Understanding Heat Transfer and the Role of Bed Hydrodynamics in High-Temperature Fluidized Beds

IF 3.8 3区 工程技术 Q2 ENGINEERING, CHEMICAL Industrial & Engineering Chemistry Research Pub Date : 2024-12-26 DOI:10.1021/acs.iecr.4c03348
Zeshi Chen, Han Gao, Qingjin Zhang, Ting Li, Liangliang Fu, Guangwen Xu, Dingrong Bai
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Abstract

A comprehensive understanding of heat transfer between the bed and immersed surfaces is critical for successfully designing and operating high-temperature gas–solid fluidized bed reactors. However, the impact of temperature on heat transfer, particularly in beds operating above 1000 °C, remains underexplored. This study investigates heat transfer between a fluidized bed and an immersed vertical surface over a temperature range of 300–1500 °C, with a focus on the relationship between heat transfer and bed hydrodynamics. The results indicate that below 1200 °C, the heat transfer coefficient (h0) increases gradually with temperature, with radiative heat transfer contributing less than 18% to h0. Above 1200 °C, h0 exhibits an exponential increase for Al2O3 and ZrO2 particles, while it decreases for MgO particles due to enhanced interparticle forces from particle softening and agglomeration. At 1500 °C, radiative heat transfer accounts for up to 30% of the total heat transfer. Additionally, smaller particles demonstrate higher h0 but lower radiative contributions than larger particles. Increasing superficial gas velocity significantly reduces h0 below 1200 °C but has minimal impact at higher temperatures. Larger beds reduce wall confinement effects, enhancing particle mixing and subsequently increasing h0. A comparison of the experimental data with predictions from existing correlations reveals their inadequacy across the studied temperature range. To address this, a new empirical correlation is proposed to improve accuracy for predicting heat transfer in high-temperature fluidized beds.

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来源期刊
Industrial & Engineering Chemistry Research
Industrial & Engineering Chemistry Research 工程技术-工程:化工
CiteScore
7.40
自引率
7.10%
发文量
1467
审稿时长
2.8 months
期刊介绍: ndustrial & Engineering Chemistry, with variations in title and format, has been published since 1909 by the American Chemical Society. Industrial & Engineering Chemistry Research is a weekly publication that reports industrial and academic research in the broad fields of applied chemistry and chemical engineering with special focus on fundamentals, processes, and products.
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