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Measuring radon concentrations in air at the progeny non-secular equilibrium time frame 在子代非长期平衡时间范围内测量空气中的氡浓度
Pub Date : 2023-05-05 DOI: 10.12681/hnpsanp.5131
N. Petropoulos, Sotia Argyrou
The Nuclear Engineering Laboratory of NTUA (NEL-NTUA) regularly tests radon-in-air concentration measuring instruments. Most common instruments involve open ionization chambers, radon absorbing devices and grab sampling devices. Most types of such instruments do not provide a calibrated radon concentration as soon as the air sampling has ended, since there should exist an adequate time gap, within which sampled radon would reach secular equilibrium with some or most of its immediate progeny. This gap should be around 10-20 min for radon to equilibrate with the Po-218 nucleus, or it could be more than about 3 hours for radon to equilibrate with the Bi-214 / Po-214 progeny. However, if there could be organized calibration experiments at the progeny non-secular equilibrium state, there are some instrument cases, for which this time gap difficulty may be better understood and overcome. To this end, in this work, the Bateman differential equations for all gamma and alpha emitting radon daughters are solved for radon daughters activity at any given time between 0 min and 3 hours using a spreadsheet. This would allow for obtaining a calibration correction factor to be applied at any given time before equilibrium, resulting for radon concentration estimations without the limitations of waiting. Following this solution, the results were theoretically assessed in terms of applicability. Calibration experiments performed for ionization chambers, radon absorbents and Lucas Cells at various radon concentrations in air at the progeny non-secular equilibrium time frame corroborate the theoretical approach.
核工程实验室定期对空气中氡浓度测量仪器进行检测。最常见的仪器包括开放电离室、氡吸收装置和抓取取样装置。大多数类型的这类仪器在空气取样结束后不会立即提供校准的氡浓度,因为应该存在一个适当的时间间隔,在这个时间间隔内,取样的氡将与它的一些或大部分直接子代达到长期平衡。氡与Po-218核的平衡时间应该在10-20分钟左右,或者氡与Bi-214 / Po-214子代的平衡时间可能超过3小时。然而,如果能够在后代非长期平衡状态下进行有组织的校准实验,在某些仪器情况下,可能会更好地理解和克服这一时间间隙困难。为此,在这项工作中,使用电子表格求解了所有γ和α发射氡子子在0分钟至3小时之间任何给定时间的氡子活性的贝特曼微分方程。这将允许在平衡之前的任何给定时间获得校准校正因子,从而在不受等待限制的情况下进行氡浓度估计。根据该解决方案,从理论上对结果的适用性进行了评估。在子代非长期平衡时间框架下,对空气中不同氡浓度的电离室、氡吸收剂和卢卡斯细胞进行了校准实验,证实了理论方法。
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引用次数: 0
First results from the 63Cu(α,γ)67Ga reaction study for nuclear astrophysics purposes 核子天体物理学研究63Cu(α,γ)67Ga反应的第一个结果
Pub Date : 2023-05-05 DOI: 10.12681/hnpsanp.5091
M. Peoviti, N. Patronis, M. Axiotis, V. Foteinou, D. Rogalla, Fotios Maragkos, S. Harissopulos
The 63Cu(α,γ)67Ga reaction cross-section was measured in the energy range between 5 and 9 MeV, which is relevant to p-process nucleosynthesis. The experiment was conducted at the Dynamitron Tandem Laboratory, of the Ruhr-University Bochum in Germany, by applying the 4π γ-summing method, using a 12"×12" NaI(Tl) single crystal scintillator. The preliminary results are compared with previous measurements and theoretical TALYS calculations as well.
