Dual-Mode Stretchable Emitter with Programmable Emissivity and Air Permeability

IF 8.3 2区 材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY ACS Applied Materials & Interfaces Pub Date : 2024-11-05 DOI:10.1021/acsami.4c1506810.1021/acsami.4c15068
Yinhyui Joo, Dongkyun Kang and Myeongkyu Lee*, 
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Abstract

Materials with anisotropic emission characteristics have attracted considerable attention for thermal management. Although many dual-mode emitters have been developed for this purpose in the form of textiles, multilayer films, and photonic structures, multiple functionalities are essential for their versatile applications. Herein, a highly stretchable dual-mode emitter with programmable emissivity and air permeability is presented. The emitter comprises a planar Ge2Sb2Te5 (GST) cavity on one side of a perforated elastomer substrate and an infrared-reflecting metal layer on the other side. With a laser-induced phase transition from amorphous to crystalline GST, the emitter exhibits a large emissivity difference of 0.52 between both sides. The dual-mode emitter remains highly stable without mechanical failure after repeated stretching cycles to a strain of 50%. This air-permeable and stretchable emitter can be attached to any curved surface, including the human body. The GST-side emissivity can be programmed into an arbitrary emissivity pattern using a spatially modulated laser beam, ultimately enabling the printing of mutually independent visible and thermal images in a single emitter. This study provides a promising structure for multispectral optical security as well as thermal management.

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具有可编程发射率和透气性的双模可伸缩发射器
具有各向异性发射特性的材料在热管理方面备受关注。尽管许多双模发射器已经以纺织品、多层薄膜和光子结构的形式被开发出来,但多种功能对于它们的多用途应用至关重要。本文介绍了一种具有可编程发射率和透气性的高度可拉伸双模发射器。该发射器由一个平面 Ge2Sb2Te5(GST)空腔和一个红外反射金属层组成,空腔位于穿孔弹性体基底的一侧,金属层位于另一侧。在激光诱导下,GST 从非晶态转变为晶体态,发射器两侧的发射率相差 0.52。这种双模发射器在反复拉伸至 50%应变后,仍能保持高度稳定,不会出现机械故障。这种透气、可拉伸的发射器可以附着在包括人体在内的任何曲面上。利用空间调制激光束可将 GST 边发射率编程为任意发射率模式,最终在单个发射器中打印出相互独立的可见光和热图像。这项研究为多光谱光学安全和热管理提供了一种前景广阔的结构。
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来源期刊
ACS Applied Materials & Interfaces
ACS Applied Materials & Interfaces 工程技术-材料科学:综合
CiteScore
16.00
自引率
6.30%
发文量
4978
审稿时长
1.8 months
期刊介绍: ACS Applied Materials & Interfaces is a leading interdisciplinary journal that brings together chemists, engineers, physicists, and biologists to explore the development and utilization of newly-discovered materials and interfacial processes for specific applications. Our journal has experienced remarkable growth since its establishment in 2009, both in terms of the number of articles published and the impact of the research showcased. We are proud to foster a truly global community, with the majority of published articles originating from outside the United States, reflecting the rapid growth of applied research worldwide.
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