Yeong Min Kwon, Yeseul Son, Do Hyung Lee, Min Hyeok Lim, Jin Kyu Han, Moonjeong Jang, Seoungwoong Park, Saewon Kang, Soonmin Yim, Sung Myung, Jongsun Lim, Sun Sook Lee, Garam Bae, Soo-Hyun Kim, Wooseok Song
{"title":"Enhancing selectivity and sensitivity in gas sensors through noble metal-decorated ZnO and machine learning","authors":"Yeong Min Kwon, Yeseul Son, Do Hyung Lee, Min Hyeok Lim, Jin Kyu Han, Moonjeong Jang, Seoungwoong Park, Saewon Kang, Soonmin Yim, Sung Myung, Jongsun Lim, Sun Sook Lee, Garam Bae, Soo-Hyun Kim, Wooseok Song","doi":"10.1016/j.apsusc.2025.162750","DOIUrl":null,"url":null,"abstract":"The growing need for highly sensitive and selective gas sensors has spurred extensive research on enhancing metal–oxide–semiconductor-based sensors. In this study, we explored the gas-sensing performance of ZnO thin films functionalized with noble metals (Ir, Ru, and IrRu alloys) via atomic layer deposition for the detection of hazardous gases. The incorporation of noble metals led to significant improvements in the gas-sensing behavior driven by both electronic and chemical sensitization mechanisms. To further enhance gas selectivity, machine learning-based data analysis was employed, enabling precise classification of various gases with 100 % accuracy. These findings underscore the potential of noble metal-functionalized ZnO sensors for advanced gas detection, illustrating the effective combination of material engineering and cutting-edge data analysis techniques for the development of intelligent, selective, and stable gas sensor platforms.","PeriodicalId":247,"journal":{"name":"Applied Surface Science","volume":"47 1","pages":""},"PeriodicalIF":6.3000,"publicationDate":"2025-02-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Applied Surface Science","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1016/j.apsusc.2025.162750","RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
引用次数: 0
Abstract
The growing need for highly sensitive and selective gas sensors has spurred extensive research on enhancing metal–oxide–semiconductor-based sensors. In this study, we explored the gas-sensing performance of ZnO thin films functionalized with noble metals (Ir, Ru, and IrRu alloys) via atomic layer deposition for the detection of hazardous gases. The incorporation of noble metals led to significant improvements in the gas-sensing behavior driven by both electronic and chemical sensitization mechanisms. To further enhance gas selectivity, machine learning-based data analysis was employed, enabling precise classification of various gases with 100 % accuracy. These findings underscore the potential of noble metal-functionalized ZnO sensors for advanced gas detection, illustrating the effective combination of material engineering and cutting-edge data analysis techniques for the development of intelligent, selective, and stable gas sensor platforms.
期刊介绍:
Applied Surface Science covers topics contributing to a better understanding of surfaces, interfaces, nanostructures and their applications. The journal is concerned with scientific research on the atomic and molecular level of material properties determined with specific surface analytical techniques and/or computational methods, as well as the processing of such structures.