63Cu(α,γ)67Ga反应截面在5 ~ 9 MeV能量范围内,与p-过程核合成有关。该实验是在德国波鸿鲁尔大学的Dynamitron串联实验室进行的,采用4π γ-求和方法,使用12“×12”NaI(Tl)单晶闪烁体。初步结果与以往的测量结果和理论计算结果进行了比较。
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引用次数: 0
A study of proton-induced reactions on natural Silicon targets 天然硅靶上质子诱导反应的研究
Pub Date : 2023-05-05 DOI: 10.12681/hnpsanp.5086
N. Nicolis, Georgia Zafeiri
Experimental excitation functions of isotopes produced in reactions p + natSi are compared with the results of nuclear reaction program TALYS 1.95 and semi-empirical cross section formulas. We consider excitation functions of 7 isotopes (28Mg, 26Al, 24,22Na, 18F and 10,7Be) produced in  reactions at bombarding energies of 20-144 MeV. They are compared with the predictions of the code TALYS 1.95, the semi-empirical formulas of Silberberg-Tsao (code yieldx) and SPACS. Comparisons of the results of the code TALYS 1.95 and previously published results of code ALICE are made. The predictive power of code TALYS 1.95 may be questioned for reaction products with mass number very much smaller than the target and of semi-empirical formulas at lower energies.
将p + natSi反应中同位素的实验激发函数与核反应程序TALYS 1.95和半经验截面公式的结果进行了比较。我们考虑了7种同位素(28Mg, 26Al, 24,22na, 18F和10,7be)在轰击能量为20- 144mev的反应中产生的激发函数。并与代码TALYS 1.95、Silberberg-Tsao(代码yieldx)的半经验公式和SPACS的预测结果进行了比较。将代码TALYS 1.95的结果与先前发布的代码ALICE的结果进行了比较。对于质量数远小于目标的反应产物和能量较低的半经验公式,代码TALYS 1.95的预测能力可能受到质疑。
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引用次数: 0
Microscopic analysis of octupole shape phase transitions and critical points in neutron rich actinides 富中子锕系元素八极形相变和临界点的显微分析
Pub Date : 2023-05-05 DOI: 10.12681/hnpsanp.5132
Vaia Prassa
Octupole constrained energy surfaces, and spectroscopic observables of four isotopic chains of: Cm, Cf, Fm and No with neutron numbers 186 N200 are analysed using a collective quadrupole - octupole Hamiltonian (QOCH). The parameters of the Hamiltonian are determined by axially reflection-asymmetric relativistic Hartree-Bogoliubov calculations based on the energy density functional DD-PC1, and a finite-range pairing interaction. The theoretical results suggest quantum phase transitions from non-octupole to octupole deformed shapes and to octupole vibrations with increasing neutron number. 288Cm is possibly close to the critical point of a simultaneous phase transition from spherical to prolate deformed and from non-octupole to stable octupole deformed configurations.
用四极-八极哈密顿量(QOCH)对中子数为186 N200的Cm、Cf、Fm和No四种同位素链的八极约束能面和光谱观测结果进行了分析。基于能量密度泛函DD-PC1和有限范围配对相互作用,通过轴向反射-非对称相对论Hartree-Bogoliubov计算确定了哈密顿量的参数。理论结果表明,随着中子数的增加,量子相位从非八极向八极变形转变,并向八极振动转变。288Cm可能接近同时发生从球形到长条形、从非八极到稳定八极形相变的临界点。
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引用次数: 0
Semiconductor Detector Study for Detecting Fusion Neutrons using Geant4 Simulations 利用Geant4模拟研究用于探测聚变中子的半导体探测器
Pub Date : 2023-05-05 DOI: 10.12681/hnpsanp.5184
K. Kaperoni, M. Diakaki, M. Kokkoris, M. Axiotis, A. Ziagkova, C. Weiss, R. Vlastou
Accurate neutron flux measurements in fusion reactors are essential, in order to determine the feasibility and progress of the reaction as well as for safety issues. Semiconductor neutron detectors exhibit promising characteristics for operation in the extreme environmental conditions of fusion reactors. Silicon, Diamond and Silicon Carbide are the most studied and anticipated materials for constructing detectors with high efficiency and irradiation resistance. The ITER fusion reactor is expected to run D-D plasma measurements in the near future, so the detection of 2.45 MeV neutrons with appropriate detectors is of great and immediate importance. In the present work the study of 2.45 MeV neutrons interactions with a silicon, diamond and silicon carbide detector was made, using GEANT4 [1] simulations, in order to compare their response. An experimental study will follow at the neutron production facility of the TANDEM accelerator of the I.N.P.P. of the NCSR “Demokritos”, with detectors provided by CIVIDEC Instrumentation GmbH, so the geometry of the simulations was built accordingly. A quasi-monoenergetic neutron beam of 2.45 MeV was produced through 3H(p,n) reactions in a TiT target. Due to the low cross section of the reaction, biasing techniques were implemented in the simulation to increase the counting rate and thus producing realistic results. These biasing techniques were studied, with various tests and the parameters affecting the choice of the biasing factor are shown and discussed.
