高富集Ge同位素在16.4 ~ 18.9 MeV能量范围内(n,x)反应的截面测量

S. Chasapoglou, R. Vlastou, M. Kokkoris, M. Diakaki, V. Michalopoulou, A. Stamatopoulos, M. Axiotis, S. Harissopulos, A. Lagoyannis, M. Savva, I. Stamatelatos, T. Vasilopoulou, C. Lederer-Woods
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引用次数: 0

摘要

本文利用活化技术,在16.4 ~ 18.9 MeV能量范围内测量了中子诱导反应70Ge(n,2n)69Ge、76Ge(n,2n)75Ge、73Ge(n,p)73Ga、72Ge(n,p)72Ga、73Ge(n,d/np)72Ga、74Ge(n,d/np)73Ga、74Ge(n,α)71mZn、72Ge(n,α)69mZn、73Ge(n,nα)69mZn的截面,并与参考反应27Al(n,α)24Na进行了对比。在文献中发现的这些反应的大多数现有实验数据集都是使用natGe靶标获得的。然而,在这种情况下,一些反应通道产生的残余核也可能是由中子诱导的邻近同位素的反应产生的,这些同位素存在于自然丰度的natGe中,对感兴趣的反应的测量产率起污染作用。然后应该根据理论计算减去这种寄生贡献,理论计算本身具有不确定性。另一方面,同位素富集的目标不受这种污染,导致更准确的实验截面结果。在这项工作中,使用了五个高富集靶,有助于确定准确的截面数据,特别是在73Ge(n,d/np)72Ga, 74Ge(n,d/np)73Ga和73Ge(n,nα)69mZn挑战反应的情况下,这将在本文中详细介绍。实验在ncsrs“Demokritos”的5.5 MV串联Van de Graaff加速器上进行,实现了产生准单能中子束的3H(d,n)4He反应。
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Cross Section Measurements of (n,x) Reactions In the Energy Range Between 16.4 and 18.9 MeV Using Highly Enriched Ge Isotopes
In this work, the cross sections of the neutron induced reactions 70Ge(n,2n)69Ge, 76Ge(n,2n)75Ge, 73Ge(n,p)73Ga, 72Ge(n,p)72Ga, 73Ge(n,d/np)72Ga, 74Ge(n,d/np)73Ga, 74Ge(n,α)71mZn, 72Ge(n,α)69mZn, 73Ge(n,nα)69mZn have been measured in the energy range between 16.4 and 18.9 MeV via the activation technique with respect to the 27Al(n,α)24Na reference reaction. Most of the existing experimental datasets found in literature for these reactions, were obtained with the use of a natGe target. In this case however, the residual nucleus produced from some reaction channels, could also be produced from neutron induced reactions in neighboring isotopes that exist in the natGe in their natural abundance, acting as a contamination to the measured yield of the reaction of interest. This parasitic contribution should then be subtracted, based on theoretical calculations that bear their own uncertainties. Isotopically enriched targets on the other hand, do not suffer from such contaminations, leading to more accurate experimental cross section results. In this work, five highly enriched targets have been used that helped in the determination of accurate cross section data, especially in the case of the73Ge(n,d/np)72Ga, 74Ge(n,d/np)73Ga and 73Ge(n,nα)69mZn challenging reactions, that will be presented in detail in this manuscript. The experiments were carried out at the 5.5 MV Tandem Van de Graaff accelerator of N.C.S.R. “Demokritos”, implementing the 3H(d,n)4He reaction for the production of the quasi-monoenergetic neutron beams.
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