基于层流的平面微流控燃料电池

IF 8.1 2区 工程技术 Q1 CHEMISTRY, PHYSICAL Journal of Power Sources Pub Date : 2017-05-31 DOI:10.1016/j.jpowsour.2017.03.102
Seoung Hwan Lee, Yoomin Ahn
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引用次数: 27

摘要

微流控燃料电池的功率密度仍然不够高,不足以应用于电源。在这项研究中,我们提出了一种新的平面堆来提高微流体燃料电池的总功率。通过使用多个层流,在一个通道内进行串行或并联的电气连接。采用铂电极的平面结构,便于与其他平面微器件集成。这些结构是通过薄膜工艺的微机械加工制成的。用甲酸基燃料实验测量了燃料电池的性能和总欧姆电阻。结果表明,与燃料电池阵列相比,所提出的单堆能以相对较小的总欧姆电阻提供更高的功率密度,并且所需的空间更小。在300 μL min−1流速下,并联和串行电连接分别提高了97.5%和39.3%的峰值体积功率密度。利用这种单一堆叠,我们相信微流体燃料电池可以集成到一个紧凑的平面结构中,以获得足够高的能量,用于能源应用。
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A laminar flow-based single stack of flow-over planar microfluidic fuel cells

Power densities of microfluidic fuel cells are still not high enough for power source applications. In this study, we propose a novel planar stack to increase the total power of a microfluidic fuel cell. Electrical connections in serial or parallel are made within one channel by using multiple laminar flow. A planar structure with flow-over electrodes of platinum are adopted for easy integration with other planar micro devices. These structures are made by micromachining with a thin film process. Fuel cell performance and total ohmic resistances are measured experimentally with a formic acid-based fuel. The results show that the proposed single stacks provide more power density with a comparatively small total ohmic resistance and require less space than that of the fuel cell arrays. The peak volumetric power density improves by 97.5% and 39.3% using parallel and serial electrical connections, respectively, at a 300 μL min−1 flow rate. Utilizing this single stack, we believe that microfluidic fuel cells can be integrated into a compact planar configuration to achieve a power high enough for energy source applications.

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来源期刊
Journal of Power Sources
Journal of Power Sources 工程技术-电化学
CiteScore
16.40
自引率
6.50%
发文量
1249
审稿时长
36 days
期刊介绍: The Journal of Power Sources is a publication catering to researchers and technologists interested in various aspects of the science, technology, and applications of electrochemical power sources. It covers original research and reviews on primary and secondary batteries, fuel cells, supercapacitors, and photo-electrochemical cells. Topics considered include the research, development and applications of nanomaterials and novel componentry for these devices. Examples of applications of these electrochemical power sources include: • Portable electronics • Electric and Hybrid Electric Vehicles • Uninterruptible Power Supply (UPS) systems • Storage of renewable energy • Satellites and deep space probes • Boats and ships, drones and aircrafts • Wearable energy storage systems
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