为了确定聚变反应堆的可行性和进展以及安全问题,精确的中子通量测量是必不可少的。半导体中子探测器在聚变反应堆的极端环境条件下表现出良好的运行特性。硅、金刚石和碳化硅是构建高效耐辐照探测器的重要材料。ITER聚变反应堆有望在不久的将来进行D-D等离子体测量,因此用合适的探测器探测2.45 MeV中子具有重要而紧迫的意义。在本工作中,研究了2.45 MeV中子与硅、金刚石和碳化硅探测器的相互作用,使用GEANT4[1]模拟,以比较它们的响应。随后将在NCSR“Demokritos”的I.N.P.P.的TANDEM加速器的中子生产设施进行实验研究,探测器由CIVIDEC仪器有限公司提供,因此相应地建立了模拟的几何形状。在TiT靶中通过3H(p,n)反应产生了2.45 MeV的准单能中子束。由于反应截面小,在模拟中采用偏置技术来提高计数率,从而产生逼真的结果。对这些偏置技术进行了研究,进行了各种试验,并对影响偏置系数选择的参数进行了说明和讨论。
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引用次数: 0
Radioactivity measurements in eastern Lesvos, Greece 希腊莱斯沃斯岛东部的放射性测量
Pub Date : 2023-05-05 DOI: 10.12681/hnpsanp.5136
F. Pappa
The radioactive background of the eastern side of Lesvos Island in Greece, an island rich in natural radioactivity, was studied by means of gamma ray spectroscopy. Dose rates and concentrations of natural radionuclides (232Th series, 226Ra and 40K) and 137Cs were measured in-situ and in the laboratory, respectively. A total of twenty soil samples and ten beach sand samples was collected and processed according to the IAEA protocol. For the in-situ measurement and the dose rate determination a portable NaI scintillation detector was utilized. The activity concentration calculations were held in the laboratory, using a high-purity germanium detector. These activity concentrations were also used to estimate dose rates, so as to compare the obtained results with the in-situ measurements. The maximum detected values of activity concentrations of 232Th series, 226Ra, 40K and 137Cs were found to be 190, 90, 960 and 70 Bq kg-1, respectively. As for the dose rates, both measured and estimated, the maximum values were 230 and 190 nGy h-1, respectively. A significant difference regarding activity concentrations and dose rates was observed between the two matrices (soil, beach sand), with the values of soil samples quite surpassing those of beach sand samples. That can be attributed to the granulometry of each matrix. Furthermore, the study attempts to compare the radioactive background between the eastern and the western side of Lesvos Island, with the larger values being found in the eastern part.
