相关电子附近的狄拉克带反常现象

IF 5.1 3区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY Nanoscale Pub Date : 2024-07-02 DOI:10.1039/D4NR01535E
Sawani Datta, Khadiza Ali, Rahul Verma, Bahadur Singh, Saroj P. Dash, A. Thamizhavel and Kalobaran Maiti
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摘要

狄拉克费米子是一种静止质量为零的粒子,在拓扑材料中可以观察到它的存在,并被认为在基础科学的奇异性和量子技术的进步中发挥着关键作用。迄今研究的大多数拓扑系统都是弱相关系统,而它们在电子相关情况下的性质是一个有趣的新兴研究领域,电子相关有望增强粒子的有效质量。在此,我们利用高分辨率角度分辨光发射光谱和第一原理计算,研究了非非晶层状近藤晶格体系 CeAgSb$_2$ 中的狄拉克带性质。除了由于非对称性而产生的狄拉克锥之外,这种材料在邻近表现出 Kondo 行为的强相关 Ce 层的方网层中还存在狄拉克费米子。实验结果表明,由于非对称性,在布里渊区边界存在高色散线性带交叉。此外,还存在各向异性的狄拉克锥,由形成菱形结线的正方形 Sb 5$p$ 态构成。这些狄拉克带在很宽的能量范围内呈线性,斜率异常高。有趣的是,在局部 Ce 4$f$ 带附近,这些带的斜率发生了变化,类似于在其他材料中观察到的由于电子-声子耦合而形成的 "扭结"。在强相关电子态附近出现这种奇异特性,对研究包括非常规超导体在内的复杂量子材料具有重要意义。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

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Anomalies in the Dirac bands in the proximity of correlated electrons

Dirac fermions, particles with zero rest mass, are observed in topological materials and are believed to play a key role in the exotic phenomena in fundamental science and the advancement of quantum technology. Most of the topological systems studied so far are weakly correlated systems and the study of their properties in the presence of electron correlation is an interesting emerging area of research, where the electron correlation is expected to enhance the effective mass of the particles. Here, we studied the properties of Dirac bands in a non-symmorphic layered Kondo lattice system, CeAgSb2, employing high-resolution angle-resolved photoemission spectroscopy and first-principles calculations. In addition to the Dirac cones due to non-symmorphic symmetry, this material hosts Dirac fermions in the squarenet layer in the proximity of a strongly correlated Ce layer exhibiting Kondo behavior. Experimental results reveal crossings of the highly dispersive linear bands at the Brillouin zone boundary due to non-symmorphic symmetry. In addition, there are anisotropic Dirac cones constituted by the squarenet Sb 5p states forming a diamond-shaped nodal line. These Dirac bands are linear in a wide energy range with an unusually high slope. Interestingly, near the local Ce 4f bands, these bands exhibit a change in the slope akin to the formation of a ‘kink’ observed in other materials due to electron–phonon coupling. The emergence of such exotic properties in proximity to strongly correlated electronic states has significant implications in the study of complex quantum materials including unconventional superconductors.

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来源期刊
Nanoscale
Nanoscale CHEMISTRY, MULTIDISCIPLINARY-NANOSCIENCE & NANOTECHNOLOGY
CiteScore
12.10
自引率
3.00%
发文量
1628
审稿时长
1.6 months
期刊介绍: Nanoscale is a high-impact international journal, publishing high-quality research across nanoscience and nanotechnology. Nanoscale publishes a full mix of research articles on experimental and theoretical work, including reviews, communications, and full papers.Highly interdisciplinary, this journal appeals to scientists, researchers and professionals interested in nanoscience and nanotechnology, quantum materials and quantum technology, including the areas of physics, chemistry, biology, medicine, materials, energy/environment, information technology, detection science, healthcare and drug discovery, and electronics.
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