Improved Pearson Correlation Coefficient-Based Graph Neural Network for Dynamic Soft Sensor of Polypropylene Industries

IF 3.9 3区 工程技术 Q2 ENGINEERING, CHEMICAL Industrial & Engineering Chemistry Research Pub Date : 2024-12-26 DOI:10.1021/acs.iecr.4c02832
Yongming Han, Xuehai Liu, Chong Guo, Hao Wu, Min Liu, Zhiqiang Geng
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Abstract

Polypropylene is an important product in the chemical industry and also a raw material for packaging bags, masks, and building boards. The melt index (MI) is a key indicator for evaluating the quality and efficiency of the polypropylene production process. Accurate measurement of the MI is beneficial to increase the polypropylene yield and save energy. The polypropylene production process is characterized by strong nonlinearity, obvious dynamic features, and complex structure, so the current soft sensor methods cannot carry out real-time and accurate soft sensor of the MI. In order to fully mine the complex relationship between variables of temporal data and extract the characteristics of time-series space in chemical production processes, this paper proposes a novel dynamic soft sensor method using an improved Pearson correlation coefficient-based graph neural network (GNN) (Pearson-GNN) method. The adjacency matrix is updated through the correlation coefficient of the data, which is integrated into the graph convolution and time sequence convolution modules of GNN to improve the accuracy of the soft sensing. Finally, the performance of the proposed Pearson-GNN is verified in time-series data soft-sensing task on the public air quality data set and actual polypropylene production processes. Compared with the diffusion concurrent recurrent neural networks (DCRNN), the multivariate time-series forecasting with graph neural networks (MTGNN), the spatiotemporal graph convolutional networks (STGCN), and the GNN based on a fully dynamic adjacency matrix without Pearson correlation updates (Fully GNN), the experimental results show that proposed Pearson-GNN is superior to other methods in terms of the mean absolute percentage error, the root-mean-square error, and mean absolute error.

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基于改进Pearson相关系数的图神经网络在聚丙烯工业动态软测量中的应用
聚丙烯是化工领域的重要产品,也是包装袋、口罩、建筑板材的原材料。熔体指数(MI)是评价聚丙烯生产过程质量和效率的关键指标。准确测定聚丙烯产率,有利于提高聚丙烯产率,节约能源。聚丙烯生产过程具有非线性强、动态特征明显、结构复杂等特点,现有的软测量方法无法对化工生产过程进行实时、准确的MI软测量。为了充分挖掘化工生产过程中时间数据变量间的复杂关系,提取化工生产过程的时间序列空间特征,本文提出了一种基于改进的Pearson相关系数图神经网络(Pearson-GNN)的动态软测量方法。通过数据的相关系数更新邻接矩阵,并将其集成到GNN的图卷积和时间序列卷积模块中,以提高软检测的精度。最后,在公共空气质量数据集和实际聚丙烯生产过程的时间序列数据软测量任务中验证了所提出的Pearson-GNN的性能。实验结果表明,与扩散并发递归神经网络(DCRNN)、基于图神经网络的多元时间序列预测(MTGNN)、时空图卷积网络(STGCN)和基于不含Pearson相关更新的完全动态邻边矩阵的GNN (fully GNN)相比,本文提出的Pearson-GNN在平均绝对百分比误差、均方根误差和平均绝对误差方面均优于其他方法。
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来源期刊
Industrial & Engineering Chemistry Research
Industrial & Engineering Chemistry Research 工程技术-工程:化工
CiteScore
7.40
自引率
7.10%
发文量
1467
审稿时长
2.8 months
期刊介绍: ndustrial & Engineering Chemistry, with variations in title and format, has been published since 1909 by the American Chemical Society. Industrial & Engineering Chemistry Research is a weekly publication that reports industrial and academic research in the broad fields of applied chemistry and chemical engineering with special focus on fundamentals, processes, and products.
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