利用伽玛射线能谱法研究了天然放射性丰富的希腊莱斯沃斯岛东侧的放射性背景。在现场和实验室分别测量了天然放射性核素(232Th系列、226Ra和40K)和137Cs的剂量率和浓度。根据原子能机构议定书,共收集和处理了20个土壤样品和10个海滩砂样品。采用便携式NaI闪烁检测器进行原位测量和剂量率测定。活度浓度计算在实验室进行,使用高纯度锗检测器。这些活性浓度也用于估计剂量率,以便将所得结果与原位测量结果进行比较。232Th系列、226Ra、40K和137Cs活性浓度的最大检出值分别为190、90、960和70 Bq kg-1。在剂量率方面,测量值和估计值的最大值分别为230和190 nGy h-1。两种基质(土壤、沙滩沙)在活性浓度和剂量率方面存在显著差异,其中土壤样品的活性浓度和剂量率远远超过沙滩沙样品。这可以归因于每个基质的粒度。此外,本研究试图比较莱斯沃斯岛东部和西部的放射性本底值,发现东部的值较大。
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引用次数: 1
Measurement of differential cross sections for proton elastic scattering on natO at Ep= 4-6 MeV, suitable for EBS 质子弹性散射在Ep= 4-6 MeV的北约上的微分截面测量,适用于EBS
Pub Date : 2023-05-05 DOI: 10.12681/hnpsanp.5183
M. Kokkoris, Kostas Bosbotinis, V. Foteinou, A. Lagoyannis, F. Maragkos, N. Patronis, E. Taimpiri, A. Ziagkova
In this study we present the experimental differential cross sections of natO(p,p0) elastic scattering, determined via the relative measurement technique, in the proton beam energy range Elab=4-6 MeV with a varying step (from 5-15 keV), at six backscattering detector angles between 120o and 170o (every 10o). A thin, self-supporting target manufactured in the lab was used in this experiment and the determination of its stoichiometry was carried out according to the currently existing evaluation, which has also been benchmarked recently. The measurements were performed using the Van de Graaff Tandem 5.5 MV Accelerator of N.C.S.R. “Demokritos” in Athens, Greece. The differential cross-section datasets obtained in the present work and already existing ones in literature for this extended proton beam energy range are shown and the observed peculiarities and discrepancies are discussed and analyzed.
在本研究中,我们展示了通过相对测量技术在质子束能量范围Elab=4-6 MeV的不同步长(从5-15 keV)下,在6个背向散射探测器角度在120°到170°之间(每100°)时,北约(p,p0)弹性散射的实验微分截面。本实验使用实验室制造的一种薄的、自支撑的靶材,根据目前已有的评价进行化学计量测定,最近也进行了基准测试。测量是在希腊雅典的“Demokritos”nc.s.r. Van de Graaff串联5.5 MV加速器上进行的。给出了本工作中得到的和文献中已有的质子束能量范围的微分截面数据集,并讨论和分析了观察到的特点和差异。
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引用次数: 0
Activation Cross Section Measurement of the (n,2n) Reaction on 203Tl at 16.4 MeV, 18.9 MeV and Theoretical Calculations via the EMPIRE code 203Tl在16.4 MeV, 18.9 MeV下(n,2n)反应的活化截面测量及EMPIRE码理论计算
Pub Date : 2023-05-05 DOI: 10.12681/hnpsanp.5154
Stavros Patas, Sotiris Chasapoglou, Michalis Axiotis, Maria Diakaki, George Gkatis, Sotirios Harissopulos, Michael Kokkoris, Anastasios Lagoyannis, Eleni Tsivouraki, Roza Vlastou
The aim of the present work was to study the cross-section of the (n,2n) and (n,3n) reactions on 203Tl, by irradiating a natural TlCl pellet target with monoenergetic neutron beams at 16.4, and 18.9 MeV. The cross section measurements were carried out using the activation method, with respect to the 197Au(n,2n)196Au and 27Al(n,α)24Na reference reactions. The monoenergetic neutron beams were generated in the 5.5 MV Tandem accelerator of NCSR “Demokritos”, using the 3H(d,n)4He reaction. Monte Carlo simulations have been performed to take into account the gamma-ray self-absorption results as well as the estimation of the neutron flux through the reference foils. Theoretical calculations with the code EMPIRE have also been performed, using the same parameterization implemented in the theoretical study of Ir and Au nuclei in an attempt to find a suitable model for the description of all the experimental results in this mass region.
