利用 APCS-MLR 模型对滕州市农用车道上不同人群和不同来源的重金属进行健康风险评估。

IF 3.2 3区 环境科学与生态学 Q3 ENGINEERING, ENVIRONMENTAL Environmental Geochemistry and Health Pub Date : 2024-09-24 DOI:10.1007/s10653-024-02227-5
Beibei Yan, Xinfeng Li, Jian Yang, Min Wang, Ruilin Zhang, Xiaoyu Song
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引用次数: 0

摘要

确定当地土壤中重金属的来源及其对人体健康的危害。本研究对在中国滕州采集的 504 份土壤样本中的八种重金属浓度进行了量化。采用单一重金属生态风险指数(EI)、综合生态风险指数(RI)和健康风险评估模型来评估该市的污染程度。研究结果表明,滕州市城乡农业区的重金属污染程度不同。此外,汞(Hg)的空间变异性很大,达到 0.96,表明人为活动的影响很大。在生态风险方面,EI 值最高的重金属元素是汞,平均值为 67.22,峰值为 776.00。平均 EI 值最低的重金属元素是锌,仅为 1.03。同时,平均 RI 值仅为 128.59,但有些地区的 RI 值高达 842.2。利用主成分分析、相关性分析和绝对主成分得分多元线性回归模型(APCS-MLR)确定了重金属的来源。儿童的非致癌风险、儿童的致癌风险和成人的致癌风险分别为 1.23、2.42×10-4 和 1.00×10-4,这些值都超过了各自的建议值,As 和 Cr 有一定的致癌危害。土壤中的重金属来源于自然、工业、交通和农业,分别占 39.59%、29.48%、25.17% 和 5.77%。当地农业土壤中重金属的主要来源是地质背景,政府需要加强对饮用水资源中 As 和 Cr 的监测,并减少交通污染和工厂废物排放,以降低土壤中的汞含量。
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Assessment of health risks based on different populations and sources of heavy metals on agricultural lane in Tengzhou City by APCS-MLR models.

To identify the sources of heavy metals in local soils and their risks to human health. This study quantified the concentrations of eight heavy metals in 504 soil samples collected in Tengzhou, China. The ecological risks of a single heavy metal (EI), a comprehensive ecological risk index (RI), and a health risk assessment model were used to evaluate the level of contamination in the city. The results of the research study indicate that there are different levels of heavy metal pollution in rural and urban agricultural areas in Tengzhou. Moreover, the spatial variability of mercury (Hg) is considerable, reaching 0.96, indicating a significant impact of anthropogenic activities. For the ecological risk, the heavy metal element with the highest EI value was mercury with a mean value of 67.22 and a peak value of 776.00. The heavy metal with the lowest mean EI value was Zn with only 1.03. Meanwhile, the average RI is only 128.59, but some areas have an RI as high as 842.2. The sources of heavy metals were identified using principal component analysis, correlation analysis, and an absolute principal component score multiple linear regression model (APCS-MLR). The non-carcinogenic risk for children, the carcinogenic risk for children, and the carcinogenic risk for adults were 1.23, 2.42×10-4 and 1.00×10-4, respectively, and these values exceeded their respective recommended values, and As and Cr had some carcinogenic hazards. Heavy metals in the soil come from natural, industrial, traffic and agricultural sources and represent 39.59%, 29.48%, 25.17% and 5.77%, respectively. The main source of heavy metals in local agricultural soils is the geological background, and the government needs to strengthen the monitoring of As and Cr in drinking water resources, as well as reduce traffic pollution and factory waste emissions to reduce Hg in soils.

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来源期刊
Environmental Geochemistry and Health
Environmental Geochemistry and Health 环境科学-工程:环境
CiteScore
8.00
自引率
4.80%
发文量
279
审稿时长
4.2 months
期刊介绍: Environmental Geochemistry and Health publishes original research papers and review papers across the broad field of environmental geochemistry. Environmental geochemistry and health establishes and explains links between the natural or disturbed chemical composition of the earth’s surface and the health of plants, animals and people. Beneficial elements regulate or promote enzymatic and hormonal activity whereas other elements may be toxic. Bedrock geochemistry controls the composition of soil and hence that of water and vegetation. Environmental issues, such as pollution, arising from the extraction and use of mineral resources, are discussed. The effects of contaminants introduced into the earth’s geochemical systems are examined. Geochemical surveys of soil, water and plants show how major and trace elements are distributed geographically. Associated epidemiological studies reveal the possibility of causal links between the natural or disturbed geochemical environment and disease. Experimental research illuminates the nature or consequences of natural or disturbed geochemical processes. The journal particularly welcomes novel research linking environmental geochemistry and health issues on such topics as: heavy metals (including mercury), persistent organic pollutants (POPs), and mixed chemicals emitted through human activities, such as uncontrolled recycling of electronic-waste; waste recycling; surface-atmospheric interaction processes (natural and anthropogenic emissions, vertical transport, deposition, and physical-chemical interaction) of gases and aerosols; phytoremediation/restoration of contaminated sites; food contamination and safety; environmental effects of medicines; effects and toxicity of mixed pollutants; speciation of heavy metals/metalloids; effects of mining; disturbed geochemistry from human behavior, natural or man-made hazards; particle and nanoparticle toxicology; risk and the vulnerability of populations, etc.
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