核设施退役和拆除过程中水中放射性浓度的拟议检测限值

Raquel Idoeta, Susana Petisco-Ferrero, Saroa Rozas, Concepción Olondo, Margarita Herranz
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摘要

核设施的拆除和退役(D&D)给参与环境辐射监测计划的放射性测量实验室带来了多项挑战。其中之一就是确定不同样品中放射性核素分析所要达到的检测限。在设定检测限时,应确保每种放射性核素的浓度值都能很容易地与特定的最大放射性活度浓度水平区分开来。这些最大放射性活度浓度水平通常是根据每种放射性核素各自的剂量贡献而设定的。一些国家立法规定了饮用水的检测限值。但是,目前还没有关于地下水或地表水检测限值的法规。因此,不同的机构或公司在评估与 D&D 活动相关的这些类型的水体中的放射性浓度时所要求的检测限值大相径庭。在这项工作中,我们的重点是雨水、地表水和地下水中 D&D 活动所需的检测限。我们建议采用世界卫生组织(WHO)的最大放射性活度浓度方法来确定检测限值,并与放射性废物管理机构和监管机构所要求的检测限值进行比较。我们还分析了一些实际案例,在这些案例中,我们的建议可以识别事件并得出结论。
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Proposed Detection Limits for Radioactivity Concentrations in Water in the Decommissioning and Dismantling of Nuclear Facilities
The Dismantling and Decommissioning (D&D) of nuclear facilities poses several challenges for radioactivity measurement laboratories involved in environmental radiation monitoring plans. One of them is the definition of the detection limits to be achieved for the radionuclides analysis in different samples. The detection limits should be set in such a way that the obtained concentration values for each radionuclide are easily discriminated from certain maximum activity concentration levels. These maximum activity concentration levels are usually set in view of the respective dose contributions from each radionuclide. There are some national legislations that settle detection limits for drinking water. However, there is no regulation containing detection limits for groundwater or surface water. In this way, different institutions or companies require very different detection limits for radioactivity concentration assessment in those types of water associated with D&D activities. In this work, we focus on the detection limits required for the D&D activities in rainwater, surface water and groundwater. We propose detection limits obtained by applying the WHO methodology for maximum activity concentration levels and compare with those requested by radioactive waste management agencies and regulatory bodies. Some real cases where our proposal allows identification of events are analysed and conclusions are extracted.
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