本研究的目的是用16.4和18.9 MeV的单能中子束辐照天然TlCl球靶,研究203Tl上(n,2n)和(n,3n)反应的截面。采用活化法对197Au(n,2n)196Au和27Al(n,α)24Na参比反应进行了截面测量。在NCSR“Demokritos”5.5 MV串联加速器中,利用3H(d,n)4He反应产生单能中子束。为了考虑伽玛射线的自吸收结果以及通过参考箔估计中子通量,进行了蒙特卡罗模拟。用EMPIRE代码进行了理论计算,使用在Ir和Au核的理论研究中实现的相同的参数化,试图找到一个合适的模型来描述这个质量区域的所有实验结果。
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引用次数: 0
Chernobyl and Fukushima nuclear accidents: similarities and differences 切尔诺贝利和福岛核事故:异同
Pub Date : 2023-05-05 DOI: 10.12681/hnpsanp.5094
John Kalef Ezra
During the almost seven decades of use of nuclear fission for electric energy production two major nuclear accidents took place, i.e., the 1986 Chernobyl accident and the 2011 Fukushima one. They were caused by reactor power-surge and loss-of-coolant, respectively. Both accidents occurred during hot power reactor shutdown and had identical root causes, i.e., poor safety culture and safety management in nuclear industry and state authorities. A brief comparison of the facility and the accident characteristics, disaster response methods, as well as of their health, social, economic, and political adverse effects is attempted. The radiological impact of the Chernobyl accident was much higher than that of the Fukushima one; however, a similar statement may not hold for the other types of impact.
在利用核裂变发电的近70年期间,发生了两次重大核事故,即1986年的切尔诺贝利事故和2011年的福岛事故。它们分别是由反应堆功率激增和冷却剂损失引起的。这两起事故都发生在热电堆停堆期间,其根本原因是相同的,即核工业和国家主管部门的安全文化和安全管理不善。本文试图对设施和事故特点、灾害应对方法及其对健康、社会、经济和政治的不利影响进行简要比较。切尔诺贝利核事故的辐射影响远高于福岛核事故;然而,类似的说法可能不适用于其他类型的影响。
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引用次数: 0
Recent Progress in the Study of the Reaction 70Zn (15 MeV/nucleon) + 64Ni with the MAGNEX Spectrometer 70Zn (15mev /核子)+ 64Ni反应的磁谱仪研究进展
Pub Date : 2023-05-05 DOI: 10.12681/hnpsanp.5090
S. Koulouris, G. Souliotis, F. Cappuzzello, D. Carbone, A. Pakou, C. Agodi, G. Brischetto, M. Cavallaro, S. Calabrese, I. Ciraldo, O. Fasoula, J. Klimo, Konstantina Palli, O. Sgouros, V. Soukeras, A. Spatafora, D. Torresi, M. Veselský
The present paper is focused on our recent efforts to study the production and identification of neutron-rich medium-mass rare isotopes from peripheral reactions at beam energies around and below the Fermi energy. We obtained high-quality experimental data from a recent experiment with the MAGNEX spectrometer at the INFN-LNS in Catania, Italy. The main aim of this experiment was to check the feasibility of ejectile identification in this energy regime with the use of a large acceptance magnetic spectrometer. Our developed technique for particle identification depends mainly on a reconstruction of both the atomic number Z and the ionic charge q of the ions, followed by the identification of the mass. Our method was successfully applied to identify neutron-rich ejectiles from multinucleon transfer from the reaction of 70Zn (15 MeV/nucleon) + 64Ni. Preliminary results indicate that the extracted experimental distributions, along with comparisons with the theoretical models could help us to shed light to the complex reaction mechanism of multinucleon transfer in this energy regime.
本文重点介绍了我们最近在费米能量附近和以下束流能量的外围反应中产生和鉴定富中子中等质量稀有同位素的工作。我们最近在意大利卡塔尼亚的INFN-LNS用磁谱仪进行了一次实验,获得了高质量的实验数据。本实验的主要目的是利用大接受度磁谱仪检验在该能量区进行弹射识别的可行性。我们开发的粒子识别技术主要依赖于离子的原子序数Z和离子电荷q的重建,然后是质量的识别。我们的方法成功地用于鉴定70Zn (15mev /核子)+ 64Ni反应中多核子转移产生的富中子抛射体。初步结果表明,所提取的实验分布,以及与理论模型的比较,有助于揭示该能量域中多核子转移的复杂反应机理。
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引用次数: 0
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HNPS Advances in Nuclear Physics
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