accuracy. These findings underscore the potential of noble metal-functionalized ZnO sensors for advanced gas detection, illustrating the effective combination of material engineering and cutting-edge data analysis techniques for the development of intelligent, selective, and stable gas sensor platforms.

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利用贵金属修饰ZnO和机器学习提高气体传感器的选择性和灵敏度
对高灵敏度和高选择性气体传感器的需求日益增长,促进了对增强金属氧化物半导体传感器的广泛研究。在这项研究中,我们通过原子层沉积的方式探索了贵金属(Ir, Ru和IrRu合金)功能化ZnO薄膜的气敏性能,用于检测有害气体。贵金属的掺入导致了由电子和化学敏化机制驱动的气体敏化行为的显著改善。为了进一步提高气体选择性,采用了基于机器学习的数据分析,能够以100%的准确率对各种气体进行精确分类。这些发现强调了贵金属功能化ZnO传感器在先进气体检测中的潜力,说明了材料工程和前沿数据分析技术的有效结合,可以开发智能,选择性和稳定的气体传感器平台。
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来源期刊
Applied Surface Science
Applied Surface Science 工程技术-材料科学:膜
CiteScore
12.50
自引率
7.50%
发文量
3393
审稿时长
67 days
期刊介绍: Applied Surface Science covers topics contributing to a better understanding of surfaces, interfaces, nanostructures and their applications. The journal is concerned with scientific research on the atomic and molecular level of material properties determined with specific surface analytical techniques and/or computational methods, as well as the processing of such structures.
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