IF 6.5 1区 物理与天体物理 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY ACS Photonics Pub Date : 2025-02-28 DOI:10.1021/acsphotonics.4c02516
Antonios Pelekanidis, Fengling Zhang, Kjeld S. E. Eikema, Stefan Witte
{"title":"Generation Dynamics of Broadband Extreme Ultraviolet Vortex Beams","authors":"Antonios Pelekanidis, Fengling Zhang, Kjeld S. E. Eikema, Stefan Witte","doi":"10.1021/acsphotonics.4c02516","DOIUrl":null,"url":null,"abstract":"Light beams carrying orbital angular momentum (OAM) can be generated in the extreme ultraviolet and soft X-ray spectra by means of high harmonic generation (HHG). In HHG, phase properties of the drive laser, such as curvature, aberrations, and topological charge, are upconverted to the harmonic beams and coherently added to the inherent dipole phase. The strong nonlinearity of the HHG process, combined with the rapid phase variations corresponding to large OAM values in these vortex beams, leads to a high sensitivity to small variations in the driving field. However, a study of the generation dynamics via an accurate reconstruction of multiwavelength OAM beams is challenging. Here we show full complex field measurements of multiple individual harmonics of the HHG vortex beams. By using spectrally resolved ptychographic wavefront sensing, we retrieve the high-resolution amplitude and phase profiles for harmonics 23 to 29 in parallel, enabling detailed multiwavelength beam reconstructions. We study the influence of generation conditions and drive laser aberrations on the resulting vortex fields by comparing measured fields to numerical simulations and retrieving the propagation conditions around the focus and the OAM content of the beams. Specifically, we find that the multimodal content of such vortex beams can significantly influence the propagation and field distributions in the focal region. Such a beam propagation analysis allows a prediction of the resulting attosecond pulse trains and associated attosecond light springs that can be generated under realistic driving conditions.","PeriodicalId":23,"journal":{"name":"ACS Photonics","volume":"28 1","pages":""},"PeriodicalIF":6.5000,"publicationDate":"2025-02-28","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"ACS Photonics","FirstCategoryId":"101","ListUrlMain":"https://doi.org/10.1021/acsphotonics.4c02516","RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"MATERIALS SCIENCE, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0

摘要

通过高次谐波发生(HHG)技术,可以在极紫外和软 X 射线光谱中产生携带轨道角动量(OAM)的光束。在高次谐波发生(HHG)中,驱动激光器的相位特性,如曲率、畸变和拓扑电荷,被上转换为谐波束,并与固有偶极相位相干。HHG 过程具有很强的非线性,再加上这些涡旋光束中与大 OAM 值相对应的快速相位变化,因此对驱动场的微小变化非常敏感。然而,通过精确重建多波长 OAM 波束来研究生成动力学是一项挑战。在这里,我们展示了对 HHG 涡旋束的多个单独谐波的全复场测量。通过使用光谱分辨双色波前传感技术,我们平行地检索到了 23 至 29 次谐波的高分辨率振幅和相位剖面,从而实现了详细的多波长光束重建。通过将测量的场与数值模拟进行比较,并检索焦点周围的传播条件和光束的 OAM 含量,我们研究了产生条件和驱动激光畸变对所产生的涡旋场的影响。具体来说,我们发现这种涡旋光束的多模态含量会显著影响焦点区域的传播和场分布。通过这种光束传播分析,可以预测在实际驱动条件下产生的阿秒脉冲串和相关阿秒光泉。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

摘要图片

查看原文
分享 分享
微信好友 朋友圈 QQ好友 复制链接
本刊更多论文
Generation Dynamics of Broadband Extreme Ultraviolet Vortex Beams
Light beams carrying orbital angular momentum (OAM) can be generated in the extreme ultraviolet and soft X-ray spectra by means of high harmonic generation (HHG). In HHG, phase properties of the drive laser, such as curvature, aberrations, and topological charge, are upconverted to the harmonic beams and coherently added to the inherent dipole phase. The strong nonlinearity of the HHG process, combined with the rapid phase variations corresponding to large OAM values in these vortex beams, leads to a high sensitivity to small variations in the driving field. However, a study of the generation dynamics via an accurate reconstruction of multiwavelength OAM beams is challenging. Here we show full complex field measurements of multiple individual harmonics of the HHG vortex beams. By using spectrally resolved ptychographic wavefront sensing, we retrieve the high-resolution amplitude and phase profiles for harmonics 23 to 29 in parallel, enabling detailed multiwavelength beam reconstructions. We study the influence of generation conditions and drive laser aberrations on the resulting vortex fields by comparing measured fields to numerical simulations and retrieving the propagation conditions around the focus and the OAM content of the beams. Specifically, we find that the multimodal content of such vortex beams can significantly influence the propagation and field distributions in the focal region. Such a beam propagation analysis allows a prediction of the resulting attosecond pulse trains and associated attosecond light springs that can be generated under realistic driving conditions.
求助全文
通过发布文献求助,成功后即可免费获取论文全文。 去求助
来源期刊
ACS Photonics
ACS Photonics NANOSCIENCE & NANOTECHNOLOGY-MATERIALS SCIENCE, MULTIDISCIPLINARY
CiteScore
11.90
自引率
5.70%
发文量
438
审稿时长
2.3 months
期刊介绍: Published as soon as accepted and summarized in monthly issues, ACS Photonics will publish Research Articles, Letters, Perspectives, and Reviews, to encompass the full scope of published research in this field.
期刊最新文献
Flat-Band Lasing in Silicon Waveguide-Integrated Metasurfaces Ultracompact Programmable Silicon Photonics Using Layers of Low-Loss Phase-Change Material Sb2Se3 of Increasing Thickness Coherent Spin Dynamics of Electrons and Holes Photogenerated with Large Kinetic Energy in Lead Halide Perovskite Crystals Opportunities and Challenges in Quantum-Enhanced Optical Target Detection Distinctness of Electroluminescence and Optical Gain in Laser Diodes with Wide Polar Quantum Wells
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
现在去查看 取消
×
提示
确定
0
微信
客服QQ
Book学术公众号 扫码关注我们
反馈
×
意见反馈
请填写您的意见或建议
请填写您的手机或邮箱
已复制链接
已复制链接
快去分享给好友吧!
我知道了
×
扫码分享
扫码分享
Book学术官方微信
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术
文献互助 智能选刊 最新文献 互助须知 联系我们:info@booksci.cn
Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。
Copyright © 2023 Book学术 All rights reserved.
ghs 京公网安备 11010802042870号 京ICP备2023020795号-1