Field Dynamics in the Gap of a Semiconductor Nanodimer

Zi Wang, T. Wong
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Abstract

Semiconductor nanodimer provides substantial terahertz electric field intensification in the gap region as a result of geometric local field effect and surface plasmon resonance. In a dimer formed by two nanoparticles with unequal doping levels, the intrinsic resonances of the nanoparticles are carried over to the coupled configuration of the dimer, giving rise to two resonances, slightly shifted from those of the intrinsic particles. An important characteristic of the enhanced field in the gap is the intensity profile swaying when the frequency of the applied field is varied from one resonance to the other. In this work, the field distribution in an asymmetric semiconductor nanodimer is computed by numerical simulation of the charge-field interaction in the semiconductor, employing a transport formulation for charge dynamics. Charge distribution in the semiconductor, field intensity in the gap and the collective response in terms of the total dipole moment are obtained. Interpretation of the results is presented in light of polarization coupling and interference effects between the particles. Potential application of the dynamical response as a field scanning sensor in the terahertz range is explored.
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半导体纳米二聚体间隙中的场动力学
半导体纳米二聚体由于几何局部场效应和表面等离子体共振在间隙区提供了大量的太赫兹电场增强。在由两个不相等掺杂水平的纳米颗粒组成的二聚体中,纳米颗粒的本征共振被传递到二聚体的耦合构型中,产生两个共振,与本征粒子的共振略有不同。当外加场的频率从一个共振变化到另一个共振时,间隙中增强场的强度分布会发生摇摆,这是增强场的一个重要特征。在这项工作中,采用电荷动力学的输运公式,通过对半导体中电荷场相互作用的数值模拟,计算了非对称半导体纳米二聚体中的场分布。得到了半导体中的电荷分布、间隙中的场强以及用总偶极矩表示的集体响应。从偏振耦合和粒子间干涉效应的角度对结果进行了解释。探讨了动态响应在太赫兹范围内作为场扫描传感器的潜在应用。
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