{"title":"在贫氢预混合小火焰中通过强化应变缓解优先扩散效应","authors":"Alessandro Porcarelli, Ivan Langella","doi":"10.1016/j.proci.2024.105728","DOIUrl":null,"url":null,"abstract":"The interplay between strain and preferential diffusion in lean premixed hydrogen flamelets is investigated numerically. Lean conditions are established at an equivalence ratio of 0.5. Detailed chemistry, one-dimensional simulations are performed on a reactants-to-products counterflow configuration, both including and artificially excluding preferential diffusion effects. A comprehensive analysis of the flame physical properties is performed, showing that preferential diffusion tends to weaken the flame as compared to the case where it is artificially suppressed, as it triggers a local leaning of the mixture ahead of the flame front. Counterintuitively, strain is observed to counteract or limit this preferential diffusion effect, with the peaks of radicals and reaction rate, flame thickness, and consumption speed, progressively approaching and in some cases overtaking the corresponding solution obtained with equal diffusivities as strain increases. This is shown to be a consequence of the fluid elements being increasingly preferentially transported in the flame tangential direction rather than diffusing in the flame normal direction. Hence, the flame weakening effect due to different diffusive fluxes of fuel and oxidizer across the flame front is progressively compensated by their differential transport on the flame tangential direction triggered by increasing applied strain rate, which instead enables an overall enrichment of the burning mixture. This analysis provides a different view as compared to previous studies attributing to strain an enhancing influence on the effects of preferential diffusion. In this work the opposite interpretation is proposed instead, where strain acts as a limiting factor to the weakening effect of preferential diffusion on lean hydrogen flames.","PeriodicalId":408,"journal":{"name":"Proceedings of the Combustion Institute","volume":"59 1","pages":""},"PeriodicalIF":5.3000,"publicationDate":"2024-08-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Mitigation of preferential diffusion effects by intensive strain in lean premixed hydrogen flamelets\",\"authors\":\"Alessandro Porcarelli, Ivan Langella\",\"doi\":\"10.1016/j.proci.2024.105728\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"The interplay between strain and preferential diffusion in lean premixed hydrogen flamelets is investigated numerically. Lean conditions are established at an equivalence ratio of 0.5. Detailed chemistry, one-dimensional simulations are performed on a reactants-to-products counterflow configuration, both including and artificially excluding preferential diffusion effects. A comprehensive analysis of the flame physical properties is performed, showing that preferential diffusion tends to weaken the flame as compared to the case where it is artificially suppressed, as it triggers a local leaning of the mixture ahead of the flame front. Counterintuitively, strain is observed to counteract or limit this preferential diffusion effect, with the peaks of radicals and reaction rate, flame thickness, and consumption speed, progressively approaching and in some cases overtaking the corresponding solution obtained with equal diffusivities as strain increases. This is shown to be a consequence of the fluid elements being increasingly preferentially transported in the flame tangential direction rather than diffusing in the flame normal direction. Hence, the flame weakening effect due to different diffusive fluxes of fuel and oxidizer across the flame front is progressively compensated by their differential transport on the flame tangential direction triggered by increasing applied strain rate, which instead enables an overall enrichment of the burning mixture. This analysis provides a different view as compared to previous studies attributing to strain an enhancing influence on the effects of preferential diffusion. In this work the opposite interpretation is proposed instead, where strain acts as a limiting factor to the weakening effect of preferential diffusion on lean hydrogen flames.\",\"PeriodicalId\":408,\"journal\":{\"name\":\"Proceedings of the Combustion Institute\",\"volume\":\"59 1\",\"pages\":\"\"},\"PeriodicalIF\":5.3000,\"publicationDate\":\"2024-08-22\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Proceedings of the Combustion Institute\",\"FirstCategoryId\":\"5\",\"ListUrlMain\":\"https://doi.org/10.1016/j.proci.2024.105728\",\"RegionNum\":2,\"RegionCategory\":\"工程技术\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"ENERGY & FUELS\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Proceedings of the Combustion Institute","FirstCategoryId":"5","ListUrlMain":"https://doi.org/10.1016/j.proci.2024.105728","RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"ENERGY & FUELS","Score":null,"Total":0}
Mitigation of preferential diffusion effects by intensive strain in lean premixed hydrogen flamelets
The interplay between strain and preferential diffusion in lean premixed hydrogen flamelets is investigated numerically. Lean conditions are established at an equivalence ratio of 0.5. Detailed chemistry, one-dimensional simulations are performed on a reactants-to-products counterflow configuration, both including and artificially excluding preferential diffusion effects. A comprehensive analysis of the flame physical properties is performed, showing that preferential diffusion tends to weaken the flame as compared to the case where it is artificially suppressed, as it triggers a local leaning of the mixture ahead of the flame front. Counterintuitively, strain is observed to counteract or limit this preferential diffusion effect, with the peaks of radicals and reaction rate, flame thickness, and consumption speed, progressively approaching and in some cases overtaking the corresponding solution obtained with equal diffusivities as strain increases. This is shown to be a consequence of the fluid elements being increasingly preferentially transported in the flame tangential direction rather than diffusing in the flame normal direction. Hence, the flame weakening effect due to different diffusive fluxes of fuel and oxidizer across the flame front is progressively compensated by their differential transport on the flame tangential direction triggered by increasing applied strain rate, which instead enables an overall enrichment of the burning mixture. This analysis provides a different view as compared to previous studies attributing to strain an enhancing influence on the effects of preferential diffusion. In this work the opposite interpretation is proposed instead, where strain acts as a limiting factor to the weakening effect of preferential diffusion on lean hydrogen flames.
期刊介绍:
The Proceedings of the Combustion Institute contains forefront contributions in fundamentals and applications of combustion science. For more than 50 years, the Combustion Institute has served as the peak international society for dissemination of scientific and technical research in the combustion field. In addition to author submissions, the Proceedings of the Combustion Institute includes the Institute''s prestigious invited strategic and topical reviews that represent indispensable resources for emergent research in the field. All papers are subjected to rigorous peer review.
Research papers and invited topical reviews; Reaction Kinetics; Soot, PAH, and other large molecules; Diagnostics; Laminar Flames; Turbulent Flames; Heterogeneous Combustion; Spray and Droplet Combustion; Detonations, Explosions & Supersonic Combustion; Fire Research; Stationary Combustion Systems; IC Engine and Gas Turbine Combustion; New Technology Concepts
The electronic version of Proceedings of the Combustion Institute contains supplemental material such as reaction mechanisms, illustrating movies, and other data.